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author:

Fang, Biyun (Fang, Biyun.) [1] | Zhang, Chuanfeng (Zhang, Chuanfeng.) [2] | Qi, Zeliang (Qi, Zeliang.) [3] | Li, Chunyan (Li, Chunyan.) [4] | Ni, Jun (Ni, Jun.) [5] (Scholars:倪军) | Wang, Xiuyun (Wang, Xiuyun.) [6] (Scholars:王秀云) | Lin, Jianxin (Lin, Jianxin.) [7] (Scholars:林建新) | Au, Chak-Tong (Au, Chak-Tong.) [8] | Lin, Bingyu (Lin, Bingyu.) [9] (Scholars:林炳裕) | Jiang, Lilong (Jiang, Lilong.) [10] (Scholars:江莉龙)

Indexed by:

EI Scopus SCIE

Abstract:

The design of an efficient non-noble metal catalyst is of burgeoning interest for ammonia synthesis. Herein, we report a Mo2C/CeO2 catalyst that is superior in ammonia synthesis activity. In this catalyst, molybdenum carbide coexisted with the ceria overlayers which is from the ceria support as the strong metal-support interaction. There is a high proportion of low-valent Mo species, as well as high concentration of Ce3+ and surface oxygen species. The presence of Mo2C and CeO2 overlayers not only leads to enhancement of hydrogen and nitrogen adsorption, but also facilitates the desorption and exchange of adsorbed species with the gaseous reagents. Compared with the Mo/CeO2 catalyst prepared without carbonization, the Mo2C/CeO2 catalyst is more than sevenfold higher in ammonia synthesis rate. This work not only presents an explicit example of designing Mo-based catalyst that is highly efficient for ammonia synthesis by tuning the adsorption and desorption properties of the reactant gases, but opens a perspective for other elements in ammonia synthesis.

Keyword:

ammonia synthesis ceria molybdenum carbide

Community:

  • [ 1 ] [Fang, Biyun]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Coll Chem Engn, Fuzhou 350002, Fujian, Peoples R China
  • [ 2 ] [Zhang, Chuanfeng]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Coll Chem Engn, Fuzhou 350002, Fujian, Peoples R China
  • [ 3 ] [Qi, Zeliang]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Coll Chem Engn, Fuzhou 350002, Fujian, Peoples R China
  • [ 4 ] [Li, Chunyan]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Coll Chem Engn, Fuzhou 350002, Fujian, Peoples R China
  • [ 5 ] [Ni, Jun]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Coll Chem Engn, Fuzhou 350002, Fujian, Peoples R China
  • [ 6 ] [Wang, Xiuyun]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Coll Chem Engn, Fuzhou 350002, Fujian, Peoples R China
  • [ 7 ] [Lin, Jianxin]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Coll Chem Engn, Fuzhou 350002, Fujian, Peoples R China
  • [ 8 ] [Au, Chak-Tong]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Coll Chem Engn, Fuzhou 350002, Fujian, Peoples R China
  • [ 9 ] [Lin, Bingyu]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Coll Chem Engn, Fuzhou 350002, Fujian, Peoples R China
  • [ 10 ] [Jiang, Lilong]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Coll Chem Engn, Fuzhou 350002, Fujian, Peoples R China

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Source :

AICHE JOURNAL

ISSN: 0001-1541

Year: 2022

Issue: 11

Volume: 68

3 . 7

JCR@2022

3 . 5 0 0

JCR@2023

ESI Discipline: CHEMISTRY;

ESI HC Threshold:74

JCR Journal Grade:2

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count: 8

SCOPUS Cited Count: 8

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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