• Complex
  • Title
  • Keyword
  • Abstract
  • Scholars
  • Journal
  • ISSN
  • Conference
成果搜索

author:

Wu, Jionghua (Wu, Jionghua.) [1] (Scholars:吴炯桦) | Wang, Renjie (Wang, Renjie.) [2] | Zhang, Rui (Zhang, Rui.) [3] | Portale, Giuseppe (Portale, Giuseppe.) [4] | Solano, Eduardo (Solano, Eduardo.) [5] | Liu, Xiaoke (Liu, Xiaoke.) [6] | Gao, Feng (Gao, Feng.) [7]

Indexed by:

EI Scopus SCIE

Abstract:

We report a simple, effective, and universal lattice reconstruction approach to improve the quality of perovskite films by using nonpolar solvents with high Gutmann donor numbers (DNs). We find that high-DN nonpolar solvents, for instance, ethyl acetate, can interact with perovskite precursors. Such a solvent can make the perovskite lattice more ordered and "harder" and promote the formation of heterostructures with low-dimensional perovskite impurities and residual solvent molecules. As a result, the lattice-reconstructed perovskite films exhibit reduced defect densities and suppressed ion migration. The resultant mixed-halide blue perovskite light-emitting diodes (PeLEDs) show greatly enhanced tolerance to high driving current densities and voltages, demonstrating high brightness, outstanding color stability and low efficiency roll-off. Our work provides a deep understanding of the interactions between nonpolar solvents and perovskites and offers useful guidelines for further development of high-power PeLEDs.

Keyword:

color stability high brightness ion migration low efficiency roll-off mixed halide perovskite

Community:

  • [ 1 ] [Wu, Jionghua]Linkoping Univ, Dept Phys Chem & Biol IFM, S-58183 Linkoping, Sweden
  • [ 2 ] [Zhang, Rui]Linkoping Univ, Dept Phys Chem & Biol IFM, S-58183 Linkoping, Sweden
  • [ 3 ] [Liu, Xiaoke]Linkoping Univ, Dept Phys Chem & Biol IFM, S-58183 Linkoping, Sweden
  • [ 4 ] [Gao, Feng]Linkoping Univ, Dept Phys Chem & Biol IFM, S-58183 Linkoping, Sweden
  • [ 5 ] [Wu, Jionghua]Fuzhou Univ, Inst Micronano Devices & Solar Cells, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China
  • [ 6 ] [Wang, Renjie]Fuzhou Univ, Inst Micronano Devices & Solar Cells, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China
  • [ 7 ] [Portale, Giuseppe]Univ Groningen, Zernike Inst Adv Mat, Nijenborgh 4, NL-9747 AG Groningen, Netherlands
  • [ 8 ] [Solano, Eduardo]ALBA Synchrotron, Expt Div, Carrer Llum 2-2608290, Barcelona, Spain

Reprint 's Address:

  • [Liu, Xiaoke]Linkoping Univ, Dept Phys Chem & Biol IFM, S-58183 Linkoping, Sweden;;[Gao, Feng]Linkoping Univ, Dept Phys Chem & Biol IFM, S-58183 Linkoping, Sweden;;

Show more details

Related Keywords:

Source :

SCIENCE CHINA-MATERIALS

ISSN: 2095-8226

Year: 2024

Issue: 11

Volume: 67

Page: 3553-3560

6 . 8 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

Online/Total:308/10000064
Address:FZU Library(No.2 Xuyuan Road, Fuzhou, Fujian, PRC Post Code:350116) Contact Us:0591-22865326
Copyright:FZU Library Technical Support:Beijing Aegean Software Co., Ltd. 闽ICP备05005463号-1