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author:

Gao, Hongjin (Gao, Hongjin.) [1] | Qie, Yuan (Qie, Yuan.) [2] | Zhao, Haobing (Zhao, Haobing.) [3] | Li, Fushan (Li, Fushan.) [4] | Guo, Tailiang (Guo, Tailiang.) [5] | Hu, Hailong (Hu, Hailong.) [6]

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EI

Abstract:

We report here high-efficiency, high-resolution quantum dot (QD) light-emitting diodes patterned by ultraviolet-induced ligand exchange. A ligand passivation strategy is carried out to remove the surface defects of QDs after patterning, and thus the device efficiency shows more than 3-fold increase. Moreover, in order to reduce the leakage current occurring in the non-luminance area between QD arrays, a polymethyl methacrylate film is inserted as a charge barrier layer to separate the hole- and electron-transport layers from direct contact. As a result, the leakage current of the devices is effectively decreased. By optimizing the ligand passivation and synergistically suppressing the leakage current, the device with 5-μm diameter QD arrays exhibits luminance over 125000 cd/m2 and maximum external quantum efficiency of 10.5%. This work provides a feasible way to achieving high resolution, high-performance quantum dot light-emitting diodes for next-generation display applications. © 2022 Elsevier B.V.

Keyword:

Electron transport properties Ligands Luminance Nanocrystals Organic light emitting diodes (OLED) Passivation Quantum efficiency Semiconductor quantum dots Surface defects

Community:

  • [ 1 ] [Gao, Hongjin]Institute of Optoelectronic Technology, Fuzhou University, Fuzhou; 350108, China
  • [ 2 ] [Qie, Yuan]Institute of Optoelectronic Technology, Fuzhou University, Fuzhou; 350108, China
  • [ 3 ] [Zhao, Haobing]Institute of Optoelectronic Technology, Fuzhou University, Fuzhou; 350108, China
  • [ 4 ] [Li, Fushan]Institute of Optoelectronic Technology, Fuzhou University, Fuzhou; 350108, China
  • [ 5 ] [Li, Fushan]Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China, Fuzhou; 350108, China
  • [ 6 ] [Guo, Tailiang]Institute of Optoelectronic Technology, Fuzhou University, Fuzhou; 350108, China
  • [ 7 ] [Guo, Tailiang]Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China, Fuzhou; 350108, China
  • [ 8 ] [Hu, Hailong]Institute of Optoelectronic Technology, Fuzhou University, Fuzhou; 350108, China
  • [ 9 ] [Hu, Hailong]Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China, Fuzhou; 350108, China

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Source :

Organic Electronics

ISSN: 1566-1199

Year: 2022

Volume: 108

3 . 2

JCR@2022

2 . 7 0 0

JCR@2023

ESI HC Threshold:55

JCR Journal Grade:2

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 14

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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