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学者姓名:李小娟
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The key to achieve sustainable treatment of high-salinity dye-containing wastewater is effective fractionation of dyes and salts. In this study, a thin-film composite electro-nanofiltration membrane was successfully fabricated by co-deposition of levodopa and ε-polylysine onto a porous ultrafiltration membrane substrate. With the co-deposition of the polylevodopa/ε-polylysine composite coating on the substrate membrane, the surface properties were significantly regulated, resulting in decreased pore size, reduced surface negative charge density and lower specific electric resistance, thus enhancing their ion transfer and dye/salt fractionation efficacy. Specifically, the fabricated LDP-4 membrane (molecular weight cut-off of 408 Da) with a 4-h co-deposition experienced a 99.12 % reactive orange 16 dye rejection and 10.15 % NaCl rejection, indicating an impressive selectivity between dyes and salts. Additionally, the LDP-4 electro-nanofiltration membrane as anion conducting membrane exhibited a fast and efficient electro-driven transfer of Cl− ions. Notably, under an electric field, the fabricated LDP-4 electro-nanofiltration membrane can efficiently fractionate NaCl from the reactive orange 16/NaCl mixed solution, achieving a 98.89 % desalination efficiency and 99.79 % dye recovery. Furthermore, the LDP-4 membrane demonstrated remarkable anti-fouling property and long-term stability over an 8-cycle electro-nanofiltration operation. Therefore, the electro-nanofiltration membranes fabricated by co-deposition of levodopa and ε-polylysine show a promising potential in sustainable resource recovery from high-salinity dye-containing wastewater. © 2024 Elsevier B.V.
Keyword :
Co-deposition Co-deposition Dopamine-based modification Dopamine-based modification Electro-nanofiltration membrane Electro-nanofiltration membrane High-salinity wastewater High-salinity wastewater Resource recovery Resource recovery
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GB/T 7714 | Xie, S. , Yu, Z. , Chen, L. et al. Thin-film composite electro-nanofiltration membrane for one-step and efficient fractionation of dyes and salts in high-salinity textile wastewater [J]. | Desalination , 2024 , 591 . |
MLA | Xie, S. et al. "Thin-film composite electro-nanofiltration membrane for one-step and efficient fractionation of dyes and salts in high-salinity textile wastewater" . | Desalination 591 (2024) . |
APA | Xie, S. , Yu, Z. , Chen, L. , Du, J. , Li, J. , Yuan, W. et al. Thin-film composite electro-nanofiltration membrane for one-step and efficient fractionation of dyes and salts in high-salinity textile wastewater . | Desalination , 2024 , 591 . |
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随着锂离子电池(LIBs)需求量的急剧增长,必将产生大量废旧LIBs,如若处置不当,将带来严重的环境污染问题.废旧LIBs的正极材料中含有大量稀缺有价金属,对这些金属进行回收会产生环境和经济的双重效益.相较于传统的正极材料中金属组分的分离纯化回收技术,正极材料直接再生的策略因其具有工艺简单、能耗低、回收周期短、产品附加值高等优势而备受关注.本文综述了共沉淀法、溶胶-凝胶法、固相烧结法、水热法、离子热/熔盐法和电化学修复法6种废旧LIBs正极材料直接再生技术及其优缺点.其中共沉淀法和溶胶-凝胶法因其相对复杂的步骤、较高的设备要求和试剂成本,在工业化应用中具有一定的局限性;固相烧结法、水热法、离子热/熔盐法和电化学修复法因其便捷性和经济性,具有巨大的发展机会.同时展望了废旧LIBs正极材料直接再利用的前景和发展趋势,旨在为废旧LIBs回收领域研究提供参考.
Keyword :
回收 回收 正极材料 正极材料 直接再生 直接再生 锂离子电池(LIBs) 锂离子电池(LIBs)
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GB/T 7714 | 李红彦 , 谢书涵 , 张燕如 et al. 废旧锂离子电池正极材料直接再生技术研究进展 [J]. | 化工进展 , 2024 , 43 (9) : 5207-5216 . |
MLA | 李红彦 et al. "废旧锂离子电池正极材料直接再生技术研究进展" . | 化工进展 43 . 9 (2024) : 5207-5216 . |
APA | 李红彦 , 谢书涵 , 张燕如 , 王永净 , 王永好 , 吕源财 et al. 废旧锂离子电池正极材料直接再生技术研究进展 . | 化工进展 , 2024 , 43 (9) , 5207-5216 . |
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Developing the Co-based catalysts with high reactivity for the sulfate radical (SO4−·)–based advanced oxidation processes (SR-AOPs) has been attracting numerous attentions. To improve the peroxymonosulfate (PMS) activation process, a novel Co-based catalyst simultaneously modified by bamboo carbon (BC) and vanadium (V@CoO-BC) was fabricated through a simple solvothermal method. The atenolol (ATL) degradation experiments in V@CoO-BC/PMS system showed that the obtained V@CoO-BC exhibited much higher performance on PMS activation than pure CoO, and the V@CoO-BC/PMS system could fully degrade ATL within 5 min via the destruction of both radicals (SO4−· and O2−··) and non-radicals (1O2). The quenching experiments and electrochemical tests revealed that the enhancing mechanism of bamboo carbon and V modification involved four aspects: (i) promoting the PMS and Co ion adsorption on the surface of V@CoO-BC; (ii) enhancing the electron transfer efficiency between V@CoO-BC and PMS; (iii) activating PMS with V3+ species; (iv) accelerating the circulation of Co2+ and Co3+, leading to the enhanced yield of reactive oxygen species (ROS). Furthermore, the V@CoO-BC/PMS system also exhibited satisfactory stability under broad pH (3–9) and good efficiency in the presence of co-existing components (HCO3−, NO3−, Cl−, and HA) in water. This study provides new insights to designing high-performance, environment-friendly bimetal catalysts and some basis for the remediation of antibiotic contaminants with SR-AOPs. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2024.
Keyword :
Antibiotic degradation Antibiotic degradation Biochar modification Biochar modification Co-based catalyst Co-based catalyst Peroxymonosulfate activation Peroxymonosulfate activation V modification V modification
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GB/T 7714 | Hu, Y. , Yang, K. , Lin, Y. et al. Performance and mechanistic studies of rapid atenolol degradation through peroxymonosulfate activation by V, Co, and bamboo carbon catalyst [J]. | Environmental Science and Pollution Research , 2024 , 31 (25) : 36761-36777 . |
MLA | Hu, Y. et al. "Performance and mechanistic studies of rapid atenolol degradation through peroxymonosulfate activation by V, Co, and bamboo carbon catalyst" . | Environmental Science and Pollution Research 31 . 25 (2024) : 36761-36777 . |
APA | Hu, Y. , Yang, K. , Lin, Y. , Weng, X. , Jiang, Y. , Huang, J. et al. Performance and mechanistic studies of rapid atenolol degradation through peroxymonosulfate activation by V, Co, and bamboo carbon catalyst . | Environmental Science and Pollution Research , 2024 , 31 (25) , 36761-36777 . |
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The key to achieve sustainable treatment of high-salinity dye-containing wastewater is effective fractionation of dyes and salts. In this study, a thin-film composite electro-nanofiltration membrane was successfully fabricated by co-deposition of levodopa and epsilon-polylysine onto a porous ultrafiltration membrane substrate. With the codeposition of the polylevodopa/epsilon-polylysine composite coating on the substrate membrane, the surface properties were significantly regulated, resulting in decreased pore size, reduced surface negative charge density and lower specific electric resistance, thus enhancing their ion transfer and dye/salt fractionation efficacy. Specifically, the fabricated LDP-4 membrane (molecular weight cut-off of 408 Da) with a 4-h co-deposition experienced a 99.12 % reactive orange 16 dye rejection and 10.15 % NaCl rejection, indicating an impressive selectivity between dyes and salts. Additionally, the LDP-4 electro-nanofiltration membrane as anion conducting membrane exhibited a fast and efficient electro-driven transfer of Cl ions. Notably, under an electric field, the fabricated LDP-4 electro-nanofiltration membrane can efficiently fractionate NaCl from the reactive orange 16/NaCl mixed solution, achieving a 98.89 % desalination efficiency and 99.79 % dye recovery. Furthermore, the LDP-4 membrane demonstrated remarkable anti-fouling property and long-term stability over an 8-cycle electronanofiltration operation. Therefore, the electro-nanofiltration membranes fabricated by co-deposition of levodopa and epsilon-polylysine show a promising potential in sustainable resource recovery from high-salinity dye-containing wastewater.
Keyword :
Co-deposition Co-deposition Dopamine-based modification Dopamine-based modification Electro-nanofiltration membrane Electro-nanofiltration membrane High-salinity wastewater High-salinity wastewater Resource recovery Resource recovery
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GB/T 7714 | Xie, Shuangling , Yu, Zijian , Chen, Lianxin et al. Thin-film composite electro-nanofiltration membrane for one-step and efficient fractionation of dyes and salts in high-salinity textile wastewater [J]. | DESALINATION , 2024 , 591 . |
MLA | Xie, Shuangling et al. "Thin-film composite electro-nanofiltration membrane for one-step and efficient fractionation of dyes and salts in high-salinity textile wastewater" . | DESALINATION 591 (2024) . |
APA | Xie, Shuangling , Yu, Zijian , Chen, Lianxin , Du, Jiale , Li, Jiangjing , Yuan, Weishuang et al. Thin-film composite electro-nanofiltration membrane for one-step and efficient fractionation of dyes and salts in high-salinity textile wastewater . | DESALINATION , 2024 , 591 . |
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Developing adsorbents with high performance and long service life for effective extracting the trace organochlorine pesticides (OCPs) from real water is attracting numerous attentions. Herein, a self-standing covalent organic framework (COF-TpPa) membrane with fiber morphology was successfully synthesized by using electrospun nanofiber membranes as template and employed as solid-phase microextraction (SPME) coating for ultra-high sensitivity extraction and analysis of trace OCPs in water. The as-synthesized COF-TpPa membrane exhibited a high specific surface area (800.83 m(2) g(-1)), stable nanofibrous structure, and excellent chemical and thermal stability. Based on the COF-TpPa membrane, a new SPME analytical method in conjunction with gas chromatography-mass spectrometry (GC-MS) was established. This proposed method possessed favorable linearity in concentration of 0.05-2000 ng L-1, high sensitivity with enrichment factors ranging from 2175 to 5846, low limits of detection (0.001-0.150 ng L-1), satisfactory precision (RSD < 10 %), and excellent repeatability (>150 cycles), which was better than most of the reported works. Additionally, the density functional theory (DFT) calculations and XPS results demonstrated that the outstanding enrichment performance of the COF-TpPa membrane was owing to synergistic effect of pi-pi stacking effects, high specific surface area and hydrogen bonding. This work will expect to extend the applications of COF membrane to captures trace organic pollutants in complex environmental water, as well as offer a multiscale interpretation for the design of effective adsorbents.
Keyword :
Covalent organic framework nanofibrous Covalent organic framework nanofibrous Direct immersion solid-phase microextraction Direct immersion solid-phase microextraction Gas chromatography-mass spectrometry Gas chromatography-mass spectrometry membrane membrane Organochlorine pesticides Organochlorine pesticides
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GB/T 7714 | Lin, Chunxiang , Weng, Yufang , Lin, Yule et al. Porous covalent organic framework nanofibrous membrane for excellent enrichment and ultra-high sensitivity detection of trace organochlorine pesticides in water [J]. | JOURNAL OF CHROMATOGRAPHY A , 2024 , 1721 . |
MLA | Lin, Chunxiang et al. "Porous covalent organic framework nanofibrous membrane for excellent enrichment and ultra-high sensitivity detection of trace organochlorine pesticides in water" . | JOURNAL OF CHROMATOGRAPHY A 1721 (2024) . |
APA | Lin, Chunxiang , Weng, Yufang , Lin, Yule , Liu, Yifan , Li, Xiaojuan , Lv, Yuancai et al. Porous covalent organic framework nanofibrous membrane for excellent enrichment and ultra-high sensitivity detection of trace organochlorine pesticides in water . | JOURNAL OF CHROMATOGRAPHY A , 2024 , 1721 . |
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Developing the transition metal catalysts with high reactivity for the sulfate radical (SO4 -center dot) based advanced oxidation processes (SR-AOPs) has been attracting numerous attentions. To improve the peroxymonosulfate (PMS) activation process mediated by Co-based catalysts, a vanadium-cobalt bimetallic catalyst (V@CoO) was fabricated by modification vanadium through a simple solvothermal method. The pollutants degradation experiments showed that the obtained V@CoO exhibited much higher performance on PMS activation (5.55-8.33 times larger of apparent rate constants) than pure CoO, and the V@CoO/PMS system could quickly degrade various organic contaminants within 5 min under the attack of both radicals (SO4 -center dot and O2-center dot) and non-radicals (1O2). The density functional theory (DFT) calculations and electrochemical tests revealed that the enhancing mechanism of V modification involved four aspects: (i) promoting the PMS adsorption on the surface of V@CoO; (ii) enhancing the electron transfer efficiency between V@CoO and PMS; (iii) activating PMS with V3+ and V4+ species; (iv) accelerating the circulation of Co2+ and Co3+, leading to the promotion on the production of reactive oxygen species (ROS). Furthermore, the V@CoO/PMS system also exhibited satisfactory stability in a broad pH range and good efficiency in the presence of co-existing components (HCO3-, NO3-, PO43- , Cl- and HA) in water. This study will provide new insights to designing high-performance, environment-friendly bimetal catalysts and some basis for the remediation of organic contaminants with SR-AOPs.
Keyword :
Co-based catalyst Co-based catalyst Degradation Degradation Organic pollutants Organic pollutants Peroxymonosulfate activation Peroxymonosulfate activation V modification V modification
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GB/T 7714 | Jiang, Yanting , Weng, Xin , Hu, Yihui et al. Enhanced peroxymonosulfate (PMS) activation process mediated by vanadium modified CoO catalyst for rapid degradation of organic pollutants: Insights into the role of V [J]. | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING , 2024 , 12 (2) . |
MLA | Jiang, Yanting et al. "Enhanced peroxymonosulfate (PMS) activation process mediated by vanadium modified CoO catalyst for rapid degradation of organic pollutants: Insights into the role of V" . | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING 12 . 2 (2024) . |
APA | Jiang, Yanting , Weng, Xin , Hu, Yihui , Lv, Yuancai , Yu, Zhendong , Liu, Yifan et al. Enhanced peroxymonosulfate (PMS) activation process mediated by vanadium modified CoO catalyst for rapid degradation of organic pollutants: Insights into the role of V . | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING , 2024 , 12 (2) . |
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Detecting trace endocrine disruptors in water is crucial for evaluating the water quality. In this work, a innovative modified polyacrylonitrile@cyanuric chloride-triphenylphosphine nanofiber membrane (PAN@CC-TPS) was prepared by in situ growing triazine porous organic polymers on the polyacrylonitrile (PAN) nanofibers, and used in the dispersive solid phase extraction (DSPE) to enrich trace nitrobenzene phenols (NPs) in water. The resluted PAN@CC-TPS nanofiber membrane consisted of numerous PAN nanofibers cover with CC-TPS solid spheres (similar to 2.50 mu m) and owned abundant functional groups, excellent enrichment performance and good stability. In addition, the method based on PAN@CC-TPS displayed outstanding capacity in detecting the trace nitrobenzene phenols, with 0.50-1.00 mu g/L of the quantification, 0.10-0.80 mu g/L of the detection limit, 85.35-113.55 % of the recovery efficiency, and 98.08-103.02 of the enrichment factor, which was comparable to most materials. Meanwhile, when PAN@CC-TPS was adopted in the real water samples (sea water and river water), the high enrichment factors and recovery percentages strongly confirmed the feasibility of PAN@CC-TPS for enriching and detecting the trace NPs. Besides, the related mechanism of extracting NPs on PAN@CC-TPS mainly involved the synergistic effect of hydrogen bonding, pi-pi stacking and hydrophobic effect.
Keyword :
Adsorption Adsorption Dispersive solid phase extraction Dispersive solid phase extraction Enrichment Enrichment Nanofiber membrane Nanofiber membrane Nitro-phenol Nitro-phenol Triazine Triazine
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GB/T 7714 | Weng, Xin , Liu, Shuting , Huang, Jian et al. Efficient dispersive solid phase extraction of trace nitrophenol pollutants in water with triazine porous organic polymer modified nanofiber membrane [J]. | JOURNAL OF CHROMATOGRAPHY A , 2024 , 1717 . |
MLA | Weng, Xin et al. "Efficient dispersive solid phase extraction of trace nitrophenol pollutants in water with triazine porous organic polymer modified nanofiber membrane" . | JOURNAL OF CHROMATOGRAPHY A 1717 (2024) . |
APA | Weng, Xin , Liu, Shuting , Huang, Jian , Lv, Yuancai , Liu, Yifan , Li, Xiaojuan et al. Efficient dispersive solid phase extraction of trace nitrophenol pollutants in water with triazine porous organic polymer modified nanofiber membrane . | JOURNAL OF CHROMATOGRAPHY A , 2024 , 1717 . |
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With the rapid growth of the demand for lithium-ion battery (LIBs), a large number of waste LIBs will be produced. If not disposed of properly, it will bring serious environmental pollution problems. The cathode materials of spent LIBs contain a large number of rare valuable metals, and the recovery of these metals will produce both environmental and economic benefits. Compared with the traditional separation, purification and recovery technologies of metal components from cathode materials, the strategy of direct regeneration of cathode materials has attracted much attention due to its advantages of simple process, low energy consumption, short recycling cycle and high added value of products. Six direct regeneration technologies for cathode materials from spent LIBs such as coprecipitation method, sol-gel method, solid phase sintering method, hydrothermal method, ion thermal/molten salt method and electrochemical repair method were reviewed and their advantages and disadvantages were also summarized. Among them, coprecipitation method and sol-gel method had some limitations in industrial application because of their relatively complex steps, high equipment requirements and reagent cost. Solid phase sintering method, hydrothermal method, ion thermal/molten salt method and electrochemical repair method had great opportunities for development because of their convenience and economy. In addition, the prospect and development trend of direct recycling of cathode materials from spent LIBs were prospected in order to provide reference for the research in the field of spent LIBs recycling. © 2024 Chemical Industry Press Co., Ltd.. All rights reserved.
Keyword :
Bioreactors Bioreactors Bioremediation Bioremediation Coprecipitation Coprecipitation Energy efficiency Energy efficiency Lithium-ion batteries Lithium-ion batteries Palladium Palladium Recycling Recycling Sintering Sintering Sol-gel process Sol-gel process
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GB/T 7714 | Li, Hongyan , Xie, Shuhan , Zhang, Yanru et al. Research progress on the direct regeneration technology for cathode materials from spent lithium-ion batteries [J]. | Chemical Industry and Engineering Progress , 2024 , 43 (9) : 5207-5216 . |
MLA | Li, Hongyan et al. "Research progress on the direct regeneration technology for cathode materials from spent lithium-ion batteries" . | Chemical Industry and Engineering Progress 43 . 9 (2024) : 5207-5216 . |
APA | Li, Hongyan , Xie, Shuhan , Zhang, Yanru , Wang, Yongjing , Wang, Yonghao , Lyu, Yuancai et al. Research progress on the direct regeneration technology for cathode materials from spent lithium-ion batteries . | Chemical Industry and Engineering Progress , 2024 , 43 (9) , 5207-5216 . |
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In this study, the boron-doped iron-carbon composite (Fe@B/C-2) was prepared via a simple solvothermal and secondary calcination process by using iron metal-organic frameworks (Fe-MOFs) as precursor. The obtained Fe@B/C-2 possessed abundant active sites and low iron ion leaching, and exhibited excellent performance on peroxydisulfate (PDS) activation for efficient PFOS (10 mg/L) degradation (94 %) in 60 min, with 0.2 g/L of catalyst dosage, 1.0 g/L of PDS dosage and at 5.0 of initial pH. The radical scavenging and electron paramagnetic resonance (EPR) tests demonstrated that SO4 & sdot;- and & sdot;OH were the primary active species during PFOS elimination. Under the attack of these species, PFOS was first transformed into PFOA, followed by a sequential defluorination process, and lastly mineralized into CO2 and F. Notably, DFT results revealed that Fe species,-BC3/-BC2O structures on the carbon matrix performed crucial roles in PDS activation. The extraordinary catalytic activity of Fe@B/C-2 was attributable to the synergistic effects of Fe nanoparticles and the B-doped on carbon matrix. The doped B not only could activate the inert carbon skeleton and provided more catalytic centers, but also could accelerate the electron transfer efficiency, leading to a boost in PDS decomposition.
Keyword :
Degradation Degradation Fe -based catalyst Fe -based catalyst Perfluorooctane sulfonic acid Perfluorooctane sulfonic acid Peroxydisulfate activation Peroxydisulfate activation
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GB/T 7714 | Jiang, Yanting , Yu, Zhendong , Lv, Yuancai et al. Insights to PFOS elimination with peroxydisulfate activation mediated by boron modified Fe/C catalysts: Enhancing mechanism of boron and PFOS degradation pathway [J]. | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2023 , 652 : 1743-1755 . |
MLA | Jiang, Yanting et al. "Insights to PFOS elimination with peroxydisulfate activation mediated by boron modified Fe/C catalysts: Enhancing mechanism of boron and PFOS degradation pathway" . | JOURNAL OF COLLOID AND INTERFACE SCIENCE 652 (2023) : 1743-1755 . |
APA | Jiang, Yanting , Yu, Zhendong , Lv, Yuancai , Li, Xiaojuan , Lin, Chunxiang , Ye, Xiaoxia et al. Insights to PFOS elimination with peroxydisulfate activation mediated by boron modified Fe/C catalysts: Enhancing mechanism of boron and PFOS degradation pathway . | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2023 , 652 , 1743-1755 . |
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A boron and iron co-doped biochar (B-Fe/biochar) from Masson pine bark was fabricated and used to activate peroxydisulfate (PDS) for the degradation of guaiacol (GL). The roles of the dopants and the contribution of the radical and non-radical oxidations were investigated. The results showed that the doping of boron and iron significantly improved the catalytic activity of the biochar catalyst with a GL removal efficiency of 98.30% within 30 min. The degradation of the GL mainly occurred through the generation of hydroxyl radicals (center dot OHs) and electron transfer on the biochar surface, and a non-radical degradation pathway dominated by direct electron transfer was proposed. Recycling the B-Fe/biochar showed low metal leaching from the catalyst and satisfactory long-term stability and reusability, providing potential insights into the use of metal and non-metal co-doped biochar catalysts for PDS activation.
Keyword :
B/Fe co-doping B/Fe co-doping biochar biochar Masson pine bark Masson pine bark peroxydisulfate activation peroxydisulfate activation
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GB/T 7714 | Huang, Jian , Zhu, Yu , Bian, Huiyang et al. Insights into Enhanced Peroxydisulfate Activation with B and Fe Co-Doped Biochar from Bark for the Rapid Degradation of Guaiacol [J]. | MOLECULES , 2023 , 28 (22) . |
MLA | Huang, Jian et al. "Insights into Enhanced Peroxydisulfate Activation with B and Fe Co-Doped Biochar from Bark for the Rapid Degradation of Guaiacol" . | MOLECULES 28 . 22 (2023) . |
APA | Huang, Jian , Zhu, Yu , Bian, Huiyang , Song, Liang , Liu, Yifan , Lv, Yuancai et al. Insights into Enhanced Peroxydisulfate Activation with B and Fe Co-Doped Biochar from Bark for the Rapid Degradation of Guaiacol . | MOLECULES , 2023 , 28 (22) . |
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