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学者姓名：吕源财
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Abstract ：
Para-arsanilic acid (p-ASA) is widely used as a feed additive, making it a pervasive environmental pollutant. Due to its migratory and transformative nature, p-ASA can easily convert into more toxic inorganic arsenic during its migration, thereby increasing the ecological burden and posing a threat to human health. Efficient removal of p- ASA from water is crucial for mitigating arsenic contamination. Efficient removal of p-ASA from water is crucial for mitigating arsenic contamination. This study introduced zirconium-loaded collagen fiber membrane (CFM-Zr), a novel, sustainable membrane adsorption material synthesized by retanning collagen fiber membranes (CFM) with zirconium (Zr). Leveraging the physicochemical properties of CFM and the strong affinity of Zr forp-ASA, CFM-Zr achieved highly efficient p-ASA removal. The resulting membrane was made entirely from green, low-carbon and recyclable raw materials, achieving sustainable removal of p-ASA while realizing the concept of treating waste with waste for environmental recovery. Remarkably, the retanning with zirconium significantly enhanced the Zeta potential of CFM-Zr, strengthening its electrostatic attraction to p-ASA, with a maximum adsorption capacity of 289.02 mg & sdot;g- 1, which was 19.72 times higher than that of the CFM before retanning (13.95 mg & sdot;g-1). Its adsorption rate constant was 12.54 mg & sdot;g-1 & sdot;min- 1. Moreover, CFM-Zr showed good reusability and exhibited electrostatic adsorption and metal coordination effects on the "organic" parts (-OH,-NH2) and "inorganic" parts (As-O) of p-ASA, effectively removing it. This work provided a promising bio-based material for water purification, promoted the sustainable utilization of leather industry waste, and offered significant advancements in environmental remediation and resource recovery.
Keyword ：
Adsorption and separation Adsorption and separation Metal modification Metal modification Waste-to-resource conversion Waste-to-resource conversion Wastewater treatment Wastewater treatment
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| GB/T 7714 | Ye, Xiaoxia , Huang, Jian , Zhang, Yuqing et al. Efficient removal of p-arsanilic acid using a waste-derived collagen fiber-Zr composite membrane [J]. | JOURNAL OF WATER PROCESS ENGINEERING , 2025 , 71 . |
| MLA | Ye, Xiaoxia et al. "Efficient removal of p-arsanilic acid using a waste-derived collagen fiber-Zr composite membrane" . | JOURNAL OF WATER PROCESS ENGINEERING 71 (2025) . |
| APA | Ye, Xiaoxia , Huang, Jian , Zhang, Yuqing , Lin, Yi , Lv, Yuancai , Lin, Chunxiang et al. Efficient removal of p-arsanilic acid using a waste-derived collagen fiber-Zr composite membrane . | JOURNAL OF WATER PROCESS ENGINEERING , 2025 , 71 . |
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Heterogeneous electro-Fenton (hetero-EF) system was one of the most promising approaches for treating antibiotic-laden wastewater. However, the rational design of cost-effective, eco-friendly, and efficient earthabundant electrocatalysts remains a significant challenge. This study synthesized a novel catalyst, lignin-based metal biochar (Co-L@C), from coniferous lignin via hydrothermal reaction and temperature-controlled pyrolysis. The results demonstrated that Co-L@C achieved nearly 100% oxytetracycline hydrochloride (OTC) removal within 30 min employing the hetero-EF system, consistently exhibiting efficient OTC degradation rates across a wide pH range (3-9) and in various practical water matrices. In conjunction with the burst test and electron paramagnetic resonance (EPR) analysis, singlet oxygen (1O2) was shown to play a dominant role in OTC degradation. At the same time, further investigation revealed that hydroxyl radicals (& sdot;OH), superoxide radicals (O2 & sdot;- ), and dissolved oxygen (DO) all contributed to 1O2 production. This work offers a potential technology for the effective degradation of antibiotic-contaminated wastewater.
Keyword ：
Biochar Biochar Heterogeneous electro-Fenton Heterogeneous electro-Fenton Lignin Lignin Oxytetracycline hydrochloride Oxytetracycline hydrochloride Singlet oxygen Singlet oxygen
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| GB/T 7714 | Zou, Niao , Guo, Hong , Zheng, Zhihong et al. Effective degradation of OTC by Co-L@C cathode in heterogeneous Electro-Fenton system: Preeminent role of singlet oxygen species [J]. | PROCESS SAFETY AND ENVIRONMENTAL PROTECTION , 2025 , 193 : 1343-1353 . |
| MLA | Zou, Niao et al. "Effective degradation of OTC by Co-L@C cathode in heterogeneous Electro-Fenton system: Preeminent role of singlet oxygen species" . | PROCESS SAFETY AND ENVIRONMENTAL PROTECTION 193 (2025) : 1343-1353 . |
| APA | Zou, Niao , Guo, Hong , Zheng, Zhihong , Lv, Yuancai , Liu, Yifan , Chen, Zengpeng et al. Effective degradation of OTC by Co-L@C cathode in heterogeneous Electro-Fenton system: Preeminent role of singlet oxygen species . | PROCESS SAFETY AND ENVIRONMENTAL PROTECTION , 2025 , 193 , 1343-1353 . |
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《生物质的开发与利用》是资源循环科学与工程专业的核心必修课，是一门知识面广泛、实践性强的交叉学科课程。针对传统教学中存在的问题，教学团队提出了“以学生为中心、产出为导向、持续改进”的教学理念，并通过实施“四维”混合式教学法，对教学内容、方法和考核方式进行了全面的改革。引入科研项目，设计了一系列与课程内容密切相关的实验教学，涉及皮革废弃物（皮胶原纤维膜）改性利用、优化以及乳液分离性能的测试等实验，并对材料的结构和形貌进行表征，使用Origin软件对实验数据进行处理和分析。通过这些改革措施，不仅提高了课程的教学质量，也促进了学生创新能力和综合素质的有效提高。
Keyword ：
实践教学 实践教学 混合式教学 混合式教学 生物质 生物质 皮胶原纤维膜 皮胶原纤维膜 皮革废弃物 皮革废弃物 金属有机框架 金属有机框架
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| GB/T 7714 | 叶晓霞 , 吴秋 , 吕源财 et al. 生物质的开发与利用课程教学改革探讨 [J]. | 皮革科学与工程 , 2025 , 35 (3) : 120-125 . |
| MLA | 叶晓霞 et al. "生物质的开发与利用课程教学改革探讨" . | 皮革科学与工程 35 . 3 (2025) : 120-125 . |
| APA | 叶晓霞 , 吴秋 , 吕源财 , 刘以凡 , 林春香 , 陈杰 . 生物质的开发与利用课程教学改革探讨 . | 皮革科学与工程 , 2025 , 35 (3) , 120-125 . |
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以活性炭纤维毡(ACFF)为基底,采用水热法与超声法相结合方式制备了活性炭纤维毡负载N-TiO2/MoS2/N-TiO2光催化剂(NT/MS/NT/ACFF),并以此作为载体,通过共价结合法制得NT/MS/NT/ACFF固定化漆酶.利用扫描电子显微镜、X射线衍射仪、比表面积分析、拉曼光谱、紫外-可见分光光度计和傅里叶变换红外光谱等手段对样品的形貌、微观结构进行了表征,研究了不同体系对双酚A(BPA)的降解效果、反应动力学及矿化率,考察了催化剂的重复使用性能.结果表明,与其他体系相比,可见光下NT/MS/NT/ACFF固定化漆酶对BPA降解率高达82.5％,表观速率常数kobs为0.00764min-1,矿化率可达64.5％.NT/MS/NT/ACFF固定化漆酶具有良好的光催化、酶催化的活性及稳定性,循环使用4次后BPA降解率仍可达到69.4％.通过气相色谱-质谱(GC-MS)结果分析,推断BPA被NT/MS/NT/ACFF固定化漆酶的催化降解过程包括断裂重组、氧化分解、开环等反应.
Keyword ：
二硫化钼 二硫化钼 催化剂载体 催化剂载体 双酚A 双酚A 固定化 固定化 漆酶 漆酶 纳米二氧化钛 纳米二氧化钛
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| GB/T 7714 | 李章良 , 杨月珠 , 伍传田 et al. 活性炭纤维毡负载N-TiO2/MoS2/N-TiO2固定化漆酶降解双酚A [J]. | 化工进展 , 2025 , 44 (2) : 887-898 . |
| MLA | 李章良 et al. "活性炭纤维毡负载N-TiO2/MoS2/N-TiO2固定化漆酶降解双酚A" . | 化工进展 44 . 2 (2025) : 887-898 . |
| APA | 李章良 , 杨月珠 , 伍传田 , 吕源财 . 活性炭纤维毡负载N-TiO2/MoS2/N-TiO2固定化漆酶降解双酚A . | 化工进展 , 2025 , 44 (2) , 887-898 . |
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The presence of polyethylene terephthalate (PET) microplastics (MPs) in waters has posed considerable threats to the environment and humans. In this work, a heterogeneous electro-Fenton-activated persulfate oxidation system with the FeS2-modified carbon felt as the cathode (abbreviated as EF-SR) was proposed for the efficient degradation of PET MPs. The results showed that i) the EF-SR system removed 91.3 ± 0.9 % of 100 mg/L PET after 12 h at the expense of trace loss (< 0.07 %) of [Fe] and that ii) dissolved organics and nanoplastics were first formed and accumulated and then quickly consumed in the EF-SR system. In addition to the destruction of the surface morphology, considerable changes in the surface structure of PET were noted after EF-SR treatment. On top of the emergence of the O-H bond, the ratio of C-O/C=O to C-C increased from 0.25 to 0.35, proving the rupture of the backbone of PET and the formation of oxygen-containing groups on the PET surface. With the verified involvement and contributions of SO4•- and •OH, three possible paths were proposed to describe the degradation of PET towards complete mineralization through chain cleavage and oxidation in the EF-SR system. © 2024 Elsevier B.V.
Keyword ：
Electro-Fenton Electro-Fenton Hydroxyl radical Hydroxyl radical Microplastics Microplastics Polyethylene terephthalate Polyethylene terephthalate Sulfate radical Sulfate radical
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| GB/T 7714 | Lin, Y. , Zhang, Y. , Wang, Y. et al. Efficient degradation and mineralization of polyethylene terephthalate microplastics by the synergy of sulfate and hydroxyl radicals in a heterogeneous electro-Fenton-activated persulfate oxidation system [J]. | Journal of Hazardous Materials , 2024 , 478 . |
| MLA | Lin, Y. et al. "Efficient degradation and mineralization of polyethylene terephthalate microplastics by the synergy of sulfate and hydroxyl radicals in a heterogeneous electro-Fenton-activated persulfate oxidation system" . | Journal of Hazardous Materials 478 (2024) . |
| APA | Lin, Y. , Zhang, Y. , Wang, Y. , Lv, Y. , Yang, L. , Chen, Z. et al. Efficient degradation and mineralization of polyethylene terephthalate microplastics by the synergy of sulfate and hydroxyl radicals in a heterogeneous electro-Fenton-activated persulfate oxidation system . | Journal of Hazardous Materials , 2024 , 478 . |
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Lignin is a sustainable biomass resource with abundant hydroxyl groups that holds great promise for use as a feedstock for polyurethane foam production. Therefore, the flexible polyurethane foams (FPUFs) were prepared using the oxidized alkali lignin (OAL) as the matrix to enhance its compatibility. The OAL was obtained under the following conditions of 60 °C, 80 min treatment, a ratio of hydrogen peroxide to lignin of 1.2:1, and a ratio of iron hydroxide to lignin of 0.01. It was demonstrated that incorporating OAL enhanced the density, compressive strength, sound-absorbing performance and degradability of foam composites. The compressive strength was also improved by more than five times than that of blank foam under the optimal conditions, reaching 0.11 MPa. The thermogravimetric analysis (TGA) revealed that the foam composite containing 30 % modified lignin content exhibited the highest thermal stability. The results of solvent resistance testing demonstrated the durability of the foam composites in both water and solvents. Lignin-modified polyurethane foam exhibited an acoustic absorption coefficient above 0.2 across a wide frequency range, with the highest value reaching 0.84, meeting the conventional requirements for sound absorption materials (α > 0.2). The results suggested that this environmentally friendly preparation method was feasible for producing high-performance polyurethane foams, which was appropriate for the production of sound absorption boards for industry, transportation by train and automobile. © 2024
Keyword ：
Flexible polyurethane foam Flexible polyurethane foam Modified lignin Modified lignin Polyether polyol Polyether polyol Sound-absorbing property Sound-absorbing property
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| GB/T 7714 | Zhao, X. , Liu, Y. , Lv, Y. et al. Research on lignin-modified flexible polyurethane foam and its application in sound absorption [J]. | Journal of Industrial and Engineering Chemistry , 2024 , 137 : 327-337 . |
| MLA | Zhao, X. et al. "Research on lignin-modified flexible polyurethane foam and its application in sound absorption" . | Journal of Industrial and Engineering Chemistry 137 (2024) : 327-337 . |
| APA | Zhao, X. , Liu, Y. , Lv, Y. , Liu, M. . Research on lignin-modified flexible polyurethane foam and its application in sound absorption . | Journal of Industrial and Engineering Chemistry , 2024 , 137 , 327-337 . |
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China generates over 100 million tons of food waste annually, leading to significant environmental pollution and health risks if not managed properly. Converting FW into a high-value-added platform molecule, lactic acid (LA), through fermentation offers a promising approach for both waste treatment and resource recovery. This paper presents a comprehensive review of recent advancements in LA production from FW, focusing on pure strains fermentation and open fermentation technologies, metabolic mechanisms, and problems in fermentation. It also assesses purification methods, including molecular distillation, adsorption, membrane separation, precipitation, esterification and hydrolysis, solvent extraction, and in-situ separation, analyzing their efficiency, advantages, and disadvantages. However, current research encounters several challenges, including low LA yield, low optical purity of L-(+)-LA, and difficulties in the separation and purification of LA. The integration of in-situ separation technology coupled with multiple separation methods is highlighted as a promising direction for future advancements. © 2024 Elsevier Ltd
Keyword ：
Distillation Distillation
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| GB/T 7714 | Song, Liang , Cai, Chenhang , Chen, Zengpeng et al. Lactic acid production from food waste: Advances in microbial fermentation and separation technologies [J]. | Bioresource Technology , 2024 , 414 . |
| MLA | Song, Liang et al. "Lactic acid production from food waste: Advances in microbial fermentation and separation technologies" . | Bioresource Technology 414 (2024) . |
| APA | Song, Liang , Cai, Chenhang , Chen, Zengpeng , Lin, Chunxiang , Lv, Yuancai , Ye, Xiaoxia et al. Lactic acid production from food waste: Advances in microbial fermentation and separation technologies . | Bioresource Technology , 2024 , 414 . |
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A valonea tannin-immobilized cellulose-based aerogel (VTCA) was prepared by introducing valonea tannin into cellulose through crosslinking reaction in the of NaOH/urea/H2O solvent system. The structure and property of VTCA was characterized by SEM-EDS, FT-IR, XRD, etc., and the adsorption behavior for Ag(I) in aqueous solution was also investigated. The results showed that the three-dimensional VTCA displayed obvious porous structure with a porosity of 97.95%, and exhibited good adsorption efficiency (>75%) for Ag(I) under a wide pH range (1-8). The Ag(I) adsorption process obeyed the pseudo-second-order kinetic model and the Langmuir adsorption isotherm model. High temperature was favorable for adsorption, and the maximum theoretical adsorption capacity was 147.2mg/g. The mechanism of Ag(I) adsorption involved two process: Ag(I) was firstly adsorbed onto the surface of VTCA through the electrostatic attraction and chelation effects, and then in situ reduced to Ag0 by the phenolic hydroxyl group on the tannin structure. All the results revealed that VTCA owned good adsorption and reduction performance and could achieve the recycling of Ag(I) in water. © 2024 Chinese Society for Environmental Sciences. All rights reserved.
Keyword ：
adsorption adsorption Ag(I) Ag(I) cellulose-based aerogel cellulose-based aerogel reduction reduction valonea tannin valonea tannin
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| GB/T 7714 | Chen, Y. , Lin, Y.-L. , Lv, Y.-C. et al. Study of adsorption reduction behavior of Ag(I) on cured tannin cellulose-based aerogels; [固化单宁纤维素基气凝胶吸附还原 Ag(I)行为研究] [J]. | China Environmental Science , 2024 , 44 (4) : 2083-2092 . |
| MLA | Chen, Y. et al. "Study of adsorption reduction behavior of Ag(I) on cured tannin cellulose-based aerogels; [固化单宁纤维素基气凝胶吸附还原 Ag(I)行为研究]" . | China Environmental Science 44 . 4 (2024) : 2083-2092 . |
| APA | Chen, Y. , Lin, Y.-L. , Lv, Y.-C. , Liu, Y.-F. , Lin, C.-X. , Ye, X.-X. et al. Study of adsorption reduction behavior of Ag(I) on cured tannin cellulose-based aerogels; [固化单宁纤维素基气凝胶吸附还原 Ag(I)行为研究] . | China Environmental Science , 2024 , 44 (4) , 2083-2092 . |
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The study synthesized nitrogen-doped cobalt oxide precursors using a one-pot hydrothermal method. Three catalysts, N&CoO-Ar, N&CoO-N, and N&CoO-NH, were obtained by calcination under different atmospheric environments (argon, nitrogen, and nitrogen-hydrogen mixture). Characterization results showed that all the prepared materials consisted primarily of carbon components and cobalt oxide, while the catalysts calcined in a nitrogen-hydrogen atmosphere owned the highest content of pyridine nitrogen. Degradation experiments on sulfapyridine (SPD) showed that the N&CoO-NH/PMS system exhibited the best SPD degradation performance (the apparent rate constants were 3.0, 5.1 and 8.3 times larger those of N&CoO-N/PMS, N&CoO-Ar/PMS, and pure CoO/PMS), and was able to rapidly degrade the pollutant within 5 min. The quenching experiments and electrochemical experiments indicated that the nitrogen component modulation improved the chemisorption between PMS and N&CoO-NH and enhanced the electron transfer efficiency between N&CoO-NH/PMS and the pollutant. In addition, the N&CoO-NH/PMS system exhibited good stability and a wide pH applicability. Furthermore, N&CoO-NH/PMS also exhibited good anti-interference performance in the presence of Cl-, HCO3-, NO3-, PO42-, CO32-, and HA, as well as excellent feasibility of treating actual wastewater.
Keyword ：
Cobalt-based catalysts Cobalt-based catalysts Degradation of organic pollutants Degradation of organic pollutants DFT DFT N doping N doping Permonosulfate activation Permonosulfate activation
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| GB/T 7714 | Zou, Lingxiao , Yang, Kai , Hu, Yihui et al. Nitrogen-doped cobalt oxide via atmospheric modulation activates PMS for rapid degradation of organic pollutants: Role of nitrogen fraction on sulfapyridine elimination [J]. | JOURNAL OF WATER PROCESS ENGINEERING , 2024 , 67 . |
| MLA | Zou, Lingxiao et al. "Nitrogen-doped cobalt oxide via atmospheric modulation activates PMS for rapid degradation of organic pollutants: Role of nitrogen fraction on sulfapyridine elimination" . | JOURNAL OF WATER PROCESS ENGINEERING 67 (2024) . |
| APA | Zou, Lingxiao , Yang, Kai , Hu, Yihui , Guo, Xingyu , Li, Xiaojing , Lv, Yuancai et al. Nitrogen-doped cobalt oxide via atmospheric modulation activates PMS for rapid degradation of organic pollutants: Role of nitrogen fraction on sulfapyridine elimination . | JOURNAL OF WATER PROCESS ENGINEERING , 2024 , 67 . |
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以纤维素为原料,在NaOH/尿素/H2O溶解体系中通过交联作用将橡椀单宁固化在纤维素基体上,制得固化橡椀单宁纤维素基气凝胶(VTCA).通过SEM-EDS、FT-IR、XRD等对VTCA进行表征,并研究其对水溶液中Ag(Ⅰ)的吸附行为.结果表明,VTCA具有明显的三维网格多孔结构,孔隙率达到97.95％,在较宽的pH范围内(1～8)对Ag(Ⅰ)均保持较高的吸附效率(＞75％).吸附过程符合拟二级动力学模型和Langmuir吸附等温线模型,温度升高有利于吸附,最高理论吸附量为147.2mg/g.吸附还原研究机理表明,VTCA主要通过静电吸引和螯合作用将Ag(Ⅰ)吸附到其表面,并通过单宁结构上的酚羟基将其原位还原为Ag0,证明VTCA具有良好的吸附还原性能,能够实现对水体中Ag(Ⅰ)的回收.
Keyword ：
Ag(Ⅰ) Ag(Ⅰ) 吸附 吸附 橡椀单宁 橡椀单宁 纤维素基气凝胶 纤维素基气凝胶 还原 还原
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| GB/T 7714 | 陈颖 , 林昱灵 , 吕源财 et al. 固化单宁纤维素基气凝胶吸附还原Ag(Ⅰ)行为研究 [J]. | 中国环境科学 , 2024 , 44 (4) : 2083-2092 . |
| MLA | 陈颖 et al. "固化单宁纤维素基气凝胶吸附还原Ag(Ⅰ)行为研究" . | 中国环境科学 44 . 4 (2024) : 2083-2092 . |
| APA | 陈颖 , 林昱灵 , 吕源财 , 刘以凡 , 林春香 , 叶晓霞 et al. 固化单宁纤维素基气凝胶吸附还原Ag(Ⅰ)行为研究 . | 中国环境科学 , 2024 , 44 (4) , 2083-2092 . |
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