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Abstract:
Tb2Ti2O7 (TTO) single crystal with dimensions of 20 x 20 x 16 mm(3) was grown by the Czochralski method. Rietveld structure refinement of X-ray diffraction (XRD) data confirms that the compound crystallizes in the cubic system with pyrochlore structure. Transmission spectra, Magnetic circular dichroism (MCD) spectra, Faraday and inverse Faraday characteristics of TTO crystal have been measured and analyzed in detail. The results demonstrate that TTO crystal has high transmittance at 700-1400 nm waveband and a larger Verdat constant than that of TGG reported. Magnetic circular dichroism (MCD) spectra showed that the 4f -> 4f transitions of Tb3+ have significant contributions to the magneto-optical activity (MOA). In the time-resolved pump-probe spectroscopy, the rotation signals of the probe beam based on the inverse Faraday effect in magneto-optical crystal were observed at zero time delay, the full width at half maximum of the rotation and ellipticity signals can be as fast as similar to 500 fs, which indicates that TTO crystal can be a promising material for ultrafast all-optical magnetic switching. (C) 2016 Optical Society of America
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OPTICS EXPRESS
ISSN: 1094-4087
Year: 2016
Issue: 6
Volume: 24
Page: 5734-5743
3 . 3 0 7
JCR@2016
3 . 2 0 0
JCR@2023
ESI Discipline: PHYSICS;
ESI HC Threshold:186
JCR Journal Grade:1
CAS Journal Grade:2
Cited Count:
WoS CC Cited Count: 18
SCOPUS Cited Count: 19
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 1
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