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author:

Chang, Haiqing (Chang, Haiqing.) [1] | Zhu, Yingyuan (Zhu, Yingyuan.) [2] | Liu, Naiming (Liu, Naiming.) [3] | Ji, Pengwei (Ji, Pengwei.) [4] | Yan, Zhongsen (Yan, Zhongsen.) [5] (Scholars:鄢忠森) | Cheng, Xiaoxiang (Cheng, Xiaoxiang.) [6] | Qu, Dan (Qu, Dan.) [7] | Liang, Heng (Liang, Heng.) [8] | Qu, Fangshu (Qu, Fangshu.) [9]

Indexed by:

EI Scopus SCIE

Abstract:

Low pressure membrane takes a great role in hydraulic fracturing wastewater (HFW), while membrane fouling is a critical issue for the stable operation of microfiltration (MF). This study focused on fouling mitigation by sodium percarbonate (SPC) oxidation, activated by ultraviolet (UV) and ferrous ion (Fe(II)). The higher the concentration of oxidizer, the better the anti-fouling performance of MF membrane. Unlike severe MF fouling without oxidation (17.26 L/(m(2)h)), UV/SPC and Fe(II)/SPC under optimized dosage improved the final flux to 740 and 1553 L/(m(2)h), respectively, and the latter generated Fe(III) which acted as a coagulant. Fe(II)/SPC oxidation enabled a shift in fouling mechanism from complete blocking to cake filtration, while UV/SPC oxidation changed it to standard blockage. UV/SPC oxidation was stronger than Fe(II)/SPC oxidation in removing UV254 and fluorescent organics for higher oxidizing capacity, but the opposite was noted for DOC removal. The deposited foulants on membrane surface after oxidation decreased by at least 88% compared to untreated HFW. Correlation analysis showed that UV254, DOC and organic fraction were key parameters responsible for membrane fouling (correlation coefficient > 0.80), oxidizing capacity and turbidity after oxidation were also important parameters. These results provide new insights for fouling control during the HFW treatment.

Keyword:

Ferrous ion (Fe(II)) Hydraulic fracturing wastewater Microfiltration fouling Sodium percarbonate (SPC) Ultraviolet (UV)

Community:

  • [ 1 ] [Chang, Haiqing]Sichuan Univ, Coll Architecture & Environm, MOE Key Lab Deep Earth Sci & Engn, Chengdu 610207, Peoples R China
  • [ 2 ] [Zhu, Yingyuan]Sichuan Univ, Coll Architecture & Environm, MOE Key Lab Deep Earth Sci & Engn, Chengdu 610207, Peoples R China
  • [ 3 ] [Liu, Naiming]Sichuan Univ, Coll Architecture & Environm, MOE Key Lab Deep Earth Sci & Engn, Chengdu 610207, Peoples R China
  • [ 4 ] [Ji, Pengwei]Sichuan Univ, Coll Architecture & Environm, MOE Key Lab Deep Earth Sci & Engn, Chengdu 610207, Peoples R China
  • [ 5 ] [Chang, Haiqing]Sichuan Univ, State Key Lab Intelligent Construct & Hlth Operat, Chengdu 610065, Peoples R China
  • [ 6 ] [Zhu, Yingyuan]Sichuan Univ, State Key Lab Intelligent Construct & Hlth Operat, Chengdu 610065, Peoples R China
  • [ 7 ] [Liu, Naiming]Sichuan Univ, State Key Lab Intelligent Construct & Hlth Operat, Chengdu 610065, Peoples R China
  • [ 8 ] [Ji, Pengwei]Sichuan Univ, State Key Lab Intelligent Construct & Hlth Operat, Chengdu 610065, Peoples R China
  • [ 9 ] [Yan, Zhongsen]Fuzhou Univ, Coll Civil Engn, Fujian 350108, Peoples R China
  • [ 10 ] [Cheng, Xiaoxiang]Shandong Jianzhu Univ, Sch Municipal & Environm Engn, Jinan 250101, Peoples R China
  • [ 11 ] [Qu, Dan]Beijing Forestry Univ, Coll Environm Sci & Engn, Beijing Key Lab Source Control Technol Water Pollu, 35 Qinghua East Rd, Beijing 100083, Peoples R China
  • [ 12 ] [Liang, Heng]Harbin Inst Technol, Sch Environm, State Key Lab Urban Water Resource & Environm, Harbin 150090, Peoples R China
  • [ 13 ] [Qu, Fangshu]Guangzhou Univ, Key Lab Water Qual & Conservat Pearl River Delta, Guangzhou 510006, Peoples R China

Reprint 's Address:

  • [Cheng, Xiaoxiang]Shandong Jianzhu Univ, Sch Municipal & Environm Engn, Jinan 250101, Peoples R China;;[Qu, Fangshu]Guangzhou Univ, Key Lab Water Qual & Conservat Pearl River Delta, Guangzhou 510006, Peoples R China;;

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Source :

ENVIRONMENTAL RESEARCH

ISSN: 0013-9351

Year: 2024

Volume: 262

7 . 7 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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