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学者姓名：范功端
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Abstract ：
Pyrite-driven autotrophic denitrification (PAD) has been recognized as a promising treatment technology for nitrate removal. Although the occurrence of PAD has been found in recent years, there is a knowledge gap about effects of crystal plane of pyrite on the performance and mechanism of PAD system. Here, this study investigated the effects of crystal planes ({100}, {111} and {210}) of single-crystal pyrite on denitrification performance, electron transfer, and microbial mechanism in PAD system. The removal efficiency of nitrate in B-{210} reached 100%, which was 1.67-fold and 2.86-fold higher than that of B-{100} and B-{111}, respectively. X-ray photoelectron spectroscopy and electrochemical results indicated that Fe-S bonds of pyrite with {210} crystal plane were more susceptible to breakage by Fe3+ oxidation assault, and leaching microbially available Fe2+ and sulfur intermediates to drive autotrophic denitrification. Metagenomic results suggested that community of functional pyrite-driven denitrifiers varied in response to crystal plane, and abundances of N-S transformation and EETrelated microbes and genes in B-{210} notably up-regulated compared to B-{100} and B-{111}. In addition, this work proposed a dual-mode for electron transfer pathway during pyrite oxidation and nitrogen transformation in PAD system. In B-{210}, Fe(II)- and sulfur-driven denitrifiers obtained electron after pyrite oxidation-dissolution, and the enrichment of pyrite-oxidizing bacteria in B-{210} could enhance the electron transfer from pyrite through electron shuttles. This work highlighted that stronger surface reactivity and electron shuttle effect in B-{210} enhanced electron transfer, leading to favorable PAD performance in B-{210}. Overall, this study provides novel insights into the structure-activity relationship between the crystal plane structure of pyrite and denitrification activity in PAD system.
Keyword ：
Autotrophic denitrification Autotrophic denitrification Crystal plane Crystal plane Electron transfer Electron transfer Metagenome analysis Metagenome analysis Pyrite Pyrite
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| GB/T 7714 | Wang, Yingmu , Chen, Shi , Chen, Yuanjing et al. Structure-activity relationship between crystal plane and pyrite-driven autotrophic denitrification efficacy: Electron transfer and metagenome-based microbial mechanism [J]. | WATER RESEARCH , 2025 , 268 . |
| MLA | Wang, Yingmu et al. "Structure-activity relationship between crystal plane and pyrite-driven autotrophic denitrification efficacy: Electron transfer and metagenome-based microbial mechanism" . | WATER RESEARCH 268 (2025) . |
| APA | Wang, Yingmu , Chen, Shi , Chen, Yuanjing , Xu, Junge , Zhou, Jian , He, Qiang et al. Structure-activity relationship between crystal plane and pyrite-driven autotrophic denitrification efficacy: Electron transfer and metagenome-based microbial mechanism . | WATER RESEARCH , 2025 , 268 . |
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随着水环境中抗生素污染的日益严重,开发高效、稳定的抗生素去除技术至关重要.以Bi2MoO6/FeVO4核壳纳米材料为催化剂,超滤膜为分离手段,将超滤膜与声光催化技术相耦合而构建了声光催化膜反应器(SPMR),并探究其对水中环丙沙星(CIP)的去除效果.结果表明,SPMR对CIP的降解率随水力停留时间(HRT)增加而提高,当HRT为60 min时,降解率可达94.56％.中空纤维膜能有效截留催化剂,保证反应器中催化剂浓度稳定.在SPMR降解CIP过程中,羟基自由基(·OH)和空穴(h+)起主导作用.SPMR对实际水体和模拟水中的CIP均有良好的去除效果,降解率均在80％以上,证实了声光催化技术可用于去除不同水体中的CIP.
Keyword ：
声光催化 声光催化 水力停留时间 水力停留时间 环丙沙星 环丙沙星 羟基自由基 羟基自由基 超滤 超滤
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| GB/T 7714 | 邹建勇 , 林晨 , 孟玉 et al. 声光催化膜反应器构建及其对环丙沙星的去除效能 [J]. | 中国给水排水 , 2025 , 41 (3) : 1-6 . |
| MLA | 邹建勇 et al. "声光催化膜反应器构建及其对环丙沙星的去除效能" . | 中国给水排水 41 . 3 (2025) : 1-6 . |
| APA | 邹建勇 , 林晨 , 孟玉 , 顾正亚 , 范功端 . 声光催化膜反应器构建及其对环丙沙星的去除效能 . | 中国给水排水 , 2025 , 41 (3) , 1-6 . |
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Ensuring safe drinking water is a global priority, with pathogen control being an essential aspect. Chlorine disinfection is widely adopted for its affordability and potent antimicrobial effects. However, certain bacteria, known as chlorine-resistant bacteria (CRB), can still survive in water systems with residual chlorine, posing risks to water quality and distribution systems. Their emergence, ironically, can be partially attributed to the very application or increased dosage of chlorine disinfectants in certain cases, which unintentionally promoted the selection and adaptation of CRB in the environment. Despite their significance, research on CRB remains fragmented, with few systematic reviews or bibliometric analyses. Thus, this study addresses the gap by analyzing 1367 publications (1984-2025) regarding CRB in drinking water supply systems (DWSSs) using CiteSpace. Important aspects including typical species, potential risks, resistance mechanisms, and inactivation methods are reviewed. Contributions from key countries/institutions/journals/authors are also examined. More importantly, overlooked issues like CRB's impact on taste and odor (T&O) issues in water and their molecular resistance mechanisms are also highlighted. The identification of these gaps in CRB research motivates further studies on their hazards, intrinsic mechanisms and control, which would hopefully help with the delivery of high-quality, safe drinking water worldwide.
Keyword ：
chlorine resistant bacteria (CRB) chlorine resistant bacteria (CRB) CiteSpace CiteSpace control strategies control strategies genetic mechanisms genetic mechanisms infrastructure risks infrastructure risks pathogen control pathogen control resistance barriers resistance barriers taste and odor (T&O) risks taste and odor (T&O) risks
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| GB/T 7714 | Wang, Yue , Zhang, Zhiming , Xia, Mingqian et al. Mechanism and Risk Control of Chlorine-Resistant Bacteria in Drinking Water Supply Systems: A Comprehensive Bibliometric Analysis [J]. | WATER , 2025 , 17 (7) . |
| MLA | Wang, Yue et al. "Mechanism and Risk Control of Chlorine-Resistant Bacteria in Drinking Water Supply Systems: A Comprehensive Bibliometric Analysis" . | WATER 17 . 7 (2025) . |
| APA | Wang, Yue , Zhang, Zhiming , Xia, Mingqian , Zhang, Xiaomin , Lan, Rongxing , Wei, Binqing et al. Mechanism and Risk Control of Chlorine-Resistant Bacteria in Drinking Water Supply Systems: A Comprehensive Bibliometric Analysis . | WATER , 2025 , 17 (7) . |
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In recent years, the urgent need to mitigate stormwater runoff and address urban waterlogging has garnered significant attention. Low Impact Development (LID) has emerged as a promising strategy for managing urban runoff sustainably. However, the vast array of potential LID layout combinations presents challenges in quantifying their effectiveness and often results in high construction costs. To address these issues, this study proposes a simulation-optimization framework that integrates the Storm Water Management Model (SWMM) with advanced optimization techniques to minimize both runoff volume and costs. The framework incorporates random variations in rainfall intensity within the basin, ensuring robustness under diverse climatic conditions. By leveraging a multi-objective scatter search algorithm, this research optimizes LID layouts to achieve effective stormwater management. The algorithm is further enhanced by two local search techniques-namely, the 'cost-benefit' local search and path-relinking local search-which significantly improve computational efficiency. Comparative analysis reveals that the proposed algorithm outperforms the widely used NSGA-II (Non-dominated Sorting Genetic Algorithm II), reducing computation time by an average of 8.89%, 16.98%, 1.72%, 3.85%, and 1.23% across various scenarios. The results demonstrate the method's effectiveness in achieving optimal LID configurations under variable rainfall intensities, highlighting its practical applicability for urban flood management. This research contributes to advancing urban sponge city initiatives by providing a scalable, efficient, and scientifically grounded solution for sustainable urban water management. The proposed framework is expected to support decision-makers in designing cost-effective and resilient stormwater management systems, paving the way for more sustainable urban development.
Keyword ：
computational efficiency simulation optimization computational efficiency simulation optimization cost-benefit analysis cost-benefit analysis low impact development low impact development multi-objective scatter search algorithm multi-objective scatter search algorithm path-relinking path-relinking
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| GB/T 7714 | Huang, Yuzhou , Li, Debiao , Li, Qiusha et al. Optimization of Low Impact Development Layouts for Urban Stormwater Management: A Simulation-Based Approach Using Multi-Objective Scatter Search Algorithm [J]. | WATER , 2025 , 17 (6) . |
| MLA | Huang, Yuzhou et al. "Optimization of Low Impact Development Layouts for Urban Stormwater Management: A Simulation-Based Approach Using Multi-Objective Scatter Search Algorithm" . | WATER 17 . 6 (2025) . |
| APA | Huang, Yuzhou , Li, Debiao , Li, Qiusha , Xu, Kai-Qin , Xie, Jiankun , Qiang, Wei et al. Optimization of Low Impact Development Layouts for Urban Stormwater Management: A Simulation-Based Approach Using Multi-Objective Scatter Search Algorithm . | WATER , 2025 , 17 (6) . |
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Eutrophication-induced algal blooms present serious risks to aquatic ecosystems and human health by crowding out the living space of aquatic plants and animals. In this study, an Ag2CO3/WO3 photocatalyst with exceptional optical properties was synthesized using an in situ stirring method. This photocatalyst exhibited remarkable efficacy in the visible light photocatalytic inactivation of Microcystis aeruginosa, achieving nearly 100% algal removal within 180 min. To elucidate the particular effect on algae cell for visible light photocatalytic inactivation, the physiological changes in algal cells were further investigated. Our findings revealed that Ag2CO3/ WO3 severely impairs membrane permeability, disrupts stability, and interferes with the physiological metabolism of algal cells, leading to the continuous release and subsequent degradation of intra- and extracellular organic matter. Additionally, several reactive radicals, center dot OH, center dot O2-, 1O2 and h+, are considered the primary contributors to the inactivation of algal cells during visible-light photocatalytic inactivation. And efficient electron- hole separation in Ag2CO3/WO3, induced by the internal electric field, is a prerequisite for reactive oxygen species (ROSs) generation. Based on these findings, a potential mechanism for the visible light photocatalytic inactivation of M. aeruginosa by Ag2CO3/WO3 was proposed. Overall, Ag2CO3/WO3 demonstrated exceptional effectiveness in removing M. aeruginosa and held promise for application in managing harmful cyanobacteria blooms in aquatic ecosystems.
Keyword ：
Algae elimination Algae elimination Composite photocatalysts Composite photocatalysts Microcystis aeruginosa Microcystis aeruginosa Transfer mechanism Transfer mechanism
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| GB/T 7714 | Fan, Gongduan , Yao, Yixin , Cai, Chenjian et al. Enhanced visible light photocatalytic inactivation of Microcystis aeruginosa using Ag2CO3/WO3 with strong internal electric field: Performance and mechanism [J]. | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 362 . |
| MLA | Fan, Gongduan et al. "Enhanced visible light photocatalytic inactivation of Microcystis aeruginosa using Ag2CO3/WO3 with strong internal electric field: Performance and mechanism" . | SEPARATION AND PURIFICATION TECHNOLOGY 362 (2025) . |
| APA | Fan, Gongduan , Yao, Yixin , Cai, Chenjian , Du, Banghao , Shi, Antong , Xu, Kai-Qin . Enhanced visible light photocatalytic inactivation of Microcystis aeruginosa using Ag2CO3/WO3 with strong internal electric field: Performance and mechanism . | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 362 . |
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Photocatalytic technology offers broad applications in the treatment of cyanobacterial blooms. This study successfully synthesized a series of highly efficient Ag2MoO4/ZnSnO3 photocatalysts through a straightforward hydrothermal method. Among the synthesized photocatalysts, the 35 % Ag2MoO4-doped Ag2MoO4/ZnSnO3 exhibited the highest photocatalytic activity, achieving nearly 100 % algal removal within 3 h under visible light irradiation. This composite also displays excellent reusability and chemical stability, offering a more effective and sustainable solution compared to traditional methods such as chemical coagulation or physical filtration. The exceptional efficiency results from the potent oxidative capabilities of various reactive oxygen species, which are generated through the efficient Z-scheme electron transfer mechanism facilitated by Ag2MoO4/ZnSnO3. Upon photocatalytic process of Ag2MoO4/ZnSnO3, some algal cells became destabilized and sedimented, with visibly damaged cell walls. In the initial stage, the photosynthetic system was inhibited, a critical factor leading to algal cell death. The accumulation of reactive oxygen species (ROS) induced oxidative damage, leading to the collapse of the antioxidant system, cell rupture, and continuous leakage of intracellular electrolytes (K+, Ca2+, Mg2+), organic matter, and proteins. Even after five consecutive cycles, the Ag2MoO4/ZnSnO3 photocatalyst maintained an algae removal rate above 95 %, demonstrating excellent reusability and stability. In conclusion, Ag2MoO4/ ZnSnO3, as a stable and efficient photocatalyst, presents a promising approach for mitigating harmful algal blooms.
Keyword ：
Ag2MoO4/ZnSnO3 Ag2MoO4/ZnSnO3 Microcystis aeruginosa Microcystis aeruginosa Photocatalysis Photocatalysis Z -scheme heterojunction Z -scheme heterojunction
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| GB/T 7714 | Fan, Gongduan , Xu, Zongqiong , Lin, Bin et al. Efficient inactivation of Microcystis aeruginosa using Z-scheme heterojunction Ag2MoO4/ZnSnO3 photocatalysts: Synthesis, mechanism, and reusability [J]. | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 362 . |
| MLA | Fan, Gongduan et al. "Efficient inactivation of Microcystis aeruginosa using Z-scheme heterojunction Ag2MoO4/ZnSnO3 photocatalysts: Synthesis, mechanism, and reusability" . | SEPARATION AND PURIFICATION TECHNOLOGY 362 (2025) . |
| APA | Fan, Gongduan , Xu, Zongqiong , Lin, Bin , Wu, Xinyi , Huang, Yuzhou , Luo, Jing et al. Efficient inactivation of Microcystis aeruginosa using Z-scheme heterojunction Ag2MoO4/ZnSnO3 photocatalysts: Synthesis, mechanism, and reusability . | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 362 . |
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A novel dual-function ZnAl–LDH/Bi4O5Br2 nanocomposite photocatalyst was synthesized using a self-assembly process and optimized by response surface methodology for the advanced treatment of wastewater micropollutants. A series of characterizations revealed that ZnAl–LDH/Bi4O5Br2 exhibits suitable heterojunction structure and excellent optoelectronic properties. As a result, ZnAl–LDH/Bi4O5Br2 achieved the near-complete removal of bisphenol A (BPA) after 120 min through a synergistic process of adsorption and visible-light photocatalysis. The corresponding reaction rate constant for photocatalytic degradation approached 0.14 min−1, which is significantly higher than those by Bi4O5Br2 and ZnAl–LDH. Regarding the enhanced BPA removal over ZnAl–LDH/Bi4O5Br2, the adsorption behavior occurred via hydrogen bonding and π-π stacking interactions, while the photocatalytic degradation involved the efficient photoexcitation and separation of charge carriers for the formation of reactive oxygen species (ROS) under the heterojunction effect. Electron spin resonance (ESR) and radical quenching experiments indicated that ROS including ·OH, ·O2−, and 1O2, mainly contribute to BPA degradation. The predominant ROS formation mechanism was the interfacial reactions of the nanocomposite with H2O molecules, as verified by the density of states, charge density differences, and adsorption energy calculations. Furthermore, the intermediate products of BPA degradation were identified, the degradation pathways were proposed, and the related ecotoxicity consequences were evaluated. This study confirmed that ZnAl–LDH/Bi4O5Br2 has superior synergistic adsorptive and photocatalytic performance, offering guidance in the further construction and application of functional nanocomposites for wastewater treatment. © 2025 Elsevier Inc.
Keyword ：
Electron resonance Electron resonance Equilibrium constants Equilibrium constants Free radical reactions Free radical reactions Hydrogen bonds Hydrogen bonds Optical conductivity Optical conductivity Photocatalytic activity Photocatalytic activity Photodegradation Photodegradation Rate constants Rate constants Reaction intermediates Reaction intermediates
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| GB/T 7714 | Shen, Jyunhong , Shi, Antong , Li, Yujian et al. Heterostructured ZnAl–LDH/Bi4O5Br2 photocatalyst with enhanced surface molecular adsorption for efficient bisphenol A removal [J]. | Journal of Colloid and Interface Science , 2025 , 697 . |
| MLA | Shen, Jyunhong et al. "Heterostructured ZnAl–LDH/Bi4O5Br2 photocatalyst with enhanced surface molecular adsorption for efficient bisphenol A removal" . | Journal of Colloid and Interface Science 697 (2025) . |
| APA | Shen, Jyunhong , Shi, Antong , Li, Yujian , Yao, Yixin , Yao, Xiao , Zhang, Zhi et al. Heterostructured ZnAl–LDH/Bi4O5Br2 photocatalyst with enhanced surface molecular adsorption for efficient bisphenol A removal . | Journal of Colloid and Interface Science , 2025 , 697 . |
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Improving the spatial separation of photogenerated charge carriers and enhancing the direct electron utilization are crucial for photocatalytic materials and their application in water purification. In this study, a novel heterojunction, CoFe layered double oxides encapsulated by oxygen-vacancy-rich BiOBr (CoFe-LDO/BiOBr-OV, shortened to CFB), was successfully synthesized for the removal of halogenated disinfection by-products bromate and trichloroacetamide (TCAcAm) under simulated solar light. Advanced characterization techniques and density functional theory calculations demonstrated that the enhanced photoelectrochemical properties of CFB can be attributed to the heterojunction effect and OVs incorporation. The internal electric field between CoFe-LDO and BiOBr-OV facilitated S-scheme charge transfer, and more available electrons were retained a relatively negative redox potential position onto the heterojunctions. Meanwhile, the OVs in BiOBr further alleviated the consumption of electrons caused by dissolved oxygen to some extent. Owing to the efficient dehalogenation mediated by electron transfer, the photocatalytic process of CFB achieved the complete removal of bromate and TCAcAm after 20 min and 3 h, respectively. The dehalogenative removal rate of CFB approached 430, 39 and 5.7-fold higher than those of CoFe-LDO, BiOBr and BiOBr-OV, respectively. Additionally, the ecotoxicity evaluation based on the behavior of zebrafish larvae indicated that the dehalogenative removal process of bromate and TCAcAm resulted in favorable detoxification. This work provides valuable guidance for the design and application of S-scheme heterojunction photocatalysts in the advanced treatment of halogenated micropollutants. © 2025 Elsevier B.V.
Keyword ：
Air cleaners Air cleaners Dechlorination Dechlorination Detoxification Detoxification Disinfection Disinfection Electrooptical effects Electrooptical effects Electrostriction Electrostriction Halon Halon Photocatalytic activity Photocatalytic activity Redox reactions Redox reactions Water filtration Water filtration
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| GB/T 7714 | Shen, Jyunhong , Yi, Mingxiu , Yao, Xiao et al. Construction of highly efficient CoFe-LDO/BiOBr-OV S-scheme heterojunction photocatalyst for dehalogenative removal of disinfection by-products from water: Performance and mechanism [J]. | Chemical Engineering Journal , 2025 , 514 . |
| MLA | Shen, Jyunhong et al. "Construction of highly efficient CoFe-LDO/BiOBr-OV S-scheme heterojunction photocatalyst for dehalogenative removal of disinfection by-products from water: Performance and mechanism" . | Chemical Engineering Journal 514 (2025) . |
| APA | Shen, Jyunhong , Yi, Mingxiu , Yao, Xiao , Zhang, Hongyu , Chen, Jinfeng , Fan, Gongduan et al. Construction of highly efficient CoFe-LDO/BiOBr-OV S-scheme heterojunction photocatalyst for dehalogenative removal of disinfection by-products from water: Performance and mechanism . | Chemical Engineering Journal , 2025 , 514 . |
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Under the dual pressures of global climate change and rapid urbanization, urban drainage systems (UDS) face severe challenges caused by extreme precipitation events and altered surface hydrological processes. The drainage paradigm is shifting toward resilient systems integrating grey and green infrastructure, necessitating a comprehensive review of the design and operation of grey infrastructure. This study systematically summarizes advances in urban stormwater process-wide regulation, focusing on drainage network design optimization, siting and control strategies for flow control devices (FCDs), and coordinated management of Quasi-Detention Basins (QDBs). Through graph theory-driven topological design, real-time control (RTC) technologies, and multi-objective optimization algorithms (e.g., genetic algorithms, particle swarm optimization), the research demonstrates that decentralized network layouts, dynamic gate regulation, and stormwater resource utilization significantly enhance system resilience and storage redundancy. Additionally, deep learning applications in flow prediction, flood assessment, and intelligent control exhibit potential to overcome limitations of traditional models. Future research should prioritize improving computational efficiency, optimizing hybrid infrastructure synergies, and integrating deep learning with RTC to establish more resilient and adaptive urban stormwater management frameworks. © 2025 by the authors.
Keyword ：
Global warming Global warming Graph algorithms Graph algorithms Network theory (graphs) Network theory (graphs) Particle swarm optimization (PSO) Particle swarm optimization (PSO)
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| GB/T 7714 | Xie, Jiankun , Qiang, Wei , Lin, Yiyuan et al. Enhancing Urban Drainage Resilience Through Holistic Stormwater Regulation: A Review [J]. | Water (Switzerland) , 2025 , 17 (10) . |
| MLA | Xie, Jiankun et al. "Enhancing Urban Drainage Resilience Through Holistic Stormwater Regulation: A Review" . | Water (Switzerland) 17 . 10 (2025) . |
| APA | Xie, Jiankun , Qiang, Wei , Lin, Yiyuan , Huang, Yuzhou , Xu, Kai-Qin , Zheng, Dangshi et al. Enhancing Urban Drainage Resilience Through Holistic Stormwater Regulation: A Review . | Water (Switzerland) , 2025 , 17 (10) . |
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A novel Ag 3 PO 4 /ZnWO 4 -modified graphite felt electrode (AZW@GF) was prepared by drop coating method and applied to photoelectrocatalytic removal of harmful algae. Results showed that approximately 99.21% of chlorophyll a and 91.57% of Microcystin-LR (MCLR) were degraded by the AZW@GF-Pt photoelectrocatalytic system under the optimal operating conditions with a rate constant of 0.02617 min -1 and 0.01416 min -1 , respectively. The calculated synergistic coefficient of photoelectrocatalytic algal removal and MC-LR degradation by the AZW@GF-Pt system was both larger than 1.9. In addition, the experiments of quenching experiments and electron spin resonance (ESR) revealed that the photoelectrocatalytic reaction mainly generated center dot OH and center dot O 2 - for algal removal and MC-LR degradation. Furthermore, the potential pathway for photoelectrocatalytic degradation of MC-LR was proposed. Finally, the photoelectrocatalytic cycle algae removal experiments were carried out on AZW@GF electrode, which was found to maintain the algae removal efficiency at about 91% after three cycles of use, indicating that the photoelectrocatalysis of AZW@GF electrode is an effective emergency algae removal technology.
Keyword ：
Graphite felt electrode Graphite felt electrode Harmful algae Harmful algae Inactivation mechanism Inactivation mechanism Photoelectrocatalysis Photoelectrocatalysis
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| GB/T 7714 | Cai, Chenjian , Fan, Gongduan , Cao, Xingfeng et al. Novel Ag3PO4/ZnWO4-modified graphite felt electrode for photoelectrocatalytic removal of harmful algae: Performance and mechanism [J]. | JOURNAL OF HAZARDOUS MATERIALS , 2024 , 470 . |
| MLA | Cai, Chenjian et al. "Novel Ag3PO4/ZnWO4-modified graphite felt electrode for photoelectrocatalytic removal of harmful algae: Performance and mechanism" . | JOURNAL OF HAZARDOUS MATERIALS 470 (2024) . |
| APA | Cai, Chenjian , Fan, Gongduan , Cao, Xingfeng , Luo, Jing , He, Zhimin , Wang, Shichang et al. Novel Ag3PO4/ZnWO4-modified graphite felt electrode for photoelectrocatalytic removal of harmful algae: Performance and mechanism . | JOURNAL OF HAZARDOUS MATERIALS , 2024 , 470 . |
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