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author:

Xie, Jiaxing (Xie, Jiaxing.) [1] | Liu, Qun (Liu, Qun.) [2] | Huang, Lijuan (Huang, Lijuan.) [3] | Chen, Xingyu (Chen, Xingyu.) [4] | Zhao, Chunlin (Zhao, Chunlin.) [5] (Scholars:赵纯林) | Wu, Xiao (Wu, Xiao.) [6] (Scholars:吴啸) | Lin, Tengfei (Lin, Tengfei.) [7] (Scholars:林腾飞) | Wu, Yong (Wu, Yong.) [8] | Gao, Min (Gao, Min.) [9] (Scholars:高旻) | Lin, Cong (Lin, Cong.) [10] (Scholars:林枞)

Indexed by:

EI Scopus SCIE

Abstract:

The Fenton reaction, an effective advanced oxidation process (AOP) for degrading organic pollutants, requires the addition of H 2 O 2 that is expensive and not environmentally friendly to some extent. It has been reported that piezocatalysis can generate H 2 O 2 under mechanical excitation. Therefore, it is promising to carry out the Fenton catalysis utilizing in situ H 2 O 2 generated by piezocatalysis. However, the current piezocatalysis-assisted Fenton (Piezo-Fenton) reaction was realized by adding piezoelectric nanoparticles and Fe(II) ions to pollutant solutions, which would induce more iron-based chemicals that are not easy to recycle. Herein, Fe 3 O 4 -BaTiO 3 nanocomposites were prepared to demonstrate the feasibility of piezo-Fenton catalysis without the addition of H 2 O 2 or Fe(II) ions. The organic dye degradation efficiency of 98.2% is obtained using Fe 3 O 4 -BaTiO 3 nanocomposites in the acidic solution, one-third and two-thrid greater than that of pure piezocatalysis and that of iron-based Fenton reaction, respectively. Moreover, since the piezocatalysis process is the rate-determining step of the whole piezo-Fenton reaction, all the H 2 O 2 generated can be consumed. Considering that the solid nanocomposites can be magnetically recycled, piezo-Fenton catalysis leaves no additional chemicals in clean water and thus provides an environmentally friendly and low-cost approach for organic dye degradation.

Keyword:

Magnet Piezo-Fenton synergistic catalysis Recyclability

Community:

  • [ 1 ] [Xie, Jiaxing]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China
  • [ 2 ] [Liu, Qun]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China
  • [ 3 ] [Huang, Lijuan]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China
  • [ 4 ] [Chen, Xingyu]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China
  • [ 5 ] [Zhao, Chunlin]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China
  • [ 6 ] [Wu, Xiao]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China
  • [ 7 ] [Lin, Tengfei]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China
  • [ 8 ] [Gao, Min]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China
  • [ 9 ] [Lin, Cong]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China
  • [ 10 ] [Wu, Yong]Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China

Reprint 's Address:

  • 高旻 林枞

    [Gao, Min]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China;;[Lin, Cong]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China

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Source :

CHEMICAL ENGINEERING JOURNAL

ISSN: 1385-8947

Year: 2024

Volume: 487

1 3 . 4 0 0

JCR@2023

Cited Count:

WoS CC Cited Count: 12

SCOPUS Cited Count: 14

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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