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author:

Wu, S. (Wu, S..) [1] | Cheng, Y. (Cheng, Y..) [2] | Zheng, W. (Zheng, W..) [3] | Deng, Y. (Deng, Y..) [4] | Zhu, T. (Zhu, T..) [5] | Zhang, W. (Zhang, W..) [6] | Li, H. (Li, H..) [7] | Huang, J. (Huang, J..) [8] | Lai, Y. (Lai, Y..) [9]

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Scopus

Abstract:

Highly transparent, durable, and flexible liquid-repellent coatings are urgently needed in the realm of transparent materials, such as car windows, optical lenses, solar panels, and flexible screen materials. However, it has been difficult to strike a balance between the robustness and flexibility of coatings constructed by a single cross-linked network design. To overcome the conundrum, this innovative approach effectively combines two distinct cross-linked networks with unique functions, thus overcoming the challenge. Through a tightly interwoven structure comprised of added crosslinking sites, the coating achieves improved liquid repellency (WCA>100°, OSA<10°), increased durability (withstands 2,000 cycles of cotton wear), enhanced flexibility (endures 5,000 cycles of bending with a bending radius of 1 mm), and maintains high transparency (over 98 % in the range of 410 nm to 760 nm). Additionally, the coating with remarkable adhesion can be applied to multiple substrates, enabling large-scale preparation and easy cycling coating, thus expanding its potential applications. The architecture of this fluoride-free dual cross-linked network not only advances liquid-repellent surfaces but also provides valuable insights for the development of eco-friendly materials in the future. © 2024

Keyword:

Dual cross-linked network Flexible liquid-like coating Fluoride-free Highly transparent Tight entanglement

Community:

  • [ 1 ] [Wu S.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 2 ] [Cheng Y.]Zhejiang Engineering Research Center for Tissue Repair Materials, Wenzhou Institute, University of Chinese Academy of Science, Wenzhou, 325000, China
  • [ 3 ] [Zheng W.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 4 ] [Zheng W.]University of Strasbourg & CNRS, UMR7140, Strasbourg, 67000, France
  • [ 5 ] [Deng Y.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 6 ] [Zhu T.]School of Materials and Chemistry, Anhui Agricultural University, Hefei, 230036, China
  • [ 7 ] [Zhang W.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 8 ] [Li H.]Zhejiang Engineering Research Center for Tissue Repair Materials, Wenzhou Institute, University of Chinese Academy of Science, Wenzhou, 325000, China
  • [ 9 ] [Huang J.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 10 ] [Lai Y.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China

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Source :

Journal of Materials Science and Technology

ISSN: 1005-0302

CN: 21-1315/TG

Year: 2025

Volume: 206

Page: 53-61

1 1 . 2 0 0

JCR@2023

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

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Chinese Cited Count:

30 Days PV: 2

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