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author:

Huang, Haowei (Huang, Haowei.) [1] | Weng, Bo (Weng, Bo.) [2] | Zhang, Hongwen (Zhang, Hongwen.) [3] | Lai, Feili (Lai, Feili.) [4] | Long, Jinlin (Long, Jinlin.) [5] (Scholars:龙金林) | Hofkens, Johan (Hofkens, Johan.) [6] | Douthwaite, Richard E. (Douthwaite, Richard E..) [7] | Steele, Julian A. (Steele, Julian A..) [8] | Roeffaers, Maarten B. J. (Roeffaers, Maarten B. J..) [9]

Indexed by:

EI SCIE

Abstract:

Sunlight is an abundant and clean energy source, the harvesting of which could make a significant contribution to society's increasing energy demands. Metal halide perovskites (MHP) have recently received attention for solar fuel generation through photocatalysis and solar-driven electrocatalysis. However, MHP photocatalysis is limited by low solar energy conversion efficiency, poor stability, and impractical reaction conditions. Compared to photocatalysis, MHP solar-driven electrocatalysis not only exhibits higher solar conversion efficiency but also is more stable when operating under practical reaction conditions. In this Perspective, we outline three leading types of MHP solar-driven electrocatalysis device technologies now in the research spotlight, namely, (1) photovoltaic-electrochemical (PV-EC), (2) photovoltaic-photoelectrochemical (PV-PEC), and (3) photoelectrochemical (PEC) approaches for solar-to-fuel reactions, including water-splitting and the CO2 reduction reaction. In addition, we compare each technology to show their relative technical advantages and limitations and highlight promising research directions for the rapidly emerging scientific field of MHP-based solar-driven electrocatalysis.

Keyword:

Community:

  • [ 1 ] [Huang, Haowei]Katholieke Univ Leuven, Dept Microbial & Mol Syst, cMACS, B-3001 Leuven, Belgium
  • [ 2 ] [Weng, Bo]Katholieke Univ Leuven, Dept Microbial & Mol Syst, cMACS, B-3001 Leuven, Belgium
  • [ 3 ] [Zhang, Hongwen]Katholieke Univ Leuven, Dept Microbial & Mol Syst, cMACS, B-3001 Leuven, Belgium
  • [ 4 ] [Steele, Julian A.]Katholieke Univ Leuven, Dept Microbial & Mol Syst, cMACS, B-3001 Leuven, Belgium
  • [ 5 ] [Roeffaers, Maarten B. J.]Katholieke Univ Leuven, Dept Microbial & Mol Syst, cMACS, B-3001 Leuven, Belgium
  • [ 6 ] [Lai, Feili]Katholieke Univ Leuven, Dept Chem, B-3001 Heverlee, Belgium
  • [ 7 ] [Hofkens, Johan]Katholieke Univ Leuven, Dept Chem, B-3001 Heverlee, Belgium
  • [ 8 ] [Long, Jinlin]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350116, Peoples R China
  • [ 9 ] [Douthwaite, Richard E.]Univ York, Dept Chem, York YO10 5DD, N Yorkshire, England

Reprint 's Address:

  • [Steele, Julian A.]Katholieke Univ Leuven, Dept Microbial & Mol Syst, cMACS, B-3001 Leuven, Belgium;;[Roeffaers, Maarten B. J.]Katholieke Univ Leuven, Dept Microbial & Mol Syst, cMACS, B-3001 Leuven, Belgium;;[Douthwaite, Richard E.]Univ York, Dept Chem, York YO10 5DD, N Yorkshire, England

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Source :

JOURNAL OF PHYSICAL CHEMISTRY LETTERS

ISSN: 1948-7185

Year: 2021

Issue: 1

Volume: 13

Page: 25-41

6 . 8 8 8

JCR@2021

4 . 9 0 0

JCR@2023

ESI Discipline: CHEMISTRY;

ESI HC Threshold:117

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 17

SCOPUS Cited Count: 16

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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