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author:

Ke, Bingyuan (Ke, Bingyuan.) [1] | Wang, Xinghui (Wang, Xinghui.) [2] (Scholars:王星辉) | Cheng, Shoulin (Cheng, Shoulin.) [3] | Li, Wangyang (Li, Wangyang.) [4] | Deng, Renming (Deng, Renming.) [5] | Zhang, Congcong (Zhang, Congcong.) [6] | Lin, Jie (Lin, Jie.) [7] | Xie, Qingshui (Xie, Qingshui.) [8] | Peng, Dong-Liang (Peng, Dong-Liang.) [9]

Indexed by:

EI Scopus SCIE CSCD

Abstract:

Areal power density is one of the core indicators determining how large areas a microbattery need to occupy when integrated directly with microelectronic devices for the Internet of Things. Unfortunately, the low power density of microbatteries hinders their applications, because microelectronic devices only provide finite areas for integration. Herein, we show that sputtered iron oxysulfide (FeOxSy) thin films subjected to in situ plasma pretreatment display ultrahigh power density. This in situ plasma pretreatment can be regarded as a universal interface optimization strategy for suppressing mechanical degradation upon extended cycling. The synergistic effects of high structural integrity (robust interfacial adhesiveness and stress-relieving islands), perfect electrochemical reversibility, and near-surface charge exchanges (pseudocapacitive lithium storage mechanism) result in extremely high power density and stable cycling performance. The pretreated FeOxSy thin films can output an areal power density as high as 14.6 mW cm(-2) and a considerable volumetric energy density of 291 mu W h cm(-2) mu m(-1). Such a high-power density constitutes a new state-of-the-art level for sputtered thin-film materials with comparative areal capacity. This work provides an efficient and simple pretreatment method for achieving ultrahigh-power and stable thin-film electrodes for microbatteries.

Keyword:

plasma treatment solid-state batteries sputter sulfides thin-film batteries

Community:

  • [ 1 ] [Ke, Bingyuan]Fuzhou Univ, Coll Phys & Informat Engn, Inst Micronano Devices & Solar Cells, Fuzhou 350108, Peoples R China
  • [ 2 ] [Wang, Xinghui]Fuzhou Univ, Coll Phys & Informat Engn, Inst Micronano Devices & Solar Cells, Fuzhou 350108, Peoples R China
  • [ 3 ] [Cheng, Shoulin]Fuzhou Univ, Coll Phys & Informat Engn, Inst Micronano Devices & Solar Cells, Fuzhou 350108, Peoples R China
  • [ 4 ] [Li, Wangyang]Fuzhou Univ, Coll Phys & Informat Engn, Inst Micronano Devices & Solar Cells, Fuzhou 350108, Peoples R China
  • [ 5 ] [Deng, Renming]Fuzhou Univ, Coll Phys & Informat Engn, Inst Micronano Devices & Solar Cells, Fuzhou 350108, Peoples R China
  • [ 6 ] [Zhang, Congcong]Fuzhou Univ, Coll Phys & Informat Engn, Inst Micronano Devices & Solar Cells, Fuzhou 350108, Peoples R China
  • [ 7 ] [Wang, Xinghui]Fujian Sci & Technol Innovat Lab Optoelect Inform, Fuzhou 350108, Peoples R China
  • [ 8 ] [Wang, Xinghui]Jiangsu Collaborat Innovat Ctr Photovolta Sci & E, Changzhou 213000, Peoples R China
  • [ 9 ] [Lin, Jie]Xiamen Univ, Coll Mat, Collaborat Innovat Ctr Chem Energy Mat, State Key Lab Phys Chem Solid Surfaces,Fujian Key, Xiamen 361005, Peoples R China
  • [ 10 ] [Xie, Qingshui]Xiamen Univ, Coll Mat, Collaborat Innovat Ctr Chem Energy Mat, State Key Lab Phys Chem Solid Surfaces,Fujian Key, Xiamen 361005, Peoples R China
  • [ 11 ] [Peng, Dong-Liang]Xiamen Univ, Coll Mat, Collaborat Innovat Ctr Chem Energy Mat, State Key Lab Phys Chem Solid Surfaces,Fujian Key, Xiamen 361005, Peoples R China

Reprint 's Address:

  • [Wang, Xinghui]Fuzhou Univ, Coll Phys & Informat Engn, Inst Micronano Devices & Solar Cells, Fuzhou 350108, Peoples R China;;[Wang, Xinghui]Fujian Sci & Technol Innovat Lab Optoelect Inform, Fuzhou 350108, Peoples R China;;[Wang, Xinghui]Jiangsu Collaborat Innovat Ctr Photovolta Sci & E, Changzhou 213000, Peoples R China;;[Peng, Dong-Liang]Xiamen Univ, Coll Mat, Collaborat Innovat Ctr Chem Energy Mat, State Key Lab Phys Chem Solid Surfaces,Fujian Key, Xiamen 361005, Peoples R China;;

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Source :

SCIENCE CHINA-MATERIALS

ISSN: 2095-8226

CN: 10-1236/TB

Year: 2022

Issue: 1

Volume: 66

Page: 118-126

8 . 1

JCR@2022

6 . 8 0 0

JCR@2023

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:91

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 37

SCOPUS Cited Count: 32

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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