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Abstract:
Rare earth-doped upconversion nanomaterials have wide application prospects in photothermal sensing,biomedicine and so on,but it has poor thermal conductivity,low temperature measurement sensitivity and upconver⁃ sion luminescence(UCL)intensity. It’s an effective way to improve their UCL intensity and photothermal perfor⁃ mance by assembling composite films which contain single-walled carbon nanotubes(SWCNT),noble metal and pho⁃ tonic crystals(PCs). In this work,NaGdF4∶Er3+/Yb3+/Al3+ nanocrystalls(UCNPs)were synthesized by the solvother⁃ mal method. The photothermal performance of upconversion layer(UC),SWCNT/UC,Ag/SWCNT/UC and PCs/Ag/ SWCNT/UC were compared,and the effects of different film layers on the photothermal performance of UCNPs were studied. The results indicate that PCs/Ag/SWCNT/UC has the best performance,and compared with the UC film,the enhancement factors of red and green emission intensities are 3. 48 and 4. 24 times,respectively. Its photothermal conversion efficiency is 33. 79%,which is 1. 49 times of UC’s. The absolute sensitivity(SA)of the optical tempera⁃ ture measurement is obtained as 3. 14×10−3 K−1 at 353 K and the relative sensitivity(SR)is obtained as 1. 87×10−2 K−1 at 273 K. The work provides an effective way to improve the performance of the photothermal sensor. © 2025 Editorial Office of Chinese Optics. All rights reserved.
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Chinese Journal of Luminescence
ISSN: 1000-7032
Year: 2025
Issue: 1
Volume: 46
Page: 89-97
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ESI Highly Cited Papers on the List: 0 Unfold All
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30 Days PV: 6
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