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author:

Wang, Chenxi (Wang, Chenxi.) [1] | Guo, Lin (Guo, Lin.) [2] | Hu, Junjie (Hu, Junjie.) [3] | Li, Titao (Li, Titao.) [4] | Zhuo, Fangping (Zhuo, Fangping.) [5] | Wu, Hong-Hui (Wu, Hong-Hui.) [6] | Lu, Xiaoqiang (Lu, Xiaoqiang.) [7] | Zhu, Minmin (Zhu, Minmin.) [8]

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Abstract:

The growing interest in ferroelectric materials has witnessed the thriving prospect of bio-inspired artificial neuromorphic system, where multi-level polarization states play a crucial role. In this work, with typical BaTiO3 ferroelectric thin film as the model system, we explore the physical effects of inhomogeneity on polarization switching dynamics and neuromorphic performance. Inhomogeneous films exhibited pinched polarization-electric field hysteresis loops, leading to a high recognition accuracy of 96.03% for hand-written digits, compared to about 10.31% for homogeneous films. The inhomogeneity in switching dynamics was analyzed by inhomogeneous field mechanism. Diffusive distributions of switching time and local electric fields were observed, aligning with experimental results and the expected inhomogeneity. The prolonged domain wall depinning time and lowered energy consumption suggest the potential for multi-level polarization states, a possibility further confirmed by phase-field simulations that demonstrated their presence during long-term potentiation/depression. Our work highlights the positive influence of inhomogeneity in enhancing the performance of ferroelectric-based neuromorphic systems. © 2024 Author(s).

Keyword:

Barium titanate Electric fields Ferroelectricity Ferroelectric thin films Hysteresis loops Polarization

Community:

  • [ 1 ] [Wang, Chenxi]College of Physics and Information Engineering, Fuzhou University, No. 2 Wulongjiang Avenue, Minhou County, Fujian Province, Fuzhou, Fuzhou City; 350116, China
  • [ 2 ] [Wang, Chenxi]School of Advanced Materials Science and Engineering, Sungkyunkwan University (SKKU), Seoul, Korea, Republic of
  • [ 3 ] [Guo, Lin]Institute of Ion Beam Physics and Materials Research, Helmholtz-Zentrum Dresden-Rossendorf e.V. (HZDR), Bautzner Landstrasse 400, Dresden; 01328, Germany
  • [ 4 ] [Hu, Junjie]Bioengineering Department and Imperial-X, Imperial College London, London; W12 7SL, United Kingdom
  • [ 5 ] [Li, Titao]College of Physics and Information Engineering, Fuzhou University, No. 2 Wulongjiang Avenue, Minhou County, Fujian Province, Fuzhou, Fuzhou City; 350116, China
  • [ 6 ] [Zhuo, Fangping]Department of Materials and Earth Sciences, Technical University of Darmstadt, Darmstadt; 64287, Germany
  • [ 7 ] [Wu, Hong-Hui]Beijing Advanced Innovation Center for Materials Genome Engineering, Institute for Carbon Neutrality, University of Science and Technology Beijing, Beijing; 100083, China
  • [ 8 ] [Lu, Xiaoqiang]College of Physics and Information Engineering, Fuzhou University, No. 2 Wulongjiang Avenue, Minhou County, Fujian Province, Fuzhou, Fuzhou City; 350116, China
  • [ 9 ] [Zhu, Minmin]College of Physics and Information Engineering, Fuzhou University, No. 2 Wulongjiang Avenue, Minhou County, Fujian Province, Fuzhou, Fuzhou City; 350116, China

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Source :

Applied Physics Letters

ISSN: 0003-6951

Year: 2024

Issue: 19

Volume: 125

3 . 5 0 0

JCR@2023

CAS Journal Grade:3

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ESI Highly Cited Papers on the List: 0 Unfold All

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Chinese Cited Count:

30 Days PV: 0

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