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author:

Cao, Xingfeng (Cao, Xingfeng.) [1] | Fan, Gongduan (Fan, Gongduan.) [2] (Scholars:范功端) | Luo, Jing (Luo, Jing.) [3] | Zhang, Ling (Zhang, Ling.) [4] | Wu, Shiyun (Wu, Shiyun.) [5] | Yao, Yixin (Yao, Yixin.) [6] | Xu, Kai-Qin (Xu, Kai-Qin.) [7]

Indexed by:

EI Scopus SCIE

Abstract:

Algal blooms have become a widespread concern for drinking water production, threatening ecosystems and human health. Photocatalysis, a promising advanced oxidation process (AOP) technology for wastewater treatment, is considered a potential measure for in situ remediation of algal blooms. However, conventional photocatalysts often suffer from limited visible-light response and rapid recombination of photogenerated electron-hole pairs. In this study, we prepared a Z-scheme AgBr/NH2-MIL-125(Ti) 2-MIL-125(Ti) composite with excellent visible light absorption performance using co-precipitation to efficiently inactivate Microcystis aeruginosa. . The degradation efficiency of AgBr/NH2-MIL-125(Ti) 2-MIL-125(Ti) for chlorophyll a was 98.7 % after 180 min of visible light irradiation, significantly surpassing the degradation rate efficiency of AgBr and NH2-MIL-125(Ti) 2-MIL-125(Ti) by factors of 3.20 and 36.75, respectively. Moreover, the removal rate was maintained at 91.1 % even after five times of repeated use. The experimental results indicated that superoxide radicals (center dot O2- center dot O 2- ) were the dominant reactive oxygen species involved. The photocatalytic reaction altered the morphology and surface charge of algal cells, inhibited their metabolism, and disrupted their photosynthetic and antioxidant systems. In conclusion, this study presents a promising material for the application of photocatalytic technology in algal bloom remediation.

Keyword:

AgBr Mechanism Microcystis aeruginosa NH2-MIL-125(Ti) Z-scheme

Community:

  • [ 1 ] [Cao, Xingfeng]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China
  • [ 2 ] [Fan, Gongduan]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China
  • [ 3 ] [Zhang, Ling]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China
  • [ 4 ] [Wu, Shiyun]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China
  • [ 5 ] [Yao, Yixin]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China
  • [ 6 ] [Xu, Kai-Qin]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China
  • [ 7 ] [Fan, Gongduan]Fuzhou Univ, Fujian Prov Key Lab Electrochem Energy Storage Mat, Fuzhou 350002, Fujian, Peoples R China
  • [ 8 ] [Luo, Jing]Fujian Jinhuang Environm Sci Tech Co Ltd, Fuzhou 350002, Fujian, Peoples R China
  • [ 9 ] [Xu, Kai-Qin]Fuzhou Univ, Coll Environm & Safety Engn, Fuzhou 350116, Fujian, Peoples R China

Reprint 's Address:

  • [Fan, Gongduan]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China;;[Xu, Kai-Qin]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China;;

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Source :

JOURNAL OF HAZARDOUS MATERIALS

ISSN: 0304-3894

Year: 2024

Volume: 478

1 2 . 2 0 0

JCR@2023

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 7

SCOPUS Cited Count: 7

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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