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author:

Yang, Liyang (Yang, Liyang.) [1] (Scholars:杨丽阳) | Chen, Wei (Chen, Wei.) [2] | Zhuang, Wan-E (Zhuang, Wan-E.) [3] | Cheng, Qiong (Cheng, Qiong.) [4] | Li, Wenxin (Li, Wenxin.) [5] | Wang, Hui (Wang, Hui.) [6] | Guo, Weidong (Guo, Weidong.) [7] | Chen, Chen-Tung Arthur (Chen, Chen-Tung Arthur.) [8] | Liu, Minghua (Liu, Minghua.) [9]

Indexed by:

Scopus SCIE

Abstract:

Rainwater brings considerable amounts of dissolved organic matter (DOM) from atmosphere to freshwater and marine environments, but little is known about the chemical composition and bioavailability of rainwater DOM. The quantity, quality, and bioavailability of DOM were investigated for 21 rain events at a coastal site in southeast China, using dissolved organic carbon (DOC) measurements, absorption spectroscopy, and fluorescence excitation-emission matrices-parallel factor analysis (EEM-PARAFAC). The DOC concentration ranged from 35 to 457 mu M, which was affected by the prevailing monsoon, rainfall amount and terrestrial/anthropogenic inputs. The volume-weighted average DOC was 118 mu M, corresponding to a rainwater DOC flux of 1.98 g m(-2) yr(-1), Four fluorescent components were identified with EEM-PARAFAC, including three humic-like components (C1-C3) and one tyrosine-like component C4. Absorption coefficient (a(CDOM)(300)) and fluorescence intensities of C2-C4 strongly correlated with DOC, indicating they can be used for DOC estimation. Rainwater DOM was characterized by low DOC-specific UV absorbance (SUVA(254)) and humification index (HIX, which indicated a low aromaticity and humification degree. Principal component analysis (PCA) based on DOM indices revealed two principal factors, which were related to the DOM concentration and humification degree respectively. PCA, together with air-mass trajectory analysis, successfully separated different rain events with variable inputs from living plants/local sources, soil organic matter/humifiecl materials, and the marine source, Rainwater DOM generally showed a high bioavailability of 50% +/- 19%, with higher degradability of non-chromophoric constituents and C1-C2 than other components. This study demonstrated the applicability of absorption and EEM-PARAFAC combined with PCA and air-mass trajectory analysis in differentiating rain events and tracking organic matter sources, and revealed different effects of microbial degradation on individual PARAFAC components in rainwater.

Keyword:

Absorption spectroscopy Bioavaliability Dissolved organic matter EEM-PARAFAC Rainwater

Community:

  • [ 1 ] [Yang, Liyang]Fuzhou Univ, Coll Environm & Resources, Fuzhou, Fujian, Peoples R China
  • [ 2 ] [Chen, Wei]Fuzhou Univ, Coll Environm & Resources, Fuzhou, Fujian, Peoples R China
  • [ 3 ] [Cheng, Qiong]Fuzhou Univ, Coll Environm & Resources, Fuzhou, Fujian, Peoples R China
  • [ 4 ] [Li, Wenxin]Fuzhou Univ, Coll Environm & Resources, Fuzhou, Fujian, Peoples R China
  • [ 5 ] [Wang, Hui]Fuzhou Univ, Coll Environm & Resources, Fuzhou, Fujian, Peoples R China
  • [ 6 ] [Liu, Minghua]Fuzhou Univ, Coll Environm & Resources, Fuzhou, Fujian, Peoples R China
  • [ 7 ] [Zhuang, Wan-E]Fujian Agr & Forestry Univ, Coll Life Sci, Fuzhou, Fujian, Peoples R China
  • [ 8 ] [Guo, Weidong]Xiamen Univ, State Key Lab Marine Environm Sci, Xiamen, Fujian, Peoples R China
  • [ 9 ] [Chen, Chen-Tung Arthur]Natl Sun Yat Sen Univ, Dept Oceanog, Kaohsiung, Taiwan

Reprint 's Address:

  • 杨丽阳 刘明华

    [Yang, Liyang]Fuzhou Univ, Coll Environm & Resources, Fuzhou, Fujian, Peoples R China;;[Liu, Minghua]Fuzhou Univ, Coll Environm & Resources, Fuzhou, Fujian, Peoples R China

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Source :

ESTUARINE COASTAL AND SHELF SCIENCE

ISSN: 0272-7714

Year: 2019

Volume: 217

Page: 45-55

2 . 3 3 3

JCR@2019

2 . 6 0 0

JCR@2023

ESI Discipline: PLANT & ANIMAL SCIENCE;

ESI HC Threshold:103

JCR Journal Grade:2

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 58

SCOPUS Cited Count: 64

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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