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author:

Liang, Ruowen (Liang, Ruowen.) [1] | Huang, Renkun (Huang, Renkun.) [2] | Wang, Xuxu (Wang, Xuxu.) [3] | Ying, Shaoming (Ying, Shaoming.) [4] | Yan, Guiyang (Yan, Guiyang.) [5] | Wu, Ling (Wu, Ling.) [6]

Indexed by:

EI

Abstract:

A family of functionalized MIL-68(In) have been successfully synthesized and applied to photoreduction of Cr(VI) aqueous under simulated sunlight (280 nm 2BDC, H2BDC-NH2, H2BDC-NO2 and H2BDC-Br) on photocatalytic performance of MIL-68(In)-X (X = H, NH2, NO2, Br). Further experimental results demonstrated that the photoactivities of the obtained MIL-68(In)-X have been greatly affected by the electronic effect of ligand substituent. That is, the reaction rates obtained by functionalized MIL-68(In) have been linearly associated with the Hammett coefficients of different substituents. More significantly, MIL-68(In)-NH2 has also exhibited outstanding performance in a co-existed model system (Cr(VI)/dyes), which represents a first example to use the In-based MOFs as bifunctional photocatalysts. It is hope that this work not only represents the structure-property relationships on photocatalysis in MOFs, but also promotes further interest in design and construction of more efficient MOFs-based photocatalysts for environmental remediation. © 2018 Elsevier B.V.

Keyword:

Chromium compounds Ligands Nitrogen oxides Reaction rates Wastewater treatment

Community:

  • [ 1 ] [Liang, Ruowen]Province University Key Laboratory of Green Energy and Environment Catalysis, Ningde Normal University, Ningde; 352100, China
  • [ 2 ] [Liang, Ruowen]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou; 350002, China
  • [ 3 ] [Huang, Renkun]Province University Key Laboratory of Green Energy and Environment Catalysis, Ningde Normal University, Ningde; 352100, China
  • [ 4 ] [Wang, Xuxu]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou; 350002, China
  • [ 5 ] [Ying, Shaoming]Fujian Provincial Key Laboratory of Featured Materials in Biochemical Industry, Ningde Normal University, Ningde; 352100, China
  • [ 6 ] [Yan, Guiyang]Province University Key Laboratory of Green Energy and Environment Catalysis, Ningde Normal University, Ningde; 352100, China
  • [ 7 ] [Wu, Ling]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou; 350002, China

Reprint 's Address:

  • [yan, guiyang]province university key laboratory of green energy and environment catalysis, ningde normal university, ningde; 352100, china

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Source :

Applied Surface Science

ISSN: 0169-4332

Year: 2019

Volume: 464

Page: 396-403

6 . 1 8 2

JCR@2019

6 . 3 0 0

JCR@2023

ESI HC Threshold:236

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 75

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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