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author：

Zhu, Y. (Zhu, Y..) [1] | Gao, S. (Gao, S..) [2] | Zhang, S. (Zhang, S..) [3] | Chen, Y. (Chen, Y..) [4] | Liu, P. (Liu, P..) [5] | Meng, H. (Meng, H..) [6] | Luo, Z. (Luo, Z..) [7] | Chen, X. (Chen, X..) [8] | Wen, Z. (Wen, Z..) [9] | Wang, L. (Wang, L..) [10] | Luo, B. (Luo, B..) [12] | Zhou, J. (Zhou, J..) [13]

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Scopus SCIE

Abstract：

Incompatible　electrode/electrolyte　interface　often　leads　to　dendrite　growth,　parasitic　reactions,　and　corrosion,　posing　significant　challenges　to　the　application　of　Zn　anodes.　Herein,　we　introduce　a　biomimetic　antifreeze　protein　localized　gel　electrolyte　(ALGE)　with　multifunctional　capabilities　to　address　these　issues　by　combining　electrolyte　modification　with　interface　optimization.　ALGE　modifies　the　Zn2+　solvation　structure　and　the　hydrogen-bond　network　adjacent　to　the　zinc　anode,　effectively　suppressing　hydrogen　evolution.　Additionally,　ALGE　promotes　(002)Zn　crystal　plane-dominated　deposition　by　protein-zinc　surface　interactions,　enabling　a　long-range　dendrite-free　deposition.　The　absence　of　by-products　and　inhibited　corrosion　further　highlights　the　practical　potential　of　ALGE.　Symmetric　cells　with　ALGE-modified　zinc　demonstrate　an　impressive　lifespan　of　610　h　under　a　current　density　of　10 mA cm−2　and　a　capacity　of　10 mAh cm−2.　The　pouch　cell　integrating　a　manganese　dioxide　cathode　and　ALGE-modified　Zn　anode　retains　75.8%　of　its　capacity　after　200　cycles　at　1 A g−1.　This　localized　gel　electrolyte　strategy　offers　a　practical　and　scalable　approach　to　stabilizing　Zn　anodes　for　next-generation　energy　storage　systems.　©　2025　The　Author(s).　Angewandte　Chemie　International　Edition　published　by　Wiley-VCH　GmbH.

Keyword：

Hydrogen bond network Interfacial gelation Localized gel electrolyte Solvation structure Zinc anode

Community：

  • [ 1 ] [Zhu Y.]State Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology for Materials Technology, National Engineering Research Center for Fuel Cell and Hydrogen Source, Beijing University of Chemical Technology, Beijing, 100029, China
  • [ 2 ] [Gao S.]Australia Institute for Bioengineering and Nanotechnology (AIBN), The University of Queensland, Brisbane, 4072, QLD, Australia
  • [ 3 ] [Zhang S.]Australia Institute for Bioengineering and Nanotechnology (AIBN), The University of Queensland, Brisbane, 4072, QLD, Australia
  • [ 4 ] [Chen Y.]State Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology for Materials Technology, National Engineering Research Center for Fuel Cell and Hydrogen Source, Beijing University of Chemical Technology, Beijing, 100029, China
  • [ 5 ] [Liu P.]State Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology for Materials Technology, National Engineering Research Center for Fuel Cell and Hydrogen Source, Beijing University of Chemical Technology, Beijing, 100029, China
  • [ 6 ] [Meng H.]State Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology for Materials Technology, National Engineering Research Center for Fuel Cell and Hydrogen Source, Beijing University of Chemical Technology, Beijing, 100029, China
  • [ 7 ] [Luo Z.]Australia Institute for Bioengineering and Nanotechnology (AIBN), The University of Queensland, Brisbane, 4072, QLD, Australia
  • [ 8 ] [Chen X.]State Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology for Materials Technology, National Engineering Research Center for Fuel Cell and Hydrogen Source, Beijing University of Chemical Technology, Beijing, 100029, China
  • [ 9 ] [Wen Z.]State Key Laboratory of Structural Chemistry, and Fujian Provincial Key Laboratory of Materials and Techniques toward Hydrogen Energy, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fujian, 350002, China
  • [ 10 ] [Wen Z.]Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou, 350108, China
  • [ 11 ] [Wang L.]State Key Laboratory of Structural Chemistry, and Fujian Provincial Key Laboratory of Materials and Techniques toward Hydrogen Energy, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fujian, 350002, China
  • [ 12 ] [Wang L.]Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou, 350108, China
  • [ 13 ] [Wang L.]Fujian Key Laboratory of Green Extraction and High-Value Utilization of New Energy Metals, Fuzhou University, Fuzhou, China
  • [ 14 ] [Wang L.]Australia Institute for Bioengineering and Nanotechnology (AIBN), The University of Queensland, Brisbane, 4072, QLD, Australia
  • [ 15 ] [Wang L.]School of Chemical Engineering, The University of Queensland, Brisbane, 4072, QLD, Australia
  • [ 16 ] [Luo B.]Australia Institute for Bioengineering and Nanotechnology (AIBN), The University of Queensland, Brisbane, 4072, QLD, Australia
  • [ 17 ] [Zhou J.]State Key Laboratory of Chemical Resource Engineering, Beijing Key Laboratory of Electrochemical Process and Technology for Materials Technology, National Engineering Research Center for Fuel Cell and Hydrogen Source, Beijing University of Chemical Technology, Beijing, 100029, China

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Angewandte Chemie - International Edition

ISSN： 1433-7851

Year： 2025

1 6 . 1 0 0

JCR@2023

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ESI Highly Cited Papers on the List： 0 Unfold All

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