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author:

Zheng, Hui (Zheng, Hui.) [1] | Ma, Dakai (Ma, Dakai.) [2] | Pei, Maojun (Pei, Maojun.) [3] | Lin, Chenkai (Lin, Chenkai.) [4] | Liu, Yao (Liu, Yao.) [5] (Scholars:刘尧) | Deng, Shuqi (Deng, Shuqi.) [6] | Qiu, Ruoxue (Qiu, Ruoxue.) [7] | Luo, Yiyuan (Luo, Yiyuan.) [8] | Yan, Wei (Yan, Wei.) [9] (Scholars:颜蔚) | Zhang, Jiujun (Zhang, Jiujun.) [10] (Scholars:张久俊)

Indexed by:

EI Scopus SCIE

Abstract:

Transition metal sulfides as anode materials for sodium-ion batteries (SIBs) have the advantage of high capacity. However, their cycle-life and rate performance at ultra-high current density is still a thorny issue that limit the applicability of these materials. In this paper, the carbon-embedded heterojunction with sulfur-vacancies regulated by ultrafine bimetallic sulfides (vacancy-CoS2/FeS2@C) with robust interfacial C-S-Co/Fe chemical bonds is successfully synthesized and explored as an anode material for sodium-ion battery. By changing the ratio of two metal cations, the concentration of anion sulfur vacancies can be in-situ adjusted without additional post-treatment. The as-prepared vacancy-CoS2/FeS2@C anode material offers ultrahigh rate performance (285.1 mAh g-1 at 200 A g-1), and excellent long-cycle stability (389.2 mAh g-1 at 40 A g-1 after 10000 cycles), outperforming all reported transition metal sulfides-based anode materials for SIBs. Both in-situ and ex-situ characterizations provide strong evidence for the evolution mechanism of the phases and stable solid-electrolyte interface (SEI) on the vacancy-CoS2/FeS2@C surface. The density functional theory calculations show that constructing heterojunction with reasonable concentration of vacancies can significantly increase the anode electronic conductivity. Notably, the assembled vacancy-CoS2/FeS2@C//Na3V2(PO4)3/C full-cell shows a capacity of 226.2 mAh g-1 after 400 cycles at 2.0 A g-1, confirming this material's practicability. The carbon-embedded heterojunction with sulfur-vacancies regulated by ultrafine bimetallic sulfides (vacancy-CoS2/FeS2@C) is successfully synthesized and explored as an anode material for sodium-ion battery. The mechanism of vacancy-CoS2/FeS2@C for sodium storage is confirmed by in/ex-situ measurements and DFT calculations. This research has taken an important step toward the development of high-performance energy storage electrode materials. image

Keyword:

anode materials heterojunction sodium-ion batteries sulfur vacancies transition metal sulfides

Community:

  • [ 1 ] [Zheng, Hui]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 2 ] [Ma, Dakai]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 3 ] [Pei, Maojun]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 4 ] [Lin, Chenkai]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 5 ] [Liu, Yao]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 6 ] [Deng, Shuqi]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 7 ] [Qiu, Ruoxue]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 8 ] [Luo, Yiyuan]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 9 ] [Yan, Wei]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 10 ] [Zhang, Jiujun]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China

Reprint 's Address:

  • [Yan, Wei]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China;;[Zhang, Jiujun]Fuzhou Univ, Inst New Energy Mat & Engn, Sch Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China;;

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Source :

ADVANCED FUNCTIONAL MATERIALS

ISSN: 1616-301X

Year: 2024

Issue: 1

Volume: 35

1 8 . 5 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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