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Lithium metal battery is strongly deemed as the most promising next-generation energy-storage devices due to its high theoretical energy density. However, uneven lithium deposition and infinite volume change are still the main challenges that significantly hinder their practical applications. Herein, a silicon nanoparticle-decorated carbon nanofibers (Si@CNFs) mat was explored as a novel lithiophilic and conductive interlayer for commer-cial Li foil. The Si@CNFs interlayer with three-dimensional porous and conductive structure can act as a Li+ redistributor and a lithiophilic host to regulate Li deposition behaviors and buffer the volume changes during the Li plating/stripping processes. The obtained Si@CNFs-Li anodes possess outstanding cycling stability under ul-trahigh currents and capacities (e.g. 1800 cycles at 20 mA cm-2/5 mAh cm-2 and 900 cycles at 80 mA cm-2/40 mAh cm-2). This strategy is facile and efficient in inhibiting Li dendrite growth and can be extended to other alkali metal batteries.
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CHEMICAL ENGINEERING JOURNAL
ISSN: 1385-8947
Year: 2023
Volume: 462
1 3 . 4
JCR@2023
1 3 . 4 0 0
JCR@2023
ESI Discipline: ENGINEERING;
ESI HC Threshold:35
JCR Journal Grade:1
CAS Journal Grade:1
Cited Count:
WoS CC Cited Count: 9
SCOPUS Cited Count: 8
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 1
Affiliated Colleges: