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author:

Zhang, Bing (Zhang, Bing.) [1] | Lu, Yinhong (Lu, Yinhong.) [2] | Luo, Xiangbo (Luo, Xiangbo.) [3] | Wang, Wei (Wang, Wei.) [4] | Huang, Jianying (Huang, Jianying.) [5] (Scholars:黄剑莹) | Lai, Yuekun (Lai, Yuekun.) [6] (Scholars:赖跃坤) | Wang, Yuping (Wang, Yuping.) [7] | Zhang, Yi (Zhang, Yi.) [8] | Cai, Weilong (Cai, Weilong.) [9] (Scholars:蔡伟龙)

Indexed by:

EI Scopus SCIE

Abstract:

Removal of dust and NOx from flue gas is highly significant for air pollution control, and integration of these two functions in one unit can greatly improve process efficiency. In this study, a functional catalytic bag-filter material (CBFM) was fabricated from commercial PTFE felt and cheap catalyst V2O5-WO3/TiO2 via a simple immersion-fixation procedure. The attachment of catalysts on PTFE was confirmed, and the material properties of CBFM of various loadings were determined. Their denitration and dedusting performances were investigated individually in lab-scale experiments. Compared to the original PTFE, CBFMs exhibited superior denitration activities, which were positively correlated with temperature (60-90% under 150-210 degrees C) and negatively correlated with filtration velocity (50-90% under 0.5-0.9 m min-1). On the other hand, introduction of catalysts in PTFE felt did not compromise its filtration efficiency, and almost complete dust removal was achieved. A simplified kinetic model was developed based on Eley-Rideal mechanism, to correlate the materials' denitration efficiency with various operational conditions. The model's accuracy was verified in both lab and pilot environments, where real flue gas from a waste incineration plant was treated with a scaled-up CBFM. In a six-day continuous test, the CBFM maintained >70% NO removal and >99.8% dust removal, confirming its stability and applicability in industrial settings. Therefore, this study offers a low-cost and functional bi-functional filter material capable of efficient simultaneous dedusting/denitration, as well as a simple and practical procedure for its manufacture. In addition, the kinetic model could be applied to speed up production and process optimization, and direct future application of similar materials in real environments.

Keyword:

Catalytic bag-filter denitration Kinetic model Pilot-scale PTFE Simultaneous dedusting TiO2

Community:

  • [ 1 ] [Zhang, Bing]Fuzhou Univ, Coll Chem Engn, Fuzhou 350116, Peoples R China
  • [ 2 ] [Lu, Yinhong]Fuzhou Univ, Coll Chem Engn, Fuzhou 350116, Peoples R China
  • [ 3 ] [Wang, Wei]Fuzhou Univ, Coll Chem Engn, Fuzhou 350116, Peoples R China
  • [ 4 ] [Huang, Jianying]Fuzhou Univ, Coll Chem Engn, Fuzhou 350116, Peoples R China
  • [ 5 ] [Lai, Yuekun]Fuzhou Univ, Coll Chem Engn, Fuzhou 350116, Peoples R China
  • [ 6 ] [Cai, Weilong]Fuzhou Univ, Coll Chem Engn, Fuzhou 350116, Peoples R China
  • [ 7 ] [Zhang, Bing]Qingyuan Innovat Lab, Quanzhou 362801, Peoples R China
  • [ 8 ] [Wang, Yuping]Qingyuan Innovat Lab, Quanzhou 362801, Peoples R China
  • [ 9 ] [Cai, Weilong]Qingyuan Innovat Lab, Quanzhou 362801, Peoples R China
  • [ 10 ] [Luo, Xiangbo]Fujian ZEST Environm Protect Technol Co Ltd, Xiamen 361006, Peoples R China
  • [ 11 ] [Zhang, Yi]Fudan Univ, Dept Environm Sci & Engn, Shanghai 200438, Peoples R China
  • [ 12 ] [Cai, Weilong]Fuzhou Univ, Coll Chem Engn, 2 Xue Yuan Rd,Univ Town, Fuzhou 350108, Fujian, Peoples R China
  • [ 13 ] [Zhang, Yi]Fudan Univ, Dept Environm Sci & Engn, 2205 Songhu Rd, Shanghai 200438, Peoples R China

Reprint 's Address:

  • 蔡伟龙

    [Cai, Weilong]Fuzhou Univ, Coll Chem Engn, 2 Xue Yuan Rd,Univ Town, Fuzhou 350108, Fujian, Peoples R China;;[Zhang, Yi]Fudan Univ, Dept Environm Sci & Engn, 2205 Songhu Rd, Shanghai 200438, Peoples R China

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Source :

JOURNAL OF CLEANER PRODUCTION

ISSN: 0959-6526

Year: 2023

Volume: 407

9 . 8

JCR@2023

9 . 8 0 0

JCR@2023

ESI Discipline: ENGINEERING;

ESI HC Threshold:35

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 20

SCOPUS Cited Count: 9

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 3

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