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author:

Huang, Juan (Huang, Juan.) [1] | Feng, Yanli (Feng, Yanli.) [2] | Li, Jian (Li, Jian.) [3] | Xiong, Bin (Xiong, Bin.) [4] | Feng, Jialiang (Feng, Jialiang.) [5] | Wen, Sheng (Wen, Sheng.) [6] | Sheng, Guoying (Sheng, Guoying.) [7] | Fu, Jiamo (Fu, Jiamo.) [8] | Wu, Minghong (Wu, Minghong.) [9] (Scholars:吴明红)

Indexed by:

SCIE

Abstract:

The levels of carbonyl compounds in Shanghai ambient air were measured in five periods from January 2007 to October 2007 (covering winter, high-air-pollution days, spring, summer and autumn). A total of 114 samples were collected and eighteen carbonyls were identified. Formaldehyde, acetaldehyde and acetone were the most abundant carbonyls and their mean concentrations of 19.40 +/- 12.00, 15.92 +/- 12.07 and 11.86 +/- 7.04 mu g m(-3) respectively, in the daytime for five sampling periods. Formaldehyde and acetaldehyde showed similar diurnal profiles with peak mixing ratios in the morning and early afternoon during the daytime. Their mean concentrations were highest in summer and lowest in winter. Acetone showed reversed seasonal variation. The high molecular weight (HMW, a parts per thousand yenC5) carbonyls also showed obvious diurnal variations with higher concentrations in the daytime in summer and autumn, while they were all not detected in winter. Formaldehyde and acetaldehyde played an important role in removing OH radicals in the atmosphere, but the contribution of acetone was below 1%. The carbonyls levels in high-air-pollution days were reported. More carbonyl species with higher concentrations were found in high-air-pollution days than in spring. These carbonyls were transported with other pollutants from north and northwest in March 27 to April 2, 2007 and then mixed with local sources. Comparing with Beijing and Guangzhou, the concentrations of formaldehyde and acetaldehyde in Shanghai were the highest, which indicated that the air pollution in Shanghai was even worse than expected.

Keyword:

Acetaldehyde Diurnal variation Formaldehyde High-air-pollution days Seasonal variation

Community:

  • [ 1 ] [Huang, Juan]Shanghai Univ, Sch Environm & Chem Engn, Inst Environm Pollut & Hlth, Shanghai 200444, Peoples R China
  • [ 2 ] [Feng, Yanli]Shanghai Univ, Sch Environm & Chem Engn, Inst Environm Pollut & Hlth, Shanghai 200444, Peoples R China
  • [ 3 ] [Li, Jian]Shanghai Univ, Sch Environm & Chem Engn, Inst Environm Pollut & Hlth, Shanghai 200444, Peoples R China
  • [ 4 ] [Xiong, Bin]Shanghai Univ, Sch Environm & Chem Engn, Inst Environm Pollut & Hlth, Shanghai 200444, Peoples R China
  • [ 5 ] [Feng, Jialiang]Shanghai Univ, Sch Environm & Chem Engn, Inst Environm Pollut & Hlth, Shanghai 200444, Peoples R China
  • [ 6 ] [Wen, Sheng]Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangdong Key Lab Environm Protect & Resources Ut, Guangzhou 510640, Guangdong, Peoples R China
  • [ 7 ] [Sheng, Guoying]Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangdong Key Lab Environm Protect & Resources Ut, Guangzhou 510640, Guangdong, Peoples R China
  • [ 8 ] [Fu, Jiamo]Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangdong Key Lab Environm Protect & Resources Ut, Guangzhou 510640, Guangdong, Peoples R China
  • [ 9 ] [Wu, Minghong]Shanghai Univ, Sch Environm & Chem Engn, Shanghai Appl Radiat Inst, Shanghai 200444, Peoples R China

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Source :

JOURNAL OF ATMOSPHERIC CHEMISTRY

ISSN: 0167-7764

Year: 2008

Issue: 1

Volume: 61

Page: 1-20

1 . 4 7 8

JCR@2008

3 . 0 0 0

JCR@2023

JCR Journal Grade:2

Cited Count:

WoS CC Cited Count: 0

SCOPUS Cited Count: 76

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 4

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