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学者姓名：钱兴
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Abstract ：
Among many ways that can improve the electrolysis catalysts of seawater, designing the catalyst with hierarchical nanostructure has received extensive attention because it allows a larger surface area and more active sites. In this work, the NC-enveloped CoS/NiS@Cu2S catalyst with multi-level structure was successfully synthesized by using the complex of trithiocyanuric acid and copper as the metal dopant to coat the spherical Co-Ni precursor, and then by a straightforward one-step high-temperature self-vulcanization reaction. Trithiocyanuric acid not only facilitated the sulfurization of metal elements but also served as N and C source coated on the catalyst. This method constructed structure-controllable, multi-level, and yolk-shelled nanostructure in a facile manner, greatly increasing specific surface area, expanded mass transport channels, and enhancing the exposure of active sites. Besides, the coating of N and C elements significantly increased the electrical conductivity and electrochemical activity of the catalyst. As a result, CoS/NiS@Cu2S@NC exhibited excellent hydrogen evolution performance with the small overpotential of 105, 161, and 176 mV at 10 mA cm-2 in alkaline water, simulated alkaline seawater, and alkaline seawater, respectively. The present approach is proposed as an inspirational idea of the design of cobalt-nickel-copper-based multi-level structural nanomaterials as non-platinum electrocatalysts for hydrogen evolution in seawater.
Keyword ：
Alkaline seawater Alkaline seawater CoS/NiS@Cu 2 S@NC CoS/NiS@Cu 2 S@NC Hydrogen evolution reaction Hydrogen evolution reaction Non-platinum electrocatalyst Non-platinum electrocatalyst Transition metal chalcogenide Transition metal chalcogenide Yolk-shelled structure Yolk-shelled structure
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| GB/T 7714 | Guo, Ming , Luo, Ao , Guan, Guoxiang et al. Multi-level structure-controllable NC-enveloped CoS/NiS@Cu2S yolk-shelled nanospheres as Pt-free catalysts for efficient hydrogen evolution in alkaline water/seawater [J]. | FUEL , 2025 , 389 . |
| MLA | Guo, Ming et al. "Multi-level structure-controllable NC-enveloped CoS/NiS@Cu2S yolk-shelled nanospheres as Pt-free catalysts for efficient hydrogen evolution in alkaline water/seawater" . | FUEL 389 (2025) . |
| APA | Guo, Ming , Luo, Ao , Guan, Guoxiang , Qian, Xing , Yi, Ting , Chen, Ming et al. Multi-level structure-controllable NC-enveloped CoS/NiS@Cu2S yolk-shelled nanospheres as Pt-free catalysts for efficient hydrogen evolution in alkaline water/seawater . | FUEL , 2025 , 389 . |
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By a carbon nanotube (CNT) spatially confined metal-catalyzed structural reconstruction, carbon nanofibers (CNFs) with a hollow, hollow-solid, solid graphite core, and CNT shell are prepared using nitrogen heterocycle (NHC) and polycyclic aromatic hydrocarbon (PAH) as carbon sources. The formation mechanism of CNFs with oriented graphene layers and enlarged intergraphene spacing is studied by X-ray diffraction, scanning electron microscopy, transmission electron microscopy, and selected area electron diffraction analysis. It revealed that this one-dimensional nanoconfined metal-catalyzed carbon rearrangement is totally different from the reported spatially localized metal-catalyzed graphitization of electrospun polymer and nanocasted carbohydrate nanofibers, as the graphene orientation, cavity volume, and interlayer distance of CNFs can be controlled by the carbon concentration-related competitive metal-catalyzed tip growth of latitudinal and longitudinal graphene layers from NHC and PAH. The unique CNF structure renders good electronic/ionic conductivity, abundant Li+ storage interlayer gaps, and robust mechanical durability, resulting in outstanding electrochemical properties as anodes in lithium-ion batteries. The optimum CNF anode delivers a stable discharge capacity of 475 mA h g-1 at 0.1 C, an extraordinary rate capability of 303 mA h g-1 at 5 C, and a remarkable long-term cycling stability of 378 mA h g-1 after 600 cycles at 1 C. This 1D nanoconfined metal catalysis synthesis could be useful for the development of efficient CNF anodes in many electrochemical reactions with a potential for industrial applications.
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| GB/T 7714 | Chen, Ming , Zhao, Ming-Yang , Liu, Ke et al. Structural Reconstruction via Carbon Nanotube Spatially Confined Metal Catalysis: A Morphology-Controlled Approach to Convert Polycyclic Aromatic Hydrocarbon into Carbon Nanofibers for Highly Active Anodes in Li-Ion Batteries [J]. | INORGANIC CHEMISTRY , 2025 , 64 (7) : 3594-3607 . |
| MLA | Chen, Ming et al. "Structural Reconstruction via Carbon Nanotube Spatially Confined Metal Catalysis: A Morphology-Controlled Approach to Convert Polycyclic Aromatic Hydrocarbon into Carbon Nanofibers for Highly Active Anodes in Li-Ion Batteries" . | INORGANIC CHEMISTRY 64 . 7 (2025) : 3594-3607 . |
| APA | Chen, Ming , Zhao, Ming-Yang , Liu, Ke , Liu, Feng-Ming , Yuan, Zhong-Yong , Qian, Xing et al. Structural Reconstruction via Carbon Nanotube Spatially Confined Metal Catalysis: A Morphology-Controlled Approach to Convert Polycyclic Aromatic Hydrocarbon into Carbon Nanofibers for Highly Active Anodes in Li-Ion Batteries . | INORGANIC CHEMISTRY , 2025 , 64 (7) , 3594-3607 . |
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Battery lifetime prediction is critical to successfully introducing new products to the market, and a long testing time will affect the promotion of the product. In this paper, The prediction model of battery cycle life composed of cut-off voltages and state of health (SOH) is established based on an inverse power law equation to evaluate the NCM(811)battery. It is found that the capacity is more sensitive to the charge cut-off voltages (CCOV) than to the discharge cut-off voltages (DCOV). The capacity degrades to 67.3 % at 180th cycle in the range of 3-4.4 V, while it is 65.8 % at 380th cycle in the range of 2.5-4.2 V (the normal work voltage of battery is 3-4.2 V). The internal resistance and capacity degradation of the battery is analyzed by the incremental capacity curve and the hybrid pulse power characterization (HPPC) test. The error between prediction and measurement is less than 3 % within 400 cycles, and the model can predict the battery lifetime under different conditions (SOH, voltage). It helps to shorten the test time of new products and optimize the operating conditions of battery.
Keyword ：
Accelerated life test Accelerated life test Capacity degradation Capacity degradation Life prediction model Life prediction model Lithium-ion battery Lithium-ion battery
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| GB/T 7714 | Lei, Pengju , Xiong, Yonglian , Zhang, Chao et al. Life prediction model and performance degradation of lithium-ion battery under different cut-off voltages [J]. | SOLID STATE IONICS , 2025 , 420 . |
| MLA | Lei, Pengju et al. "Life prediction model and performance degradation of lithium-ion battery under different cut-off voltages" . | SOLID STATE IONICS 420 (2025) . |
| APA | Lei, Pengju , Xiong, Yonglian , Zhang, Chao , Yi, Ting , Qian, Xing . Life prediction model and performance degradation of lithium-ion battery under different cut-off voltages . | SOLID STATE IONICS , 2025 , 420 . |
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An available approach to ameliorate the property of electrocatalysts for transition metal selenides (TMSs) is to transform their structure, morphology, and elemental composition, especially for hydrogen evolution reactions (HER), which can be a long-term task. In this work, Ni-Co nanospheres were synthesized by a hydrothermal method, and then in the synchronous processes of selenization and carbonization, it reacted with the peripherally coated melamine-copper complex, which was the reactant between melamine and copper ions. Ultimately, CoSe 2 /NiSe 2 @Cu 2 Se-NC nanospheres with a core-shell structure were synthesized after annealing process. This special structure provided more active attachment sites, enabling CoSe 2 /NiSe 2 @Cu 2 Se-NC to exhibit excellent HER properties under wide-pH range. Especially, in acidic conditions, it had a low initial potential of 41.0 mV, a small Tafel slope value of 48.7 mV dec - 1 , and a long service life. The proposed scheme indicates that a new approach will be added to the synthesis of electrocatalysts based on TMSs.
Keyword ：
Core-shell structure Core-shell structure CoSe2/NiSe2@Cu2Se-NC CoSe2/NiSe2@Cu2Se-NC Hydrogen evolution reaction Hydrogen evolution reaction Non-platinum electrocatalysts Non-platinum electrocatalysts Transition metal selenides Transition metal selenides Wide-pH range Wide-pH range
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| GB/T 7714 | Guo, Ming , Chen, Siyan , Xiong, Yonglian et al. N-doped carbon-enveloped CoSe2/NiSe2@Cu2Se core-shell nanospheres as non-Pt electrocatalysts for enhanced wide-pH hydrogen evolution reactions [J]. | JOURNAL OF ALLOYS AND COMPOUNDS , 2024 , 1001 . |
| MLA | Guo, Ming et al. "N-doped carbon-enveloped CoSe2/NiSe2@Cu2Se core-shell nanospheres as non-Pt electrocatalysts for enhanced wide-pH hydrogen evolution reactions" . | JOURNAL OF ALLOYS AND COMPOUNDS 1001 (2024) . |
| APA | Guo, Ming , Chen, Siyan , Xiong, Yonglian , Chen, Ming , Xia, Juan , Chen, Wenbin et al. N-doped carbon-enveloped CoSe2/NiSe2@Cu2Se core-shell nanospheres as non-Pt electrocatalysts for enhanced wide-pH hydrogen evolution reactions . | JOURNAL OF ALLOYS AND COMPOUNDS , 2024 , 1001 . |
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Among the various non-precious metal catalysts that drive hydrogen evolution reactions (HERs) and dyesensitized solar cells (DSSCs), transition metal selenides (TMSs) stand out due to their unique electronic properties and tunable morphology. Herein, the multicomponent selenide CuSe-Co 3 Se 4 @VSe 2 was successfully synthesized by doping with metal element vanadium and selenization on the copper-cobalt carbonate hydroxide (CuCo-CH) template. CuSe-Co 3 Se 4 @VSe 2 exhibited the dandelion-like cluster structure composed of hollow nanotubes doped with VSe 2 nanoparticles. Due to the unique structure and the synergistic effect of various elements, CuSe-Co 3 Se 4 @VSe 2 showed excellent alkaline HER and DSSC performances. The DSSC based on CuSeCo 3 Se 4 @VSe 2 exhibited an impressive power conversion efficiency (PCE) of 9.64 %, which was much higher than that of Pt (8.39 %). Besides, it possessed a low HER overpotential of 76 mV@10 mA cm-2 and a small Tafel slope of 88.9 mV dec- 1 in 1.0 M KOH.
Keyword ：
Bifunctional catalyst Bifunctional catalyst CuSe-Co3Se4@VSe2 CuSe-Co3Se4@VSe2 Dye-sensitized solar cell Dye-sensitized solar cell Hollow nanotube cluster Hollow nanotube cluster Hydrogen evolution reaction Hydrogen evolution reaction Transition metal selenide Transition metal selenide
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| GB/T 7714 | Qian, Xing , Yu, Hao , Chen, Wenbin et al. Dandelion-like VSe 2-embellished CuSe-Co 3 Se 4 hollow nanotube clusters as bifunctional catalysts for high-performance alkaline hydrogen evolution and solar cells [J]. | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2024 , 675 : 761-771 . |
| MLA | Qian, Xing et al. "Dandelion-like VSe 2-embellished CuSe-Co 3 Se 4 hollow nanotube clusters as bifunctional catalysts for high-performance alkaline hydrogen evolution and solar cells" . | JOURNAL OF COLLOID AND INTERFACE SCIENCE 675 (2024) : 761-771 . |
| APA | Qian, Xing , Yu, Hao , Chen, Wenbin , Wu, Jianhua , Xia, Juan , Chen, Ming et al. Dandelion-like VSe 2-embellished CuSe-Co 3 Se 4 hollow nanotube clusters as bifunctional catalysts for high-performance alkaline hydrogen evolution and solar cells . | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2024 , 675 , 761-771 . |
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Conductive hydrogels have shown a great potential in the field of flexible electronics. However, it is difficult to combine high strength and high toughness in conductive hydrogels prepared by conventional methods, which limits their applications in various fields. In this work, we pioneered a facile and cost-effective strategy to prepare soy protein isolate/poly(vinyl alcohol) (SPI/PVA) conductive hydrogels with high strength, toughness, low- temperature resistance, and recyclability by introducing all the salts into the prescuor solution directly. To solve the problem of unable to directly introducing high concentration Na3Cit into the soy protein isolate/PVA solution, MgCl2 was used to alleviate the strong salting-out effect of Na3Cit. Thus the stable SPI/PVA/EG/MgCl2/ Na3Cit complex solution was obtained and the SPI/PVA/EG/MgCl2/Na3Cit (SPEMS) organohydrogel was prepared by the freezing/thawing process. The optimum tensile strength of the SPEMS organohydrogel was 1.1 +0.07 MPa, and the elongation at break was 701.3+23.67 %, respectively. Meanwhile, the ionic conductivity of the organohydrogel was as high as 1.7+0.01 S/m. Finally, the EG/H2O binary solvent system endowed the organohydrogel with excellent low-temperature resistance (freezing point of-19.4 degrees C). The strain sensors assembled with SPEMS organohydrogels were characterized by high sensitivity (GF = 3.2, strain range from 20 %-500 %) and long-term stability. The flexible all-solid-state supercapacitor assembled with SPEMS organohydrogel as the electrolyte and activated carbon as the electrodes has a high area specific capacitance (113.76 mF/cm2) and good cycling stability (capacitance retention of 81.62 % after 1,000 charging and discharging cycles) at room temperature.
Keyword ：
Hofmeister effect Hofmeister effect One-pot preparation One-pot preparation Poly(vinyl alcohol) Poly(vinyl alcohol) Soy protein isolate Soy protein isolate Strain sensor Strain sensor
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| GB/T 7714 | Hu, Mingqiang , Deng, Yingxue , Qian, Xing et al. One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices [J]. | EUROPEAN POLYMER JOURNAL , 2024 , 221 . |
| MLA | Hu, Mingqiang et al. "One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices" . | EUROPEAN POLYMER JOURNAL 221 (2024) . |
| APA | Hu, Mingqiang , Deng, Yingxue , Qian, Xing , Ye, Dezhan , Jiang, Xiancai , Xiao, Gao . One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices . | EUROPEAN POLYMER JOURNAL , 2024 , 221 . |
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The thermal safety of lithium-ion batteries has garnered significant attention due to its pivotal role in the field of new energy. In this work, a three-dimensional electrochemical-thermal coupling model based on the P2D model was established for predicting the thermal performance. The charge-discharge and temperature rise experiments via 18650 cylindrical Li[Ni0.6Co0.2Mn0.2]O-2 / graphite batteries are designed to confirm the rationality of the model. The simulation results show that the highest temperature of the battery surface during discharging at 1 C and 4 C are 42.85 degrees C and 61.25 degrees C, and the experimental results are 42.50 degrees C and 62.85 degrees C, respectively. The electrode heat generation mainly comes from the reaction heat of cathode and anode during 1 C charge process, the maximum power is 1.2 W and 0.6 W, respectively. In the discharge process, the cathode dominates the reaction contribution of 1.02 W and the reaction heat power from the anode is only 0.016 W. The capacity of heat dissipation can be increased by enhancing the convective heat transfer coefficient and air velocity within a reasonable range. The proposed electrochemical-thermal coupling model is valuable to evaluate the heat behavior and promote the battery development.
Keyword ：
electrochemical-thermal coupling model electrochemical-thermal coupling model electrode heat generation electrode heat generation heat dissipation heat dissipation lithium-ion batteries lithium-ion batteries thermal performance thermal performance
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| GB/T 7714 | Zhang, Chao , Shang, Jin , Xiong, Yonglian et al. Thermal Performance of a Cylindrical Li[Ni0.6Co0.2Mn0.2]O2/Graphite Battery based on the Electrochemical-Thermal Coupling Model [J]. | JOURNAL OF THE ELECTROCHEMICAL SOCIETY , 2024 , 171 (9) . |
| MLA | Zhang, Chao et al. "Thermal Performance of a Cylindrical Li[Ni0.6Co0.2Mn0.2]O2/Graphite Battery based on the Electrochemical-Thermal Coupling Model" . | JOURNAL OF THE ELECTROCHEMICAL SOCIETY 171 . 9 (2024) . |
| APA | Zhang, Chao , Shang, Jin , Xiong, Yonglian , Yi, Ting , Hou, Quanhui , Qian, Xing . Thermal Performance of a Cylindrical Li[Ni0.6Co0.2Mn0.2]O2/Graphite Battery based on the Electrochemical-Thermal Coupling Model . | JOURNAL OF THE ELECTROCHEMICAL SOCIETY , 2024 , 171 (9) . |
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Green energy such as hydrogen energy has broad development prospects in promoting the adjustment of energy structure due to its advantages in cleanliness and efficiency. Hydrogen evolution reaction (HER) for water splitting can be used as a simple and effective avenue for hydrogen production. Platinum (Pt), a noble metal, has shown excellent catalytic performance as a conventional cathode catalyst for HER, but its high price has severely hindered its commercial application. Herein, a hollow nanorod array based Pt-free self-supporting electrode with a unique structure was developed for efficient hydrogen evolution reactions. This electrode was composed of a hollow ordered Ni-CoS2@MoS2 array as the main catalyst and a highly conductive Ti foil as a conducting substrate. In the synthesis process, ammonium tetrathiomolybdate was used as a multifunctional vulcanizing agent. Thanks to the unique structure of the hollow nanorods, the active ingredient was adequately revealed, making it possible to improve catalytic activity. This unique catalyst exhibited excellent HER performance at different pH values. Ni-CoS2@MoS2/Ti electrode exhibited high HER performance in alkaline, acidic, and neutral media, with overpotentials of 153, 192, and 196 mV at 10 mA cm -2 and Tafel slopes of 65.8, 67.8, and 93.3 mV dec-1, respectively.
Keyword ：
Active cite Active cite Hollow nanorod array Hollow nanorod array Hydrogen evolution Hydrogen evolution Water splitting Water splitting Wide pH range Wide pH range
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| GB/T 7714 | Qian, Xing , Wu, Jiashuo , Yang, Yajie et al. Ni-CoS2@MoS2 hollow nanorod array in-situ synthesized on Ti foil as Pt-free self-supporting electrode for efficient wide-pH hydrogen evolution [J]. | APPLIED SURFACE SCIENCE , 2024 , 655 . |
| MLA | Qian, Xing et al. "Ni-CoS2@MoS2 hollow nanorod array in-situ synthesized on Ti foil as Pt-free self-supporting electrode for efficient wide-pH hydrogen evolution" . | APPLIED SURFACE SCIENCE 655 (2024) . |
| APA | Qian, Xing , Wu, Jiashuo , Yang, Yajie , Zhang, Wanting , Zheng, Han , Xia, Juan et al. Ni-CoS2@MoS2 hollow nanorod array in-situ synthesized on Ti foil as Pt-free self-supporting electrode for efficient wide-pH hydrogen evolution . | APPLIED SURFACE SCIENCE , 2024 , 655 . |
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Iron nitrides with the merits of high theoretical capacities, cost-effectiveness, and good electronic/ionic conductivity have been recognized as attractive anode candidates for lithium-ion batteries (LIBs). Carbon compositing, pore engineering, and nanostructure construction have proved to be effective strategies to prepare high-performance metal nitride anodes for LIBs. Herein, we synthesized a series of Fe3N-embedded and N-doped carbon nanorods (Fe3N@NCNR) with a hierarchical porous system and controllable topography by metal-catalyzed graphitization-nitridization of the Fe(III)-triazole framework (Fe-MOF) and thermal evaporation of the triblock copolymer F127 template assembled in Fe-MOF via hydrogen bonding interaction, followed by the air oxidation and urea-assisted ammonolysis processes. The Fe3N@NCNR as anodes for LIBs display extraordinary lithium storage capabilities with a high reversible capacity of 830 mA h g-1 at 0.1 C, a good rate performance of 576 mAh g-1 at 5 C, and a long-term cycling stability of 742 mA h g-1 over 600 cycles at 1 C. Such outstanding performance benefits from the spongy carbon nanorods with rich macropores for rapid electronic/ionic transport and effective accommodation of electrode volume expansion, abundant N-doped meso-/microporous carbon for the additional storage of Li+ via capacitive effect, and the efficient utilization of Fe3N nanoparticles uniformly distributed through carbon nanorods. Importantly, this work introduces an effective strategy to construct superior performance nitride anodes from MOF surfactants based on hydrogen bonding-driven interface self-assembly and provides insight into the preparation of highly efficient nanoarchitectures for Li+ storage.
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| GB/T 7714 | Chen, Ming , Liu, Feng-Ming , Zhao, Ming-Yang et al. Rational Synthesis of Spongy Fe3N@N-Doped Carbon Nanorods with Controlled Topography and Porosity for Enhanced Energy Storage Anodes in Lithium-Ion Batteries [J]. | LANGMUIR , 2024 , 40 (45) : 24017-24028 . |
| MLA | Chen, Ming et al. "Rational Synthesis of Spongy Fe3N@N-Doped Carbon Nanorods with Controlled Topography and Porosity for Enhanced Energy Storage Anodes in Lithium-Ion Batteries" . | LANGMUIR 40 . 45 (2024) : 24017-24028 . |
| APA | Chen, Ming , Liu, Feng-Ming , Zhao, Ming-Yang , Qian, Xing , Liu, Lei , Wan, Rong et al. Rational Synthesis of Spongy Fe3N@N-Doped Carbon Nanorods with Controlled Topography and Porosity for Enhanced Energy Storage Anodes in Lithium-Ion Batteries . | LANGMUIR , 2024 , 40 (45) , 24017-24028 . |
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At present, the exploration of renewable energy is a huge challenge, and water electrolysis is regarded as a promising method for producing hydrogen. However, the hydrogen evolution reaction (HER) has been hampered due to expensive Pt-based catalysts. Herein, the Fe 2 P-coated Ni 2 P/Co 2 P nanospheres with yolk-shelled structure were successfully synthesized according to a facile approach of doping transition metal elements and phosphating on the template Ni -Co nanospheres, successively. All samples were tested as HER catalysts at various pH environments. The results showed that the Fe 2 P-Ni 2 P/Co 2 P possesses superior electrocatalytic ability and good stability. The Fe 2 P-Ni 2 P/Co 2 P achieved the lower eta onset (overpotential at 1.0 mA cm -2 ) of 36.6, 64.2, and 65.9 mV, eta 10 (overpotential at 10 mA cm -2 ) of 89.7, 125, and 212 mV, and Tafel slopes of 48.0, 60.3, and 135 mV dec - 1 in acidic, alkaline, and neutral solutions, respectively, exhibiting an excellent electrocatalytic activity of the multicomponent phosphides for HER.
Keyword ：
Fe2P-Ni2P/Co2P Fe2P-Ni2P/Co2P Hydrogen evolution reaction Hydrogen evolution reaction Multicomponent material Multicomponent material Transition metal phosphide Transition metal phosphide Water electrolysis Water electrolysis Yolk-shelled structure Yolk-shelled structure
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| GB/T 7714 | Chen, Wenbin , Chen, Siyan , Guo, Ming et al. Fe2 P-coated Ni2 P/Co2 P yolk-shelled porous nanospheres as advanced Pt-free electrocatalysts for efficient pH-universal hydrogen evolution [J]. | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2024 , 78 : 851-860 . |
| MLA | Chen, Wenbin et al. "Fe2 P-coated Ni2 P/Co2 P yolk-shelled porous nanospheres as advanced Pt-free electrocatalysts for efficient pH-universal hydrogen evolution" . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 78 (2024) : 851-860 . |
| APA | Chen, Wenbin , Chen, Siyan , Guo, Ming , Jiang, Xiancai , Xia, Juan , Chen, Ming et al. Fe2 P-coated Ni2 P/Co2 P yolk-shelled porous nanospheres as advanced Pt-free electrocatalysts for efficient pH-universal hydrogen evolution . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2024 , 78 , 851-860 . |
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