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Ultrafast molecular separation through all-biomaterial membranes with a hierarchical configuration and mechanism study SCIE
期刊论文 | 2025 , 361 | SEPARATION AND PURIFICATION TECHNOLOGY
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Abstract :

Traditional nanofiltration membranes allow high rejection of low molecular weight organic matter, yet suffer from a low flux and a high operation pressure, and they pose an environmental concern because they are made of petroleum-based polymers. Herein, a novel environmentally friendly filter membrane for ultrafast molecular separation has been developed using natural and artificial biomaterials as building units. Cellulose micron fibers, a natural biopolymer, serve as a stable substrate for the growth of hydroxyapatite (HAP) nanowire bunches, which are the main inorganic components of bones and teeth. The vertically aligned HAP nanowire bunches provide abundant nanoscale surfaces and confinement space for the attachment of dopamine and subsequently self-polymerization into polydopamine (PDA) sub-micron particles, which are a melanin-like bioactive polymer. On the one hand, the as-built micro-nano hierarchical configuration enables ultrahigh permeance (>6000 L m(-2) h(-1) bar(-1)) through the filter membrane at a low pressure (62 mbar). On the other hand, molecular dynamics simulations reveal that synergy between multiple molecular interactions of HAP and PDA contributes to the universal separation of different organic pollutants from water (i.e., cationic and anionic dyes and antibiotics) at a high removal rate of > 97 %. Overall, this work ingeniously uses biocompatible biomaterials to build a hierarchical filter membrane, thereby enabling ultrafast and efficient molecular separation.

Keyword :

Biomaterials Biomaterials Cellulose Cellulose Filter Membranes Filter Membranes Hydroxyapatite Nanowires Hydroxyapatite Nanowires Polydopamine Polydopamine

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GB/T 7714 Wu, Linhan , Shi, Dehuan , Lin, Fuwang et al. Ultrafast molecular separation through all-biomaterial membranes with a hierarchical configuration and mechanism study [J]. | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 361 .
MLA Wu, Linhan et al. "Ultrafast molecular separation through all-biomaterial membranes with a hierarchical configuration and mechanism study" . | SEPARATION AND PURIFICATION TECHNOLOGY 361 (2025) .
APA Wu, Linhan , Shi, Dehuan , Lin, Fuwang , Chen, Fei-Fei , Yang, Chengkai , Yu, Yan . Ultrafast molecular separation through all-biomaterial membranes with a hierarchical configuration and mechanism study . | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 361 .
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Ultrafast molecular separation through all-biomaterial membranes with a hierarchical configuration and mechanism study EI
期刊论文 | 2025 , 361 | Separation and Purification Technology
Ultrafast molecular separation through all-biomaterial membranes with a hierarchical configuration and mechanism study Scopus
期刊论文 | 2025 , 361 | Separation and Purification Technology
Advancements and challenges in g-C3N4/ZnIn2S4 heterojunction photocatalysts SCIE
期刊论文 | 2025 , 13 (7) , 4718-4745 | JOURNAL OF MATERIALS CHEMISTRY A
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Heterojunction photocatalysts, which consist of two or more semiconductors, have garnered significant attention owing to their extensive benefits, including a broad-spectrum response, efficient carrier separation and migration, as well as robust redox capabilities. Among the myriad of semiconductors, graphitic carbon nitride (g-C3N4) and zinc indium sulfide (ZnIn2S4) have been extensively researched due to their low toxicity, straightforward and scalable synthesis processes, controllable microstructures, and exceptional chemical stability. Recently, there has been a trend towards integrating these two semiconductors to complement each other's strengths. Consequently, a systematic summary and outlook on g-C3N4/ZnIn2S4 heterojunction photocatalysts is both urgent and valuable. This review summarizes the advancements in the g-C3N4/ZnIn2S4 heterojunctions in the last 10 years. We first analyzed the charge-transfer mechanisms in the type-I, type-II, Z-scheme and S-scheme heterojunctions. Then the typical synthesis methods employed for creating g-C3N4/ZnIn2S4 heterojunctions are introduced. Subsequently, we delve into the regulation strategies for g-C3N4/ZnIn2S4 heterojunctions, including morphology optimization, heteroatom doping, defect engineering, and the construction of multinary composites. The design concept and superiorities of these strategies are thoroughly discussed. Following this, we systematically showcase the photocatalytic applications of g-C3N4/ZnIn2S4 heterojunctions, encompassing CO2 reduction, H2 evolution, pollutant degradation, H2O2 production, biomass conversion, photoelectrochemical sensors, and so forth. Last, we propose the challenges that lie ahead in future research endeavors. This comprehensive review is expected to provide an instructive guideline for rational design and applications of g-C3N4/ZnIn2S4 heterojunctions.

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GB/T 7714 Lu, Yongjun , Zhuang, Zanyong , Li, Lingyun et al. Advancements and challenges in g-C3N4/ZnIn2S4 heterojunction photocatalysts [J]. | JOURNAL OF MATERIALS CHEMISTRY A , 2025 , 13 (7) : 4718-4745 .
MLA Lu, Yongjun et al. "Advancements and challenges in g-C3N4/ZnIn2S4 heterojunction photocatalysts" . | JOURNAL OF MATERIALS CHEMISTRY A 13 . 7 (2025) : 4718-4745 .
APA Lu, Yongjun , Zhuang, Zanyong , Li, Lingyun , Chen, Fei-Fei , Wei, Peishu , Yu, Yan . Advancements and challenges in g-C3N4/ZnIn2S4 heterojunction photocatalysts . | JOURNAL OF MATERIALS CHEMISTRY A , 2025 , 13 (7) , 4718-4745 .
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Advancements and challenges in g-C3N4/ZnIn2S4 heterojunction photocatalysts Scopus
期刊论文 | 2025 , 13 (7) , 4718-4745 | Journal of Materials Chemistry A
Advancements and challenges in g-C3N4/ZnIn2S4 heterojunction photocatalysts EI
期刊论文 | 2025 , 13 (7) , 4718-4745 | Journal of Materials Chemistry A
Tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient CO2 photoreduction Scopus
期刊论文 | 2024 , 672 | Applied Surface Science
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Abstract :

Two-dimension nanosheets are ideal photocatalysts for CO2 reduction due to their high exposure of active sites and short charge transfer pathway. However, 2D photocatalysts have a tendency to agglomeration, thus compromising the performance of photocatalytic CO2 reduction. Trees, one of the most important plants for photosynthesis, have a unique “leaf-on-branch” structure. This unique two-dimension/one-dimension (2D/1D) configuration maximizes the adsorption of CO2 molecules and light harvesting. Herein, a tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient photocatalytic CO2 reduction is reported. The cobalt silicate (CoSi) nanosheets (∼0.68 nm) are in situ grown on the surfaces of hydroxyapatite (HAP) nanowires, creating a well-defined 2D/1D hierarchical structure. The vertical alignment of ultrathin CoSi nanosheets on the HAP nanowires effectively suppresses their agglomeration, leading to a large BET surface area (106.45 m2/g) and excellent CO2 adsorption (8.00 cm3 g−1). The results of photoelectrochemical characterization demonstrate that the 2D/1D hierarchical structure is powerful to expedite charge transfer. As a result, the gas generation rate of CO is as high as 28780 μmol g−1 h−1 over the CoSi-on-HAP 2D/1D heterostructure. In addition, the electron transfer mechanism and reaction pathways of CO2 reduction are revealed by in situ irradiated XPS and in situ DRIFT spectra. © 2024 Elsevier B.V.

Keyword :

CO2 reduction CO2 reduction Heterostructure Heterostructure Hydroxyapatite nanowires Hydroxyapatite nanowires Photocatalysis Photocatalysis Silicate nanosheets Silicate nanosheets

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GB/T 7714 Hu, Y. , Zhu, Y. , He, X. et al. Tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient CO2 photoreduction [J]. | Applied Surface Science , 2024 , 672 .
MLA Hu, Y. et al. "Tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient CO2 photoreduction" . | Applied Surface Science 672 (2024) .
APA Hu, Y. , Zhu, Y. , He, X. , Feng, Y.-N. , Chen, F.-F. , Yu, Y. . Tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient CO2 photoreduction . | Applied Surface Science , 2024 , 672 .
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Tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient CO2 photoreduction SCIE
期刊论文 | 2024 , 672 | APPLIED SURFACE SCIENCE
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Abstract :

Two-dimension nanosheets are ideal photocatalysts for CO2 reduction due to their high exposure of active sites and short charge transfer pathway. However, 2D photocatalysts have a tendency to agglomeration, thus compromising the performance of photocatalytic CO2 reduction. Trees, one of the most important plants for photosynthesis, have a unique "leaf-on-branch" structure. This unique two-dimension/one-dimension (2D/1D) configuration maximizes the adsorption of CO2 molecules and light harvesting. Herein, a tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient photocatalytic CO2 reduction is reported. The cobalt silicate (CoSi) nanosheets (similar to 0.68 nm) are in situ grown on the surfaces of hydroxyapatite (HAP) nanowires, creating a well-defined 2D/1D hierarchical structure. The vertical alignment of ultrathin CoSi nanosheets on the HAP nanowires effectively suppresses their agglomeration, leading to a large BET surface area (106.45 m(2)/g) and excellent CO2 adsorption (8.00 cm(3) g(-1)). The results of photoelectrochemical characterization demonstrate that the 2D/1D hierarchical structure is powerful to expedite charge transfer. As a result, the gas generation rate of CO is as high as 28780 mu mol g(-1) h(-1) over the CoSi-on-HAP 2D/1D heterostructure. In addition, the electron transfer mechanism and reaction pathways of CO2 reduction are revealed by in situ irradiated XPS and in situ DRIFT spectra.

Keyword :

CO2 reduction CO2 reduction Heterostructure Heterostructure Hydroxyapatite nanowires Hydroxyapatite nanowires Photocatalysis Photocatalysis Silicate nanosheets Silicate nanosheets

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GB/T 7714 Hu, Yingzi , Zhu, Yan , He, Xi et al. Tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient CO2 photoreduction [J]. | APPLIED SURFACE SCIENCE , 2024 , 672 .
MLA Hu, Yingzi et al. "Tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient CO2 photoreduction" . | APPLIED SURFACE SCIENCE 672 (2024) .
APA Hu, Yingzi , Zhu, Yan , He, Xi , Feng, Ya-Nan , Chen, Fei-Fei , Yu, Yan . Tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient CO2 photoreduction . | APPLIED SURFACE SCIENCE , 2024 , 672 .
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Tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient CO2 photoreduction Scopus
期刊论文 | 2024 , 672 | Applied Surface Science
Tree-inspired semiconductor-on-ceramic 2D/1D heterostructure for efficient CO2 photoreduction EI
期刊论文 | 2024 , 672 | Applied Surface Science
2D/3D NiAl-LDH/ZnIn2S4复合材料的制备及光催化CO2还原性能
期刊论文 | 2024 , (23) , 161-163 | 当代化工研究
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Abstract :

通过光催化CO2 还原实现CO2 减排和高值利用是目前科学研究的热点问题.设计合成了 2D/3D NiAl-LDH/ZnIn2S4 复合材料,电化学阻抗谱和瞬态光电流测试结果表明,NiAl-LDH和ZnIn2S4 二者之间紧密的界面接触和异质结的构筑显著促进光生电子的界面转移,从而增强光催化CO2 还原效率.2D/3D NiAl-LDH/ZnIn2S4 复合材料的CO产量分别是单相ZnIn2S4 和NiAl-LDH的23.8倍和1.7倍.

Keyword :

CO2还原 CO2还原 ZnIn2S4 ZnIn2S4 光催化 光催化 层状双金属氢氧化物 层状双金属氢氧化物

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GB/T 7714 杨霁航 , 陈飞飞 . 2D/3D NiAl-LDH/ZnIn2S4复合材料的制备及光催化CO2还原性能 [J]. | 当代化工研究 , 2024 , (23) : 161-163 .
MLA 杨霁航 et al. "2D/3D NiAl-LDH/ZnIn2S4复合材料的制备及光催化CO2还原性能" . | 当代化工研究 23 (2024) : 161-163 .
APA 杨霁航 , 陈飞飞 . 2D/3D NiAl-LDH/ZnIn2S4复合材料的制备及光催化CO2还原性能 . | 当代化工研究 , 2024 , (23) , 161-163 .
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Synergistic Effect of GO and MXene Enables Ultrasensitive, Reversible, and Self-Powered Fire Warning of a GO/MXene/Chitosan Aerogel SCIE
期刊论文 | 2024 , 16 (43) , 59346-59357 | ACS APPLIED MATERIALS & INTERFACES
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Abstract :

Graphene oxide (GO)-based fire alarm materials have garnered extensive attention because the thermal reduction of GO to reduced GO (RGO) enables rapid fire warning. However, they suffer from poor flame retardancy, irreversible fire warning, and dependence on an external power supply. Herein, a GO/MXene/chitosan aerogel with a low density of 0.018 g cm(-3) and good compressibility has been developed. The experimental results demonstrate that (i) MXene effectively reduces the peak and mean heat release rate of GO, while RGO nanosheets compensate for the structural instability of MXene in the flame due to thermal oxidation into TiO2; as such, long-lasting fire warning (>120 s) has been achieved; (ii) the reducibility and conductivity of MXene contribute to the ultrasensitive response of GO, with a fire response time of 1 s; and (iii) notably, the thermoelectric effect of MXene enables the reversible and self-powered fire warning of the GO/MXene/CS aerogel without an external power supply. Compared to pure MXene/CS aerogel, the presence of GO improves the sensitivity and stability of self-powered fire warning, owing to the formation of the highly conductive RGO nanosheets. The results of this work highlight the cooperation between GO and MXene in realizing ultrasensitive, long-lasting, reversible, and self-powered fire warning.

Keyword :

aerogel aerogel firewarning firewarning flame retardancy flame retardancy graphene oxide graphene oxide MXene MXene

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GB/T 7714 He, Xi , Xu, Yaozheng , Wang, Yuan et al. Synergistic Effect of GO and MXene Enables Ultrasensitive, Reversible, and Self-Powered Fire Warning of a GO/MXene/Chitosan Aerogel [J]. | ACS APPLIED MATERIALS & INTERFACES , 2024 , 16 (43) : 59346-59357 .
MLA He, Xi et al. "Synergistic Effect of GO and MXene Enables Ultrasensitive, Reversible, and Self-Powered Fire Warning of a GO/MXene/Chitosan Aerogel" . | ACS APPLIED MATERIALS & INTERFACES 16 . 43 (2024) : 59346-59357 .
APA He, Xi , Xu, Yaozheng , Wang, Yuan , Wu, Linhan , Chen, Fei-Fei , Yu, Yan . Synergistic Effect of GO and MXene Enables Ultrasensitive, Reversible, and Self-Powered Fire Warning of a GO/MXene/Chitosan Aerogel . | ACS APPLIED MATERIALS & INTERFACES , 2024 , 16 (43) , 59346-59357 .
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Synergistic Effect of GO and MXene Enables Ultrasensitive, Reversible, and Self-Powered Fire Warning of a GO/MXene/Chitosan Aerogel Scopus
期刊论文 | 2024 , 16 (43) , 59346-59357 | ACS Applied Materials and Interfaces
Synergistic Effect of GO and MXene Enables Ultrasensitive, Reversible, and Self-Powered Fire Warning of a GO/MXene/Chitosan Aerogel EI
期刊论文 | 2024 , 16 (43) , 59346-59357 | ACS Applied Materials and Interfaces
柔性超疏水钙钛矿复合纸及光致发光性能
期刊论文 | 2024 , 53 (12) , 2860-2863,2981 | 当代化工
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Abstract :

卤化物钙钛矿在下一代照明设备中展现出广阔的前景.然而,钙钛矿纳米晶存在柔性和水稳定性差的问题.使用羟基磷灰石(HA)纳米线作为柔性框架负载CsPbBr3 钙钛矿纳米晶,随后进行聚二甲基硅氧烷(PDMS)表面改性,制备出兼具柔性和超疏水表面的钙钛矿复合纸.所制备的 HA/CsPbBr3/PDMS 复合纸展现出卓越的柔韧性,在物理变形后可维持结构稳定.HA/CsPbBr3/PDMS 复合纸具有超疏水表面,水接触角达到151°.因此,在水中浸泡5 h后,复合纸的光致发光发射峰强度仍能保持初始值的98%,在紫外光(365 nm)照射下发射出明亮、均匀的绿色荧光.

Keyword :

光致发光 光致发光 复合材料 复合材料 纳米材料 纳米材料 表面 表面 超疏水 超疏水 钙钛矿 钙钛矿

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GB/T 7714 杨霁航 , 戴子豪 , 陈飞飞 . 柔性超疏水钙钛矿复合纸及光致发光性能 [J]. | 当代化工 , 2024 , 53 (12) : 2860-2863,2981 .
MLA 杨霁航 et al. "柔性超疏水钙钛矿复合纸及光致发光性能" . | 当代化工 53 . 12 (2024) : 2860-2863,2981 .
APA 杨霁航 , 戴子豪 , 陈飞飞 . 柔性超疏水钙钛矿复合纸及光致发光性能 . | 当代化工 , 2024 , 53 (12) , 2860-2863,2981 .
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Antibacterial Activity of M-MOF Nanomaterials (M = Fe, Co, Ni, Cu, and Zn): Impact of Metal Centers SCIE
期刊论文 | 2024 , 7 (21) , 24571-24580 | ACS APPLIED NANO MATERIALS
WoS CC Cited Count: 2
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Abstract :

Bacterial infections result in significant burdens on public health, especially with the increasing prevalence of antibiotic resistance owing to the overuse of antibiotics. The development of the next-generation nanoantibacterial materials as alternatives to antibiotics is urgently needed. Metal-organic frameworks (MOFs) have been emerging as promising antibacterial materials. However, the impact of metal centers on the properties and antibacterial activity of MOFs has not been clarified to date. In this work, five M-MOF nanomaterials (M = Fe, Co, Ni, Cu, Zn) are synthesized with 2-methylimidazole as an organic ligand. Subsequently, the minimum inhibitory concentration (MIC), minimum bactericidal concentration, and time-kill curves are studied to evaluate their antibacterial activity. In addition, the destruction of the bacterial cells after treatment with M-MOFs is observed via scanning electron microscopy. The experimental results demonstrate that the Co-MOF and Zn-MOF polyhedra exhibit optimal antibacterial activity. They can effectively inhibit the growth of both Gram-negative bacteria Escherichia coli and Gram-positive bacteria Staphylococcus aureus at a low concentration. On the other hand, the Fe-MOF irregular particles show the weakest antibacterial activity among five M-MOFs and the antibacterial activity of the Ni-MOF and Cu-MOF nanosheets are comparable to each other. The huge difference in antibacterial activity of M-MOFs is attributed to the difference in the shape and size, specific surface area, surface charge, ion release, and production of reactive oxygen species. Overall, this study clarifies the relationship between metal centers in M-MOFs and their antibacterial activity.

Keyword :

2-methylimidazole 2-methylimidazole antibacterial antibacterial metal-organic frameworks metal-organic frameworks nanoantibacterial agents nanoantibacterial agents transitionmetals transitionmetals

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GB/T 7714 Ding, Ao , He, Yupeng , Chen, Fei-Fei et al. Antibacterial Activity of M-MOF Nanomaterials (M = Fe, Co, Ni, Cu, and Zn): Impact of Metal Centers [J]. | ACS APPLIED NANO MATERIALS , 2024 , 7 (21) : 24571-24580 .
MLA Ding, Ao et al. "Antibacterial Activity of M-MOF Nanomaterials (M = Fe, Co, Ni, Cu, and Zn): Impact of Metal Centers" . | ACS APPLIED NANO MATERIALS 7 . 21 (2024) : 24571-24580 .
APA Ding, Ao , He, Yupeng , Chen, Fei-Fei , Yu, Yan . Antibacterial Activity of M-MOF Nanomaterials (M = Fe, Co, Ni, Cu, and Zn): Impact of Metal Centers . | ACS APPLIED NANO MATERIALS , 2024 , 7 (21) , 24571-24580 .
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Antibacterial Activity of M-MOF Nanomaterials (M = Fe, Co, Ni, Cu, and Zn): Impact of Metal Centers Scopus
期刊论文 | 2024 , 7 (21) , 24571-24580 | ACS Applied Nano Materials
Antibacterial Activity of M-MOF Nanomaterials (M = Fe, Co, Ni, Cu, and Zn): Impact of Metal Centers EI
期刊论文 | 2024 , 7 (21) , 24571-24580 | ACS Applied Nano Materials
Vertical MOF film supported on an organic-inorganic mixed substrate for complex wastewater purification SCIE
期刊论文 | 2024 , 652 | APPLIED SURFACE SCIENCE
WoS CC Cited Count: 9
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Abstract :

Flexible metal-organic framework (MOF) films are greatly desired for the separation of hazardous molecules and ions from wastewater. The current MOF films are usually horizontally deposited on the substrates, and thus restricted by brittleness, low exposure of surface area, as well as poor separation functions. Here, an organic-inorganic mixed substrate is firstly fabricated by growing hydroxyapatite (HA) nanowire arrays on the cellulose fiber (CF). Subsequently, MIL-100(Fe) nanocrystals are assembled on the surfaces of HA nanowire arrays through a layer-by-layer manner, leading to a unique vertical MOF film. The resulting vertical MOF films show competitive advantages over the horizontal counterparts: (i) they show excellent flexibility and they are tolerant to serious physical damage; (ii) they have multiple separation functions including ion exchange of HA, excellent adsorption of MOFs, and strong electrostatic interaction of CF; and (iii) the agglomeration of MIL-100(Fe) nanocrystals is effectively suppressed. Therefore, the average roughness, specific surface area, and average pore size of films are optimized. As a result, the vertical MOF films show universal separation of positively/ negatively-charged dyes and Pb2+ ion, with high removal rates of > 94 %. More appealing, the mixed pollutants in the complex wastewater can be one-step separated through the vertical MOF films, with high removal rates of > 96 %.

Keyword :

Dyes Dyes Heavy metal ions Heavy metal ions Hydroxyapatite Hydroxyapatite Metal -organic frameworks Metal -organic frameworks Separation Separation

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GB/T 7714 Gan, Wenxiu , Zheng, Ziyang , Yan, Jiawei et al. Vertical MOF film supported on an organic-inorganic mixed substrate for complex wastewater purification [J]. | APPLIED SURFACE SCIENCE , 2024 , 652 .
MLA Gan, Wenxiu et al. "Vertical MOF film supported on an organic-inorganic mixed substrate for complex wastewater purification" . | APPLIED SURFACE SCIENCE 652 (2024) .
APA Gan, Wenxiu , Zheng, Ziyang , Yan, Jiawei , He, Xi , Zhuang, Zanyong , Chen, Fei-Fei et al. Vertical MOF film supported on an organic-inorganic mixed substrate for complex wastewater purification . | APPLIED SURFACE SCIENCE , 2024 , 652 .
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Vertical MOF film supported on an organic–inorganic mixed substrate for complex wastewater purification EI
期刊论文 | 2024 , 652 | Applied Surface Science
Vertical MOF film supported on an organic–inorganic mixed substrate for complex wastewater purification Scopus
期刊论文 | 2024 , 652 | Applied Surface Science
MOF-derived Co3O4/ZrO2 mesoporous octahedrons with optimized charge transfer and intermediate conversion for efficient CO2 photoreduction SCIE CSCD
期刊论文 | 2024 , 67 (2) , 588-597 | SCIENCE CHINA-MATERIALS
WoS CC Cited Count: 6
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Abstract :

Regulating charge transfer and reaction pathways are effective strategies for boosting photocatalytic CO2 reduction. Herein, Co3O4/ZrO2 mesoporous octahedrons are synthesized through facile pyrolysis of UIO-66@ZIF-67 core/shell octahedrons. The as-obtained Co3O4/ZrO2 mesoporous octahedrons are assembled by highly dispersive and small-sized nanoparticles, with 13 nm average particle size and 5.8 nm pore width, leading to a high specific surface area of 43.11 m(2) g(-1). Benefiting from active-site engineering, the charge-transfer kinetics and CO2 adsorption are successfully enhanced. In addition, density functional theory calculations reveal that ZrO2 tailors the reaction pathway of CO2 reduction by promoting CO2 activation to *CO2 and intermediate formation (*COOH and *CO), as well as decreasing the energy barrier of the rate-limiting step (*CO -> CO). Thus, the Co3O4/ZrO2 mesoporous octahedrons afford a turnover frequency of 28.82 h(-1), 16.95-fold larger than pure Co3O4.

Keyword :

CO2 reduction CO2 reduction mesoporous mesoporous metal-organic frameworks metal-organic frameworks oxides oxides photocatalysis photocatalysis

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GB/T 7714 Liu, Haibing , Qiu, Yanbin , Gan, Wenxiu et al. MOF-derived Co3O4/ZrO2 mesoporous octahedrons with optimized charge transfer and intermediate conversion for efficient CO2 photoreduction [J]. | SCIENCE CHINA-MATERIALS , 2024 , 67 (2) : 588-597 .
MLA Liu, Haibing et al. "MOF-derived Co3O4/ZrO2 mesoporous octahedrons with optimized charge transfer and intermediate conversion for efficient CO2 photoreduction" . | SCIENCE CHINA-MATERIALS 67 . 2 (2024) : 588-597 .
APA Liu, Haibing , Qiu, Yanbin , Gan, Wenxiu , Zhuang, Guoxin , Chen, Fei-Fei , Yang, Chengkai et al. MOF-derived Co3O4/ZrO2 mesoporous octahedrons with optimized charge transfer and intermediate conversion for efficient CO2 photoreduction . | SCIENCE CHINA-MATERIALS , 2024 , 67 (2) , 588-597 .
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MOF-derived Co3O4/ZrO2 mesoporous octahedrons with optimized charge transfer and intermediate conversion for efficient CO2 photoreduction; [MOF衍生Co3O4/ZrO2介孔八面体: 优化电荷转移和中间体转化用于高效CO2光还原] Scopus CSCD
期刊论文 | 2024 , 67 (2) , 588-597 | Science China Materials
MOF-derived Co3O4/ZrO2 mesoporous octahedrons with optimized charge transfer and intermediate conversion for efficient CO2 photoreduction EI CSCD
期刊论文 | 2024 , 67 (2) , 588-597 | Science China Materials
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