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学者姓名：吴明红
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Abstract ：
Efficient phosphate adsorption from eutrophic waters remains challenging, fundamentally due to inherent tradeoff in common adsorbents: high-binding energy between adsorbent and phosphate compromises reusability while low-binding energy suppresses selectivity. Herein, an innovative arginine-functionalized imprinted aerogel (AFIA-1:4) was fabricated by click chemistry and imprinting modification for overcoming this trade-off through synergistic weak interactions. Results shown that AFIA-1:4 exhibited high adsorption capacity (Qmax of 40.65 mg/g, 30.44 % higher than phoslock), rapid kinetics (15 min), and broad pH applicability (3-11) at 2 mg P/L solution. Moreover, its selectivity coefficient ranged from 10 to 90 even with 15- to 125-fold excess interfering anions, surpassing common adsorbents. After 10 cycles, AFIA-1:4 still maintained 98.15 % regeneration rate with 99.14 % phosphate desorption. Characterizations and calculations confirmed core roles of multiple hydrogen bonds and shape screening in maintaining selectivity and reusability. These findings advanced development of next-generation of phosphate adsorbents, which contributed to sustainable prevention and management of eutrophication.
Keyword ：
Click chemistry Click chemistry Imprinting modification Imprinting modification Multiple hydrogen bonds Multiple hydrogen bonds Novel phosphate adsorbent Novel phosphate adsorbent Shape screening Shape screening Trade-off Trade-off
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| GB/T 7714 | Feng, Lidong , Leng, Tianxiao , Qiu, Yangbo et al. Weak interaction strategy enables enhanced selectivity and reusability of arginine-functionalized imprinted aerogel for phosphate adsorption [J]. | BIORESOURCE TECHNOLOGY , 2025 , 418 . |
| MLA | Feng, Lidong et al. "Weak interaction strategy enables enhanced selectivity and reusability of arginine-functionalized imprinted aerogel for phosphate adsorption" . | BIORESOURCE TECHNOLOGY 418 (2025) . |
| APA | Feng, Lidong , Leng, Tianxiao , Qiu, Yangbo , Wang, Chao , Ren, Long-Fei , Sun, Haoyu et al. Weak interaction strategy enables enhanced selectivity and reusability of arginine-functionalized imprinted aerogel for phosphate adsorption . | BIORESOURCE TECHNOLOGY , 2025 , 418 . |
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With the increasing demand for sustainable and resource-efficient wastewater treatment technologies, particularly in addressing metal-organic complexes contamination, herein we present a photoelectrochemical (PEC) wastewater treatment system based on a solar-driven ion confinement strategy. Employing a coordination polymer framework known as copper hexacyanoferrate (CuFe Prussian blue analogues (PBA)) as the host material for ion confinement, our strategy creates a pathway that couples photogenerated electrons with heavy-metal ions. This facilitates rapid electron transfer, enabling the effective separation of charge carriers and simultaneous capture of Cu(II) from wastewater. Taking Cu-ethylenediaminetetraacetic acid (EDTA) as a model pollutant, our proposed method demonstrates a removal efficiency of 92.2% for Cu-EDTA complexes and a recovery rate of 76.5% for Cu(II) under unbiased conditions. Analysis using X-ray absorption fine structure (XAFS) confirms the ion confinement of Cu(II) within the structure, distinguishing it from traditional PEC methods that focus on obtaining elemental Cu(0). Controlled release of metal ions not only meets specific requirements but also has significant potential for chemical recovery. Our proposed technology embodies the concept of utilizing pollutants to treat pollutants, making full use of concomitant heavy-metal ions in wastewater. It concurrently achieves the efficient degradation of organic pollutants while also facilitating resource recovery. © 2024 American Chemical Society
Keyword ：
Cu-EDTA Cu-EDTA decomplexation decomplexation ion confinement ion confinement photoelectrochemical photoelectrochemical Prussian blue analogues Prussian blue analogues
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| GB/T 7714 | Dang, Q. , Wang, L. , Sun, W. et al. Solar-Driven Ion Confinement for Synergetic Pollutants Remediation and Valuable Metal Recovery in Wastewater [J]. | ACS ES and T Engineering , 2024 , 4 (7) : 1748-1757 . |
| MLA | Dang, Q. et al. "Solar-Driven Ion Confinement for Synergetic Pollutants Remediation and Valuable Metal Recovery in Wastewater" . | ACS ES and T Engineering 4 . 7 (2024) : 1748-1757 . |
| APA | Dang, Q. , Wang, L. , Sun, W. , Wu, G. , Li, S. , Li, A. et al. Solar-Driven Ion Confinement for Synergetic Pollutants Remediation and Valuable Metal Recovery in Wastewater . | ACS ES and T Engineering , 2024 , 4 (7) , 1748-1757 . |
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Transition metal selenides are considered as one of the most promising anode materials for sodium-ion batteries (SIBs) on account of their high theoretical specific capacity. However, the poor conductivity, sluggish kinetics and volume expansion during the (de)sodiation process hinder its application. Herein, a novel heterostructure of CoSe2/Sb2Se3 nanocrystals embedded into nanocage-in-nanofiber carbon framework is designed and constructed via electrospinning, carbonization, ion exchange and selenization processes. In this structure, bimetallic selenide heterostructure accelerates electron/ion transfer kinetics and Na+ adsorption capacity, carbon nanocages structure alleviates the volume expansion and maintains structural integrity during the (de)sodiation process, and carbon nanofibers connect the nanocages in series to shorten the electron transmission path and enhance electrical conductivity. As a self-supporting anode for SIBs, as-synthesized CoSe2/Sb2Se3@C@CNF shows a high reversible capacity of 406 mAh g-1 at 0.2 A g-1 after 200 cycles and displays excellent rate capability. More remarkably, the CoSe2/Sb2Se3@C@CNF anode manifests an outstanding cycling stability for over 2000 and 12,000 cycles at 1 and 5 A g-1, with the capacity retention being 97 % and 103 % respectively. Meanwhile, the excellent sodium storage performance is revealed by kinetic analysis, energy level analysis and density functional theory calculations.
Keyword ：
CoSe2 CoSe2 Heterostructure Heterostructure Nanocage Nanocage Nanofiber Nanofiber Sb2Se3 Sb2Se3 Sodium-ion battery Sodium-ion battery Ultralong-life Ultralong-life
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| GB/T 7714 | Li, Yunbiao , Gao, Xinglong , Zhang, Long et al. Heterostructure CoSe2/Sb2Se3 nanocrystals embedded into nanocage-in-nanofiber carbon framework for ultralong-life sodium-ion batteries [J]. | JOURNAL OF ALLOYS AND COMPOUNDS , 2024 , 999 . |
| MLA | Li, Yunbiao et al. "Heterostructure CoSe2/Sb2Se3 nanocrystals embedded into nanocage-in-nanofiber carbon framework for ultralong-life sodium-ion batteries" . | JOURNAL OF ALLOYS AND COMPOUNDS 999 (2024) . |
| APA | Li, Yunbiao , Gao, Xinglong , Zhang, Long , Wei, Mingzhi , Jiang, Chaoyan , Li, Zhen et al. Heterostructure CoSe2/Sb2Se3 nanocrystals embedded into nanocage-in-nanofiber carbon framework for ultralong-life sodium-ion batteries . | JOURNAL OF ALLOYS AND COMPOUNDS , 2024 , 999 . |
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Antibiotics usually induce the hormetic effects on bacteria, featured by low-dose stimulation and high-dose inhibition, which challenges the central belief in toxicity assessment and environmental risk assessment of antibiotics. However, there are currently no ideal parameters to quantitatively characterize hormesis. In this study, an effective area in hormesis (AH) was developed to quantify the biphasic dose-responses of single antibiotics (sulfonamides (SAs), sulfonamides potentiators (SAPs), and tetracyclines (TCs)) and binary mixtures (SAs-SAPs, SAs-TCs, and SAs-SAs) to the bioluminescence of Aliivibrio fischeri. Using Ebind (the lowest interaction energy between antibiotic and target protein) and Kow (octanol-water partition coefficient) as the structural descriptors, the reliable quantitative structure-activity relationship (QSAR) models were constructed for the AH values of test antibiotics and mixtures. Furthermore, a novel method based on AH was established to judge the joint toxic actions of binary antibiotics, which mainly exhibited synergism. The results also indicated that SAPs (or TCs) contributed more than SAs in the hormetic effects of antibiotic mixtures. This study proposes a new quantitative parameter for characterizing and predicting antibiotic hormesis, and considers hormesis as an integrated whole to reveal the combined effects of antibiotics, which will promote the development of risk evaluation for antibiotics and their mixtures. © 2024 Elsevier B.V.
Keyword ：
Antibiotics Antibiotics Hormesis Hormesis Joint toxic action Joint toxic action QSAR QSAR Quantitative characterization Quantitative characterization
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| GB/T 7714 | Sun, H. , Yao, J. , Long, Z. et al. A new parameter for quantitatively characterizing antibiotic hormesis: QSAR construction and joint toxic action judgment [J]. | Journal of Hazardous Materials , 2024 , 479 . |
| MLA | Sun, H. et al. "A new parameter for quantitatively characterizing antibiotic hormesis: QSAR construction and joint toxic action judgment" . | Journal of Hazardous Materials 479 (2024) . |
| APA | Sun, H. , Yao, J. , Long, Z. , Luo, R. , Wang, J. , Liu, S.-S. et al. A new parameter for quantitatively characterizing antibiotic hormesis: QSAR construction and joint toxic action judgment . | Journal of Hazardous Materials , 2024 , 479 . |
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Zinc selenide (ZnSe) is a next-generation anode material due to its high sodium storage capacity. However, the poor conductivity and volume expansion lead to its capacity attenuation and short cycle life. Herein, Se-vacancy porous ultrathin ZnSe nanosheet/carbon composite (ZnSe@NC/N-GQD) is reported as a high-performance anode material for sodium-ion batteries. Organic-inorganic hybrid ZnSe(en)0.5 ultrathin nanosheets with abundant Se vacancies are rapidly prepared by electron beam irradiation for the first time. Using it as a precursor, Se-vacancy carbon-coated porous ultrathin ZnSe nanosheets loaded with nitrogen-doped graphene quantum dots (N-GQDs) are synthesized via carbonization and electrodeposition process. Through the design of ZnSe@NC/N-GQD, the sodium storage performance can be effectively improved by implementing nanostructure engineering (porous ultrathin nanosheet) via organic–inorganic hybrid, defect engineering (Se vacancy) via electron beam irradiation, and carbon composite (amorphous carbon and N-GQD). Consequently, ZnSe@NC/N-GQD delivers a high capacity of 483 mA h g−1 after 200 cycles at 0.5 A g−1, shows an outstanding rate capability of 381 mA h g−1 at 10.0 A g−1, and exhibits an excellent cycling stability of 86 % retention after 2800 cycles at 5.0 A g−1. This work develops a new method to rapidly prepare organic–inorganic nanohybrids, and proposes an innovative design of high-performance ZnSe-based anodes. © 2024 Elsevier B.V.
Keyword ：
Electron beam irradiation Electron beam irradiation Organic–inorganic hybrid Organic–inorganic hybrid Porous ultrathin nanosheets Porous ultrathin nanosheets Se vacancy Se vacancy Sodium storage Sodium storage Zinc selenide Zinc selenide
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| GB/T 7714 | Jiang, C. , Zhang, L. , Gao, X. et al. Se-vacancy porous ultrathin ZnSe nanosheet/carbon composite for sodium storage via electron beam irradiation strategy [J]. | Chemical Engineering Journal , 2024 , 497 . |
| MLA | Jiang, C. et al. "Se-vacancy porous ultrathin ZnSe nanosheet/carbon composite for sodium storage via electron beam irradiation strategy" . | Chemical Engineering Journal 497 (2024) . |
| APA | Jiang, C. , Zhang, L. , Gao, X. , Yu, W. , Hu, C. , Tang, W. et al. Se-vacancy porous ultrathin ZnSe nanosheet/carbon composite for sodium storage via electron beam irradiation strategy . | Chemical Engineering Journal , 2024 , 497 . |
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With the increasing severity of the plastic pollution issue, biodegradable plastics are considered a critical approach to addressing plastic pollution. However, the aging process of biodegradable plastics and the resulting microplastics adsorption of pollutants in the environment are not clearly understood. This study investigated the physicochemical property changes of different microplastics (Biodegradable microplastics and non-biodegradable microplastics) during aging, examined the adsorption processes and mechanisms of biodegradable plastics and non-degradable plastics towards typical pollutants in the environment, and elucidated the different aging mechanisms and adsorption mechanisms of biodegradable plastics and non-biodegradable plastics. The experimental results indicated that compared to non-biodegradable microplastics, biodegradable microplastics are more prone to aging in the environment, forming smaller microplastic particles and easier adsorption of environmental pollutants. Biodegradable microplastics have abundant oxygen-containing functional groups on the surface, which enhance age biodegradable microplastics adsorption capacity for pollutants through electrostatic interactions, chelation, and hydrogen bonding. The experimental results show that a strong oxidation system has unique advantages in the aging removal of biodegradable microplastics and can effectively reduce the adsorption equilibrium capacity of biodegradable microplastics. This research contributes to a deeper understanding of biodegradable microplastics’ aging and adsorption behaviors in the environment, highlighting their significant role as carriers of pollutants. © 2024 Elsevier B.V.
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| GB/T 7714 | Lei, Chen , Chengkai, Mao , Shanning, Yuan et al. Comparison of aging behavior and adsorption processes of biodegradable and conventional microplastics [J]. | Chemical Engineering Journal , 2024 , 502 . |
| MLA | Lei, Chen et al. "Comparison of aging behavior and adsorption processes of biodegradable and conventional microplastics" . | Chemical Engineering Journal 502 (2024) . |
| APA | Lei, Chen , Chengkai, Mao , Shanning, Yuan , Xianjuan, Pu , Huanhuan, Liang , Xiangyu, Chen et al. Comparison of aging behavior and adsorption processes of biodegradable and conventional microplastics . | Chemical Engineering Journal , 2024 , 502 . |
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The widespread utilization of noble metal-based catalysts for the oxygen evolution reaction (OER) is hindered by their rarity and substantial expense, posing significant challenges for large-scale applications. Therefore, developing an efficient OER electrocatalyst for proton exchange membrane (PEM) water electrolyzers remains a significant challenge. Here, we present a bottom-up synthesis strategy utilizing ultrasound-assisted exfoliation to design nickel-iron bimetallic organic framework (NiFe-MOF) nanosheets with high electrooxidation activity, in situ induced by carbon quantum dots (CQDs). This approach eliminates the reliance on intricate and inefficient exfoliation techniques, producing NiFe-MOF nanosheets with a regulated thickness of just 10 nm. This enhanced electron transport induced by CQDs plays a pivotal role in improving the OER performance of NiFe-MOF, achieving a current density of 10 mA cm-2 with an overpotential of only 280 mV, with a Tafel slope of 71.98 mV dec-1, lower Rct, and larger ECSA. In situ FTIR spectroscopy suggests that the OER mechanism in NiFe-MOF-CQD mainly follows the adsorbate evolution mechanism. The NiFe-MOF-CQD catalyst demonstrates remarkable durability and resilience during PEM water electrolysis, reaching industrially relevant current densities of 2 A cm-2 at 2 V. This research's results not only promote green and low-carbon development but also inject new vitality into the development of hydrogen energy technologies.
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| GB/T 7714 | Ni, Qianjia , Zhang, Shiyuan , Wang, Kang et al. Carbon quantum dot-mediated binary metal-organic framework nanosheets for efficient oxygen evolution at ampere-level current densities in proton exchange membrane electrolyzers [J]. | JOURNAL OF MATERIALS CHEMISTRY A , 2024 , 12 (45) : 31253-31261 . |
| MLA | Ni, Qianjia et al. "Carbon quantum dot-mediated binary metal-organic framework nanosheets for efficient oxygen evolution at ampere-level current densities in proton exchange membrane electrolyzers" . | JOURNAL OF MATERIALS CHEMISTRY A 12 . 45 (2024) : 31253-31261 . |
| APA | Ni, Qianjia , Zhang, Shiyuan , Wang, Kang , Guo, Huazhang , Zhang, Jiye , Wu, Minghong et al. Carbon quantum dot-mediated binary metal-organic framework nanosheets for efficient oxygen evolution at ampere-level current densities in proton exchange membrane electrolyzers . | JOURNAL OF MATERIALS CHEMISTRY A , 2024 , 12 (45) , 31253-31261 . |
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A large amount of antibiotics enters the soil environment and accumulates therein as individuals and mixtures, threatening the soil safety. However, there is little information regarding the influence of single and mixed antibiotics on key soil proteins at molecular level. In this study, setting sulfadiazine (SD) and tetracycline hydrochloride (TC) as the representative antibiotics, the interactions between these agents and α-amylase (an important hydrolase in soil carbon cycle) were investigated through multi-spectroscopic approaches, X-ray photoelectron spectrometry, and molecular modeling. It was found that both SD and TC spontaneously bound to α-amylase with 1:1 stoichiometry mainly via forming stable chemical bonds. The interactions altered the polarity of aromatic amino acids, protein backbone, secondary structure, hydrophobicity and activity of α-amylase. The SD-TC mixtures were designed based on the direct equipartition ray to comprehensively characterize the possible concentration distribution, and interactive effects indicated that the mixtures antagonistically impacted α-amylase. These findings reveal the binding characteristics between α-amylase and typical antibiotics, which probably influence the ecological functions of α-amylase in soil. This study clarifies the potential harm of antibiotics on soil functional enzyme, which is significant for the environmental risk assessment of antibiotics and their mixtures. © 2024 Elsevier B.V.
Keyword ：
Bond strength (chemical) Bond strength (chemical) Risk assessment Risk assessment
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| GB/T 7714 | Zhang, Yulian , Xu, Fangyu , Yao, Jingyi et al. Spontaneous interactions between typical antibiotics and soil enzyme: Insights from multi-spectroscopic approaches, XPS technology, molecular modeling, and joint toxic actions [J]. | Journal of Hazardous Materials , 2024 , 480 . |
| MLA | Zhang, Yulian et al. "Spontaneous interactions between typical antibiotics and soil enzyme: Insights from multi-spectroscopic approaches, XPS technology, molecular modeling, and joint toxic actions" . | Journal of Hazardous Materials 480 (2024) . |
| APA | Zhang, Yulian , Xu, Fangyu , Yao, Jingyi , Liu, Shu-Shen , Lei, Bo , Tang, Liang et al. Spontaneous interactions between typical antibiotics and soil enzyme: Insights from multi-spectroscopic approaches, XPS technology, molecular modeling, and joint toxic actions . | Journal of Hazardous Materials , 2024 , 480 . |
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With the increasing severity of the plastic pollution issue, biodegradable plastics are considered a critical approach to addressing plastic pollution. However, the aging process of biodegradable plastics and the resulting microplastics adsorption of pollutants in the environment are not clearly understood. This study investigated the physicochemical property changes of different microplastics (Biodegradable microplastics and nonbiodegradable microplastics) during aging, examined the adsorption processes and mechanisms of biodegradable plastics and non-degradable plastics towards typical pollutants in the environment, and elucidated the different aging mechanisms and adsorption mechanisms of biodegradable plastics and non-biodegradable plastics. The experimental results indicated that compared to non-biodegradable microplastics, biodegradable microplastics are more prone to aging in the environment, forming smaller microplastic particles and easier adsorption of environmental pollutants. Biodegradable microplastics have abundant oxygen-containing functional groups on the surface, which enhance age biodegradable microplastics adsorption capacity for pollutants through electrostatic interactions, chelation, and hydrogen bonding. The experimental results show that a strong oxidation system has unique advantages in the aging removal of biodegradable microplastics and can effectively reduce the adsorption equilibrium capacity of biodegradable microplastics. This research contributes to a deeper understanding of biodegradable microplastics' aging and adsorption behaviors in the environment, highlighting their significant role as carriers of pollutants.
Keyword ：
Adsorption mechanism Adsorption mechanism Biodegradable microplastics Biodegradable microplastics Novel aging process Novel aging process Oxygen-containing functional groups Oxygen-containing functional groups
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| GB/T 7714 | Chen, Lei , Mao, Chengkai , Yuan, Shanning et al. Comparison of aging behavior and adsorption processes of biodegradable and conventional microplastics [J]. | CHEMICAL ENGINEERING JOURNAL , 2024 , 502 . |
| MLA | Chen, Lei et al. "Comparison of aging behavior and adsorption processes of biodegradable and conventional microplastics" . | CHEMICAL ENGINEERING JOURNAL 502 (2024) . |
| APA | Chen, Lei , Mao, Chengkai , Yuan, Shanning , Pu, Xianjuan , Liang, Huanhuan , Chen, Xiangyu et al. Comparison of aging behavior and adsorption processes of biodegradable and conventional microplastics . | CHEMICAL ENGINEERING JOURNAL , 2024 , 502 . |
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Environmental engineering is confronted with new challenges and prospects. It necessitates a shift in the paradigm of scientific research, and transcending the disciplinary confinement of end-management as the primary objective. This shift is crucial for enabling environmental engineering to play a more pivotal role in addressing global ecological and environmental challenges. On the other hand, artificial intelligence (AI) stands as one of today's innovative technologies, with its application in environmental engineering marking a pivotal direction for future innovation. This study employed bibliometric methods to sift through an extensive collection of over 24 000 papers related to AI and environmental engineering, spanning from 1990 to 2023. It analyzed the prominent institutions globally involved in this field, illustrated the current research directions of AI in environmental engineering, and discussed the evolution and future trends of research hotspots. Additionally, the potential challenges were also raised. Consequently, this study aims to provide suggestions and insights for the research and development of AI in environmental engineering, facilitating the rapid advancement of China's environmental engineering disciplines. © 2024 Science Press. All rights reserved.
Keyword ：
artificial intelligence artificial intelligence challenges challenges environmental engineering environmental engineering research directions research directions trend analysis trend analysis
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| GB/T 7714 | Yang, J. , Zhang, M. , Zhu, L. et al. Application of artificial intelligence in environmental engineering: Hotspots evolution and future trends; [人工智能在环境工程中的应用：热点演化与未来趋势] [J]. | Chinese Journal of Environmental Engineering , 2024 , 18 (11) : 3049-3058 . |
| MLA | Yang, J. et al. "Application of artificial intelligence in environmental engineering: Hotspots evolution and future trends; [人工智能在环境工程中的应用：热点演化与未来趋势]" . | Chinese Journal of Environmental Engineering 18 . 11 (2024) : 3049-3058 . |
| APA | Yang, J. , Zhang, M. , Zhu, L. , Zhang, W. , Xu, M. , Wang, D. et al. Application of artificial intelligence in environmental engineering: Hotspots evolution and future trends; [人工智能在环境工程中的应用：热点演化与未来趋势] . | Chinese Journal of Environmental Engineering , 2024 , 18 (11) , 3049-3058 . |
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