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学者姓名：叶晓霞
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Abstract ：
Para-arsanilic acid (p-ASA) is widely used as a feed additive, making it a pervasive environmental pollutant. Due to its migratory and transformative nature, p-ASA can easily convert into more toxic inorganic arsenic during its migration, thereby increasing the ecological burden and posing a threat to human health. Efficient removal of p- ASA from water is crucial for mitigating arsenic contamination. Efficient removal of p-ASA from water is crucial for mitigating arsenic contamination. This study introduced zirconium-loaded collagen fiber membrane (CFM-Zr), a novel, sustainable membrane adsorption material synthesized by retanning collagen fiber membranes (CFM) with zirconium (Zr). Leveraging the physicochemical properties of CFM and the strong affinity of Zr forp-ASA, CFM-Zr achieved highly efficient p-ASA removal. The resulting membrane was made entirely from green, low-carbon and recyclable raw materials, achieving sustainable removal of p-ASA while realizing the concept of treating waste with waste for environmental recovery. Remarkably, the retanning with zirconium significantly enhanced the Zeta potential of CFM-Zr, strengthening its electrostatic attraction to p-ASA, with a maximum adsorption capacity of 289.02 mg & sdot;g- 1, which was 19.72 times higher than that of the CFM before retanning (13.95 mg & sdot;g-1). Its adsorption rate constant was 12.54 mg & sdot;g-1 & sdot;min- 1. Moreover, CFM-Zr showed good reusability and exhibited electrostatic adsorption and metal coordination effects on the "organic" parts (-OH,-NH2) and "inorganic" parts (As-O) of p-ASA, effectively removing it. This work provided a promising bio-based material for water purification, promoted the sustainable utilization of leather industry waste, and offered significant advancements in environmental remediation and resource recovery.
Keyword ：
Adsorption and separation Adsorption and separation Metal modification Metal modification Waste-to-resource conversion Waste-to-resource conversion Wastewater treatment Wastewater treatment
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| GB/T 7714 | Ye, Xiaoxia , Huang, Jian , Zhang, Yuqing et al. Efficient removal of p-arsanilic acid using a waste-derived collagen fiber-Zr composite membrane [J]. | JOURNAL OF WATER PROCESS ENGINEERING , 2025 , 71 . |
| MLA | Ye, Xiaoxia et al. "Efficient removal of p-arsanilic acid using a waste-derived collagen fiber-Zr composite membrane" . | JOURNAL OF WATER PROCESS ENGINEERING 71 (2025) . |
| APA | Ye, Xiaoxia , Huang, Jian , Zhang, Yuqing , Lin, Yi , Lv, Yuancai , Lin, Chunxiang et al. Efficient removal of p-arsanilic acid using a waste-derived collagen fiber-Zr composite membrane . | JOURNAL OF WATER PROCESS ENGINEERING , 2025 , 71 . |
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以生物大分子淀粉(ST)、海藻酸钠(SA)为骨架,采用溶液聚合法将丙烯酰胺(AM)、2-丙烯酰胺-2-甲基丙磺酸(AMPS)接枝到淀粉-海藻酸钠骨架上,合成耐盐型生物基保水剂.AMPS的加入为体系中引入磺酸基团,使产物的耐盐性提高.通过傅里叶变换红外光谱与 X-射线衍射分析得到生物基与单体成功接枝聚合.利用单因素实验优化工艺条件得出最佳制备方案.性能测试表明,该耐盐型生物基保水剂可重复使用且热稳定性良好,在质量分数为的 0.90%NaCl溶液、0.90%KCl溶液、0.90%NH4Cl溶液中吸液倍率分别为 118 g/g、117 g/g、117 g/g.该研究成功制备出一种成本低、生物可降解且在多种盐溶液中均展现较好的吸液能力的耐盐型生物基保水剂.
Keyword ：
保水剂 保水剂 吸液倍率 吸液倍率 海藻酸钠 海藻酸钠 淀粉 淀粉
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| GB/T 7714 | 黄宇诗 , 陈慧君 , 叶晓霞 et al. 耐盐型淀粉-海藻酸钠二元生物基保水剂的制备与表征及性能研究 [J]. | 纤维素科学与技术 , 2025 , 33 (1) : 31-38 . |
| MLA | 黄宇诗 et al. "耐盐型淀粉-海藻酸钠二元生物基保水剂的制备与表征及性能研究" . | 纤维素科学与技术 33 . 1 (2025) : 31-38 . |
| APA | 黄宇诗 , 陈慧君 , 叶晓霞 , 刘以凡 , 刘明华 . 耐盐型淀粉-海藻酸钠二元生物基保水剂的制备与表征及性能研究 . | 纤维素科学与技术 , 2025 , 33 (1) , 31-38 . |
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Efficient removal of p-arsanilic acid (p-ASA) from contaminated water is crucial for mitigating arsenic contamination. In this study, a membrane adsorbent named CFM-Zn is developed by retanning Zn on a collagen fiber membrane (CFM). This development leverages the unique physicochemical properties of CFM and the strong affinity of Zn for p-ASA. The membrane is composed entirely of green, low-carbon, and recyclable materials, achieving sustainable removal of p-ASA and embodying the concept of using waste to treat waste for environmental recovery. Remarkably, it exhibits an ultra-high capacity of up to 515.46 mg & sdot;g-1. Additionally, CFM-Zn demonstrates moderate reusability, with effectiveness maintained for at least five cycles. This study could advance the development of bio-based materials for water pollutant removal, expand the applications of leather waste, and significantly promote environmental purification and resource recycling.
Keyword ：
Adsorption and separation Adsorption and separation Collagen fiber membrane Collagen fiber membrane Metal modification Metal modification Metal oxides Metal oxides p-arsanilic acid p-arsanilic acid
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| GB/T 7714 | Zheng, Zhihong , Lin, Yi , Lin, Zheyu et al. Green collagen fiber-based organic-inorganic hybrid membrane material for the effective removal of p-arsanilic acid [J]. | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING , 2025 , 13 (3) . |
| MLA | Zheng, Zhihong et al. "Green collagen fiber-based organic-inorganic hybrid membrane material for the effective removal of p-arsanilic acid" . | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING 13 . 3 (2025) . |
| APA | Zheng, Zhihong , Lin, Yi , Lin, Zheyu , Zhang, Dacheng , Lin, Junhan , Ruan, Kailing et al. Green collagen fiber-based organic-inorganic hybrid membrane material for the effective removal of p-arsanilic acid . | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING , 2025 , 13 (3) . |
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《生物质的开发与利用》是资源循环科学与工程专业的核心必修课，是一门知识面广泛、实践性强的交叉学科课程。针对传统教学中存在的问题，教学团队提出了“以学生为中心、产出为导向、持续改进”的教学理念，并通过实施“四维”混合式教学法，对教学内容、方法和考核方式进行了全面的改革。引入科研项目，设计了一系列与课程内容密切相关的实验教学，涉及皮革废弃物（皮胶原纤维膜）改性利用、优化以及乳液分离性能的测试等实验，并对材料的结构和形貌进行表征，使用Origin软件对实验数据进行处理和分析。通过这些改革措施，不仅提高了课程的教学质量，也促进了学生创新能力和综合素质的有效提高。
Keyword ：
实践教学 实践教学 混合式教学 混合式教学 生物质 生物质 皮胶原纤维膜 皮胶原纤维膜 皮革废弃物 皮革废弃物 金属有机框架 金属有机框架
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| GB/T 7714 | 叶晓霞 , 吴秋 , 吕源财 et al. 生物质的开发与利用课程教学改革探讨 [J]. | 皮革科学与工程 , 2025 , 35 (3) : 120-125 . |
| MLA | 叶晓霞 et al. "生物质的开发与利用课程教学改革探讨" . | 皮革科学与工程 35 . 3 (2025) : 120-125 . |
| APA | 叶晓霞 , 吴秋 , 吕源财 , 刘以凡 , 林春香 , 陈杰 . 生物质的开发与利用课程教学改革探讨 . | 皮革科学与工程 , 2025 , 35 (3) , 120-125 . |
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Extracting uranium from seawater has become an important method to supplement the nuclear industry. Herein, we introduce a simple route to load conjugated microporous polymers onto collagen fiber membranes, resulting in a novel membrane adsorbent material (CMPA-F/CFM) for uranium capture. Its Langmuir adsorption capacity reaches 304.9 mg·g−1 (at 318 K), with fast adsorption kinetic of 60 min, and excellent adsorption selectivity with Kd = 4.69 × 104 mL·g−1 under the temperature of 298 K, initial concentration of 50 mg·L-1, and pH = 7, thus allowing a satisfactory adsorption performance in a 7-day real ocean experiment with a uranium adsorption capacity of 1.25 mg·g−1. Furthermore, in continuous dynamic adsorption experiments, CMPA-F/CFM could treat up to 19.0 L·g−1 of low-enriched uranium (LEU) solution (1 mg·L-1), with a uranium removal rate of up to 87.5 % (10 L of seawater). This study demonstrates broad potential application of membrane adsorption in extraction of low-enriched uranium. © 2024 Elsevier Ltd
Keyword ：
Adsorption Adsorption Collagen Collagen Conjugated polymers Conjugated polymers Extraction Extraction Microporosity Microporosity Nuclear industry Nuclear industry Seawater Seawater Uranium Uranium
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| GB/T 7714 | Ye, Xiaoxia , Liu, Juan , Chen, Xueying et al. Effective uranium extraction from seawater through immobilization of conjugated microporous polymers on collagen fiber membrane [J]. | Chemical Engineering Science , 2024 , 295 . |
| MLA | Ye, Xiaoxia et al. "Effective uranium extraction from seawater through immobilization of conjugated microporous polymers on collagen fiber membrane" . | Chemical Engineering Science 295 (2024) . |
| APA | Ye, Xiaoxia , Liu, Juan , Chen, Xueying , Chen, Dongjun , Qian, Zhen , Chen, Jie et al. Effective uranium extraction from seawater through immobilization of conjugated microporous polymers on collagen fiber membrane . | Chemical Engineering Science , 2024 , 295 . |
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China generates over 100 million tons of food waste annually, leading to significant environmental pollution and health risks if not managed properly. Converting FW into a high-value-added platform molecule, lactic acid (LA), through fermentation offers a promising approach for both waste treatment and resource recovery. This paper presents a comprehensive review of recent advancements in LA production from FW, focusing on pure strains fermentation and open fermentation technologies, metabolic mechanisms, and problems in fermentation. It also assesses purification methods, including molecular distillation, adsorption, membrane separation, precipitation, esterification and hydrolysis, solvent extraction, and in-situ separation, analyzing their efficiency, advantages, and disadvantages. However, current research encounters several challenges, including low LA yield, low optical purity of L-(+)-LA, and difficulties in the separation and purification of LA. The integration of in-situ separation technology coupled with multiple separation methods is highlighted as a promising direction for future advancements. © 2024 Elsevier Ltd
Keyword ：
Distillation Distillation
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| GB/T 7714 | Song, Liang , Cai, Chenhang , Chen, Zengpeng et al. Lactic acid production from food waste: Advances in microbial fermentation and separation technologies [J]. | Bioresource Technology , 2024 , 414 . |
| MLA | Song, Liang et al. "Lactic acid production from food waste: Advances in microbial fermentation and separation technologies" . | Bioresource Technology 414 (2024) . |
| APA | Song, Liang , Cai, Chenhang , Chen, Zengpeng , Lin, Chunxiang , Lv, Yuancai , Ye, Xiaoxia et al. Lactic acid production from food waste: Advances in microbial fermentation and separation technologies . | Bioresource Technology , 2024 , 414 . |
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A valonea tannin-immobilized cellulose-based aerogel (VTCA) was prepared by introducing valonea tannin into cellulose through crosslinking reaction in the of NaOH/urea/H2O solvent system. The structure and property of VTCA was characterized by SEM-EDS, FT-IR, XRD, etc., and the adsorption behavior for Ag(I) in aqueous solution was also investigated. The results showed that the three-dimensional VTCA displayed obvious porous structure with a porosity of 97.95%, and exhibited good adsorption efficiency (>75%) for Ag(I) under a wide pH range (1-8). The Ag(I) adsorption process obeyed the pseudo-second-order kinetic model and the Langmuir adsorption isotherm model. High temperature was favorable for adsorption, and the maximum theoretical adsorption capacity was 147.2mg/g. The mechanism of Ag(I) adsorption involved two process: Ag(I) was firstly adsorbed onto the surface of VTCA through the electrostatic attraction and chelation effects, and then in situ reduced to Ag0 by the phenolic hydroxyl group on the tannin structure. All the results revealed that VTCA owned good adsorption and reduction performance and could achieve the recycling of Ag(I) in water. © 2024 Chinese Society for Environmental Sciences. All rights reserved.
Keyword ：
adsorption adsorption Ag(I) Ag(I) cellulose-based aerogel cellulose-based aerogel reduction reduction valonea tannin valonea tannin
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| GB/T 7714 | Chen, Y. , Lin, Y.-L. , Lv, Y.-C. et al. Study of adsorption reduction behavior of Ag(I) on cured tannin cellulose-based aerogels; [固化单宁纤维素基气凝胶吸附还原 Ag(I)行为研究] [J]. | China Environmental Science , 2024 , 44 (4) : 2083-2092 . |
| MLA | Chen, Y. et al. "Study of adsorption reduction behavior of Ag(I) on cured tannin cellulose-based aerogels; [固化单宁纤维素基气凝胶吸附还原 Ag(I)行为研究]" . | China Environmental Science 44 . 4 (2024) : 2083-2092 . |
| APA | Chen, Y. , Lin, Y.-L. , Lv, Y.-C. , Liu, Y.-F. , Lin, C.-X. , Ye, X.-X. et al. Study of adsorption reduction behavior of Ag(I) on cured tannin cellulose-based aerogels; [固化单宁纤维素基气凝胶吸附还原 Ag(I)行为研究] . | China Environmental Science , 2024 , 44 (4) , 2083-2092 . |
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The study synthesized nitrogen-doped cobalt oxide precursors using a one-pot hydrothermal method. Three catalysts, N&CoO-Ar, N&CoO-N, and N&CoO-NH, were obtained by calcination under different atmospheric environments (argon, nitrogen, and nitrogen-hydrogen mixture). Characterization results showed that all the prepared materials consisted primarily of carbon components and cobalt oxide, while the catalysts calcined in a nitrogen-hydrogen atmosphere owned the highest content of pyridine nitrogen. Degradation experiments on sulfapyridine (SPD) showed that the N&CoO-NH/PMS system exhibited the best SPD degradation performance (the apparent rate constants were 3.0, 5.1 and 8.3 times larger those of N&CoO-N/PMS, N&CoO-Ar/PMS, and pure CoO/PMS), and was able to rapidly degrade the pollutant within 5 min. The quenching experiments and electrochemical experiments indicated that the nitrogen component modulation improved the chemisorption between PMS and N&CoO-NH and enhanced the electron transfer efficiency between N&CoO-NH/PMS and the pollutant. In addition, the N&CoO-NH/PMS system exhibited good stability and a wide pH applicability. Furthermore, N&CoO-NH/PMS also exhibited good anti-interference performance in the presence of Cl-, HCO3-, NO3-, PO42-, CO32-, and HA, as well as excellent feasibility of treating actual wastewater.
Keyword ：
Cobalt-based catalysts Cobalt-based catalysts Degradation of organic pollutants Degradation of organic pollutants DFT DFT N doping N doping Permonosulfate activation Permonosulfate activation
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| GB/T 7714 | Zou, Lingxiao , Yang, Kai , Hu, Yihui et al. Nitrogen-doped cobalt oxide via atmospheric modulation activates PMS for rapid degradation of organic pollutants: Role of nitrogen fraction on sulfapyridine elimination [J]. | JOURNAL OF WATER PROCESS ENGINEERING , 2024 , 67 . |
| MLA | Zou, Lingxiao et al. "Nitrogen-doped cobalt oxide via atmospheric modulation activates PMS for rapid degradation of organic pollutants: Role of nitrogen fraction on sulfapyridine elimination" . | JOURNAL OF WATER PROCESS ENGINEERING 67 (2024) . |
| APA | Zou, Lingxiao , Yang, Kai , Hu, Yihui , Guo, Xingyu , Li, Xiaojing , Lv, Yuancai et al. Nitrogen-doped cobalt oxide via atmospheric modulation activates PMS for rapid degradation of organic pollutants: Role of nitrogen fraction on sulfapyridine elimination . | JOURNAL OF WATER PROCESS ENGINEERING , 2024 , 67 . |
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以纤维素为原料,在NaOH/尿素/H2O溶解体系中通过交联作用将橡椀单宁固化在纤维素基体上,制得固化橡椀单宁纤维素基气凝胶(VTCA).通过SEM-EDS、FT-IR、XRD等对VTCA进行表征,并研究其对水溶液中Ag(Ⅰ)的吸附行为.结果表明,VTCA具有明显的三维网格多孔结构,孔隙率达到97.95％,在较宽的pH范围内(1～8)对Ag(Ⅰ)均保持较高的吸附效率(＞75％).吸附过程符合拟二级动力学模型和Langmuir吸附等温线模型,温度升高有利于吸附,最高理论吸附量为147.2mg/g.吸附还原研究机理表明,VTCA主要通过静电吸引和螯合作用将Ag(Ⅰ)吸附到其表面,并通过单宁结构上的酚羟基将其原位还原为Ag0,证明VTCA具有良好的吸附还原性能,能够实现对水体中Ag(Ⅰ)的回收.
Keyword ：
Ag(Ⅰ) Ag(Ⅰ) 吸附 吸附 橡椀单宁 橡椀单宁 纤维素基气凝胶 纤维素基气凝胶 还原 还原
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| GB/T 7714 | 陈颖 , 林昱灵 , 吕源财 et al. 固化单宁纤维素基气凝胶吸附还原Ag(Ⅰ)行为研究 [J]. | 中国环境科学 , 2024 , 44 (4) : 2083-2092 . |
| MLA | 陈颖 et al. "固化单宁纤维素基气凝胶吸附还原Ag(Ⅰ)行为研究" . | 中国环境科学 44 . 4 (2024) : 2083-2092 . |
| APA | 陈颖 , 林昱灵 , 吕源财 , 刘以凡 , 林春香 , 叶晓霞 et al. 固化单宁纤维素基气凝胶吸附还原Ag(Ⅰ)行为研究 . | 中国环境科学 , 2024 , 44 (4) , 2083-2092 . |
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As an emerging micropollutant, p-arsanilic acid (p-ASA) would release highly toxic arsenate and arsenite during migration transformation. Herein, a three-dimensional polyethylenimine-aminated leather collagen fiber (CF-PEI) decorated with MgZnFe (MZF) metal oxides, i.e., CF-PEI@MZF monolith, was reported for the ultradeep p-ASA removal. The synergetic functions of hydrogen bonding and electrostatic interaction from the CF-PEI and coordinative interaction from the MZF on the monolith allow an ultrarapid kinetic that could achieve ca. 80% of the adsorption equilibrium within 20 min and a benchmarked exothermic Langmuir adsorption capacity as high as 588.24 mg g(-1) for the p-ASA. It also performed an unparalleled feasibility in the continuous treatment to reduce the concentration of p-ASA to below 0.05 mg L-1 for real applications. We also highlight the monolith structure with great features of easy separation and recycling use for real industrial applications. All these demonstrate the merits of our CF-PEI@MZF monolith in addressing environmental engineering challenges.
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| GB/T 7714 | Ye, Xiaoxia , Wu, Zhihao , Chi, Ruiyang et al. Enhanced Removal of p-Arsanilic Acid Using a Collagen Fiber-Derived Mg-Zn-Fe Metal Oxide Monolith [J]. | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH , 2024 , 63 (22) : 9790-9799 . |
| MLA | Ye, Xiaoxia et al. "Enhanced Removal of p-Arsanilic Acid Using a Collagen Fiber-Derived Mg-Zn-Fe Metal Oxide Monolith" . | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 63 . 22 (2024) : 9790-9799 . |
| APA | Ye, Xiaoxia , Wu, Zhihao , Chi, Ruiyang , Chen, Jie , Zhou, Jianfei , Shi, Bi . Enhanced Removal of p-Arsanilic Acid Using a Collagen Fiber-Derived Mg-Zn-Fe Metal Oxide Monolith . | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH , 2024 , 63 (22) , 9790-9799 . |
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