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学者姓名:浦娴娟
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Abstract :
Novel catalytic silicon carbide membrane filters (SCMFs) are synthesized with Co/Al-layered double hydroxide (Co/Al-LDH)-coated silicon carbide powder. After capsuled in a self-designed membrane shell, the SCMFs are utilized in activating persulphate for aniline degradation. Thermal analysis conducted via TG/DTG/DSC examination shows that the heating treatment is beneficial in elevating the activating ability of SCMFs, and the derived Co3O4 displays superior catalytical efficiency than Co/Al-LDHs precursor. The XRD patterns and SEM images indicate the sheet-like Co/Al-LDHs are uniformly coprecipitated throughout the surface of SCMFs. Within 20 min, around 95% of aniline is eliminated under 0.7 m of flow velocity and 8:1 of persulphate to aniline ratio. Three-dimensional fluorescence and GC chromatography reveal that distinct by-products exist in the early stage of the aniline degradation process between the sintered and non-sintered Co/Al-LDH-coated SCMFs. The integration strategy of Co/Al-LDH coatings and heating treatment endows traditional SCMFs with robust catalytic properties for engineering-oriented applications in wastewater treatment.
Keyword :
aniline degradation aniline degradation Co/Al-LDHs Co/Al-LDHs long-term evaluation long-term evaluation persulphate activation persulphate activation silicon carbide silicon carbide
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GB/T 7714 | Zhang, Yunfei , Shen, Hongmei , Zheng, Wenzheng et al. Co/Al-Layered Double Hydroxide-Modified Silicon Carbide Membrane Filters as Persulphate Activator for Aniline Degradation [J]. | WATER , 2025 , 17 (3) . |
MLA | Zhang, Yunfei et al. "Co/Al-Layered Double Hydroxide-Modified Silicon Carbide Membrane Filters as Persulphate Activator for Aniline Degradation" . | WATER 17 . 3 (2025) . |
APA | Zhang, Yunfei , Shen, Hongmei , Zheng, Wenzheng , Wu, Tong , Pu, Xianjuan , Zhou, Diwen et al. Co/Al-Layered Double Hydroxide-Modified Silicon Carbide Membrane Filters as Persulphate Activator for Aniline Degradation . | WATER , 2025 , 17 (3) . |
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