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author:

Cai, Junhu (Cai, Junhu.) [1] | Lai, Wenzong (Lai, Wenzong.) [2] | Chen, Yu (Chen, Yu.) [3] | Ye, Yun (Ye, Yun.) [4] | Xu, Sheng (Xu, Sheng.) [5] | Guo, Tailiang (Guo, Tailiang.) [6] | Chen, Enguo (Chen, Enguo.) [7]

Indexed by:

SCIE

Abstract:

Exceptional temperature sensitivity and the resulting luminescence response position perovskite materials as potent contenders in wearable sensing devices. However, the mechanisms driving temperature-induced fluorescence reversibility, especially across an ultrawide temperature range or at freezing temperatures, remain poorly understood. In this study, we systematically elucidate the mechanisms governing temperature-induced fluorescence reversibility in CsPbBr3/PS composite and astonishingly observe the reversible fluorescence enhancement under freezing temperatures for the first time. Elevated temperature-induced lattice phase transitions and freezing temperature-associated lattice distortions in CsPbBr3 can modulate the electrons' non-radiative recombination process, leading to temperature-dependent fluorescence quenching and enhancement, respectively. Notably, these structural perturbations can be reversed with temperature cycling, ensuring the reversibility of thermally induced fluorescence phenomena. Leveraging these insights, we develop a CsPbBr3/PS-based wearable temperature sensor that operates over an ultrawide range (263 K similar to 423 K) with high precision (error margin within +/- 10 %). Our findings highlight the significant breakthrough of CsPbBr3 in temperature sensing and wearable applications.

Keyword:

CsPbBr (3) Lattice distortion Phase transition Polystyrene Temperature sensing

Community:

  • [ 1 ] [Cai, Junhu]Fuzhou Univ, Coll Phys & Informat Engn, Natl & Local United Engn Lab Flat Panel Display Te, Fuzhou 350108, Fujian, Peoples R China
  • [ 2 ] [Lai, Wenzong]Fuzhou Univ, Coll Phys & Informat Engn, Natl & Local United Engn Lab Flat Panel Display Te, Fuzhou 350108, Fujian, Peoples R China
  • [ 3 ] [Chen, Yu]Fuzhou Univ, Coll Phys & Informat Engn, Natl & Local United Engn Lab Flat Panel Display Te, Fuzhou 350108, Fujian, Peoples R China
  • [ 4 ] [Ye, Yun]Fuzhou Univ, Coll Phys & Informat Engn, Natl & Local United Engn Lab Flat Panel Display Te, Fuzhou 350108, Fujian, Peoples R China
  • [ 5 ] [Xu, Sheng]Fuzhou Univ, Coll Phys & Informat Engn, Natl & Local United Engn Lab Flat Panel Display Te, Fuzhou 350108, Fujian, Peoples R China
  • [ 6 ] [Guo, Tailiang]Fuzhou Univ, Coll Phys & Informat Engn, Natl & Local United Engn Lab Flat Panel Display Te, Fuzhou 350108, Fujian, Peoples R China
  • [ 7 ] [Chen, Enguo]Fuzhou Univ, Coll Phys & Informat Engn, Natl & Local United Engn Lab Flat Panel Display Te, Fuzhou 350108, Fujian, Peoples R China
  • [ 8 ] [Ye, Yun]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China
  • [ 9 ] [Xu, Sheng]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China
  • [ 10 ] [Guo, Tailiang]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China
  • [ 11 ] [Chen, Enguo]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China

Reprint 's Address:

  • [Chen, Enguo]Fuzhou Univ, Coll Phys & Informat Engn, Natl & Local United Engn Lab Flat Panel Display Te, Fuzhou 350108, Fujian, Peoples R China

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Source :

NANO ENERGY

ISSN: 2211-2855

Year: 2025

Volume: 142

1 6 . 8 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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