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In this study, we utilized time-domain terahertz magneto-optical spectroscopy to investigate the spin resonance in a c-cut TmFeO3 single crystal at T = 1.6 K under different magnetic fields and characterized its intricate internal interactions. By selectively exciting the magnetic resonance modes in the crystal, we found that as the magnetic field increases, the quasi-ferromagnetic (q-FM) mode of TmFeO3 single crystal shifts towards higher frequencies, while the quasi-antiferromagnetic (q-AFM) mode transforms into the q-FM mode at low critical magnetic fields (2.2–3.6 T). Through magnetic structure analysis and theoretical calculations, it is confirmed that the magnetic moment of TmFeO3 undergoes a magnetic-field-induced spin reorientation from Γ2 to Γ4 phase. Materials with magnetic moment flipping at low magnetic fields may find applications for antiferromagnetic spintronic devices in the future. © 2023 Elsevier B.V.
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Infrared Physics and Technology
ISSN: 1350-4495
Year: 2023
Volume: 135
3 . 1
JCR@2023
3 . 1 0 0
JCR@2023
JCR Journal Grade:2
CAS Journal Grade:3
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ESI Highly Cited Papers on the List: 0 Unfold All
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30 Days PV: 0
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