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author:

Zhang, Y. (Zhang, Y..) [1] | Zheng, X. (Zheng, X..) [2] | Chen, S. (Chen, S..) [3] | Qiu, Y. (Qiu, Y..) [4] | Luo, F. (Luo, F..) [5] | Weng, Z. (Weng, Z..) [6] | Qiu, B. (Qiu, B..) [7] | Shou, J. (Shou, J..) [8] | Lin, Z. (Lin, Z..) [9]

Indexed by:

Scopus

Abstract:

Lead halide perovskites have garnered significant attention in the field of photoelectrochemistry due to their outstanding optical properties. Nevertheless, the pronounced susceptibility of perovskite to water poses a major limitation to its practical applications. A signal-on photoelectrochemical (PEC) sensor was constructed in this work using water-resistant perovskite nanocrystals for the detection of hydrogen sulfide. Specially, the electrode surface was modified with composite nanomaterials (CsPbBr3 @PEG-PCL). In the presence of H2S, efficient heterojunctions were formed through the in-situ generation of PbS on CsPbBr3 @PEG-PCL, thereby enhancing the photocurrent signal. The potential mechanism behind this signal enhancement was extensively discussed. The designed sensor exhibited a linear relationship with the concentration of H2S ranging from 0.02 to 120 μM, with a detection limit of 6.67 nM. This work opens up new possibilities for utilizing halide perovskites in the field of sensing, with promising applications in areas such as food safety, environmental monitoring, and biomedical analysis. © 2023 Elsevier B.V.

Keyword:

H2S Heterojunction Perovskite Photoectrochemical sensor

Community:

  • [ 1 ] [Zhang Y.]College of Biological Science and Engineering, Fuzhou University, Fujian, Fuzhou, 350116, China
  • [ 2 ] [Zhang Y.]MOE Key Laboratory of Analysis and Detection for Food Safety and Biology, Fujian Provincial Key Laboratory of Analysis and Detection Technology for Food Safety, College of Chemistry, Fuzhou University, Fujian, Fuzhou, 350116, China
  • [ 3 ] [Zheng X.]Xiaoshan Hospital Affiliated to Hangzhou Normal University, Zhejiang, Hangzhou, 311200, China
  • [ 4 ] [Chen S.]Xiaoshan Hospital Affiliated to Hangzhou Normal University, Zhejiang, Hangzhou, 311200, China
  • [ 5 ] [Qiu Y.]College of Biological Science and Engineering, Fuzhou University, Fujian, Fuzhou, 350116, China
  • [ 6 ] [Qiu Y.]MOE Key Laboratory of Analysis and Detection for Food Safety and Biology, Fujian Provincial Key Laboratory of Analysis and Detection Technology for Food Safety, College of Chemistry, Fuzhou University, Fujian, Fuzhou, 350116, China
  • [ 7 ] [Luo F.]College of Biological Science and Engineering, Fuzhou University, Fujian, Fuzhou, 350116, China
  • [ 8 ] [Luo F.]MOE Key Laboratory of Analysis and Detection for Food Safety and Biology, Fujian Provincial Key Laboratory of Analysis and Detection Technology for Food Safety, College of Chemistry, Fuzhou University, Fujian, Fuzhou, 350116, China
  • [ 9 ] [Weng Z.]College of Biological Science and Engineering, Fuzhou University, Fujian, Fuzhou, 350116, China
  • [ 10 ] [Qiu B.]MOE Key Laboratory of Analysis and Detection for Food Safety and Biology, Fujian Provincial Key Laboratory of Analysis and Detection Technology for Food Safety, College of Chemistry, Fuzhou University, Fujian, Fuzhou, 350116, China
  • [ 11 ] [Shou J.]Xiaoshan Hospital Affiliated to Hangzhou Normal University, Zhejiang, Hangzhou, 311200, China
  • [ 12 ] [Lin Z.]MOE Key Laboratory of Analysis and Detection for Food Safety and Biology, Fujian Provincial Key Laboratory of Analysis and Detection Technology for Food Safety, College of Chemistry, Fuzhou University, Fujian, Fuzhou, 350116, China

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Source :

Sensors and Actuators B: Chemical

ISSN: 0925-4005

Year: 2024

Volume: 403

6 . 3 9 3

JCR@2018

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 3

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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