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author:

Wang, Yu-jie (Wang, Yu-jie.) [1] | Liao, Ri-quan (Liao, Ri-quan.) [2] | Liu, Wen-long (Liu, Wen-long.) [3] | Kannan, Kurunthachalam (Kannan, Kurunthachalam.) [4] | Ohura, Takeshi (Ohura, Takeshi.) [5] | Wu, Ming-hong (Wu, Ming-hong.) [6] (Scholars:吴明红) | Ma, Jing (Ma, Jing.) [7]

Indexed by:

SCIE

Abstract:

Chlorinated polycyclic aromatic hydrocarbons (ClPAHs) with three to five aromatic rings have been documented to ubiquitously occur in environmental matrices. In this study, residual concentrations and profiles of 20 individual ClPAHs were determined in 35 surface sediment samples from Maowei Sea, a semi-enclosed shallow inland bay located in the northwestern part of South China Sea. The concentrations of I ClPAHs pound in sediment ranged from 313 to 9650 pg/g dw with a detection rate of 43-100%. Of the individual ClPAH congeners, 9-ClPhe was the most abundant in Maowei Sea with the concentrations that ranged from 99.9 to 3610 pg/g dw (mean 1120 pg/g dw). High-molecular-weight ClPAH congeners (four to five rings) were predominant in sediments from sampling locations near a petrochemical industrial complex, whereas low-molecular-weight ClPAH congeners (three rings) were predominant in sediments from estuarine and mangrove locations. A positive matrix factorization (PMF) model in combination with dioxin-like toxic equivalency quotient (TEQ) results was used to apportion sources of ClPAHs. Vehicular emission, combustion/chemical industrial processes, and two other unknown sources accounted for 40.1, 25.5, 20.8, and 13.6%, respectively, of ClPAH sources in sediment; their contribution to TEQs in sediments were 24.2, 40.5, 19.3, and 16.0%, respectively. Further investigations are needed to elucidate potential sources and ecological risks of ClPAHs in sediments.

Keyword:

apportionment ClPAHs PMF Source Surface sediment

Community:

  • [ 1 ] [Wang, Yu-jie]Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China
  • [ 2 ] [Liu, Wen-long]Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China
  • [ 3 ] [Wu, Ming-hong]Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China
  • [ 4 ] [Ma, Jing]Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China
  • [ 5 ] [Wang, Yu-jie]Shanghai Key Lab Atmospher Particle Pollut & Prev, Shanghai 200433, Peoples R China
  • [ 6 ] [Ma, Jing]Shanghai Key Lab Atmospher Particle Pollut & Prev, Shanghai 200433, Peoples R China
  • [ 7 ] [Liao, Ri-quan]Qinzhou Univ, Guangxi Key Lab Beibu Gulf Marine Biodivers Conse, Qinzhou 535000, Guangxi, Peoples R China
  • [ 8 ] [Kannan, Kurunthachalam]SUNY Albany, New York State Dept Hlth, Wadsworth Ctr, Albany, NY 12201 USA
  • [ 9 ] [Kannan, Kurunthachalam]SUNY Albany, Sch Publ Hlth, Dept Environm Hlth Sci, Albany, NY 12201 USA
  • [ 10 ] [Ohura, Takeshi]Meijo Univ, Fac Agr, 1-501 Tempaku, Nagoya, Aichi 4688502, Japan

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Source :

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH

ISSN: 0944-1344

Year: 2017

Issue: 19

Volume: 24

Page: 16241-16252

2 . 8

JCR@2017

0 . 0 0 0

JCR@2023

JCR Journal Grade:2

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count: 20

SCOPUS Cited Count: 21

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 3

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