Aluminum/polyether　ether　ketone　(Al/PEEK)　laminates,　valued　for　lightweight　and　corrosion　resistance　in　aerospace　and　transportation,　face　challenges　in　bonding　Al　alloy　and　PEEK　due　to　mismatched　thermal　expansion　and　PEEK＇s　chemical　inertness.　This　study　introduces　a　novel　approach　combining　carbon　nanotube　(CNT)　coating　with　laser　bionic　texturing　inspired　by　natural　structures　(e.g.,　bird　feathers,　butterfly　wings).　AA6060/PEEK　shear　samples　were　fabricated　via　the　hot-pressing,　and　the　effects　of　CNT　areal　density,　laser　linear　spacing,　bionic　textures　and　fractal　number　on　the　shear　strength　were　analyzed.　Techniques　such　as　SEM,　Raman　spectroscopy,　and　X-ray　photoelectron　spectroscopy　were　employed　to　investigate　the　underlying　mechanisms　further.　The　results　demonstrate　that　the　shear　strength　of　wave-textured　samples　with　optimized　CNT　areal　density　and　fractal　number　is　about　twice　as　high　as　that　of　linear-textured　samples　without　CNTs.　Notably,　the　interface　delamination　shifts　to　AA6060　matrix　failure,　confirming　robust　bonding.　The　results　also　indicated　that　the　enhanced　mechanisms　of　this　method　include　the　micro-nano　mechanical　interlocking,　chemical　bond　formation,　and　CNT　bridging　effect　at　the　interface.　This　research　provides　new　insights　into　enhancing　the　Al/PEEK　interfacial　adhesion.　©　2025　Elsevier　Ltd