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author:

Xie, Jiaxing (Xie, Jiaxing.) [1] | Liu, Qun (Liu, Qun.) [2] | Huang, Lijuan (Huang, Lijuan.) [3] | Chen, Xingyu (Chen, Xingyu.) [4] | Zhao, Chunlin (Zhao, Chunlin.) [5] | Wu, Xiao (Wu, Xiao.) [6] | Lin, Tengfei (Lin, Tengfei.) [7] | Wu, Yong (Wu, Yong.) [8] | Gao, Min (Gao, Min.) [9] | Lin, Cong (Lin, Cong.) [10]

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EI

Abstract:

The Fenton reaction, an effective advanced oxidation process (AOP) for degrading organic pollutants, requires the addition of H2O2 that is expensive and not environmentally friendly to some extent. It has been reported that piezocatalysis can generate H2O2 under mechanical excitation. Therefore, it is promising to carry out the Fenton catalysis utilizing in situ H2O2 generated by piezocatalysis. However, the current piezocatalysis-assisted Fenton (Piezo-Fenton) reaction was realized by adding piezoelectric nanoparticles and Fe(II) ions to pollutant solutions, which would induce more iron-based chemicals that are not easy to recycle. Herein, Fe3O4-BaTiO3 nanocomposites were prepared to demonstrate the feasibility of piezo-Fenton catalysis without the addition of H2O2 or Fe(II) ions. The organic dye degradation efficiency of 98.2% is obtained using Fe3O4-BaTiO3 nanocomposites in the acidic solution, one-third and two-thrid greater than that of pure piezocatalysis and that of iron-based Fenton reaction, respectively. Moreover, since the piezocatalysis process is the rate-determining step of the whole piezo-Fenton reaction, all the H2O2 generated can be consumed. Considering that the solid nanocomposites can be magnetically recycled, piezo-Fenton catalysis leaves no additional chemicals in clean water and thus provides an environmentally friendly and low-cost approach for organic dye degradation. © 2024 Elsevier B.V.

Keyword:

Additives Barium titanate Catalysis Costs Degradation Energy efficiency Ions Magnetite Nanocomposites Organic chemicals Organic pollutants Oxidation Recycling Water treatment

Community:

  • [ 1 ] [Xie, Jiaxing]College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350108, China
  • [ 2 ] [Liu, Qun]College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350108, China
  • [ 3 ] [Huang, Lijuan]College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350108, China
  • [ 4 ] [Chen, Xingyu]College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350108, China
  • [ 5 ] [Zhao, Chunlin]College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350108, China
  • [ 6 ] [Wu, Xiao]College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350108, China
  • [ 7 ] [Lin, Tengfei]College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350108, China
  • [ 8 ] [Wu, Yong]School of Materials Science and Engineering, University of Science and Technology Beijing, Beijing; 100083, China
  • [ 9 ] [Gao, Min]College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350108, China
  • [ 10 ] [Lin, Cong]College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350108, China

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Source :

Chemical Engineering Journal

ISSN: 1385-8947

Year: 2024

Volume: 487

1 3 . 4 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 2

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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