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author:

Shi, Yanghui (Shi, Yanghui.) [1] | Yan, Xuan (Yan, Xuan.) [2] | Wang, Qiao (Wang, Qiao.) [3] | Wu, Jiawei (Wu, Jiawei.) [4] | Yan, Huaxiang (Yan, Huaxiang.) [5]

Indexed by:

SCIE

Abstract:

Per- and polyfluoroalkyl substances (PFAS) can persist and continuously affect the environment because of their innate thermal and chemical stability. The cut-off wall has emerged as a new and promising technology for pollution control at contaminated sites. This paper aims to investigate the migration of perfluorooctanesulfonic acid (PFOS) and perfluorooctanoic acid (PFOA) in a cut-off wall, aquifer and aquitard triple-domain system based on numerical simulation. The impacts of the PFAS concentration distribution, nonlinear and rate-limited adsorption and cut-off wall type are considered. The results show that the cut-off wall adsorption coefficient (K-dc) has the most considerable effect on system performance. Direct breakthrough rather than back-diffusion is the dominant failure mode when the K-dc values for PFOS and PFOA are lower than 15.4 mL/g and 7.8 mL/g, respectively. The GCL-enhanced cut-off wall (GCLW) is more suitable for installation than the composite GMB cut-off wall (GMBW) when the hole radius exceeds 1 m. Additionally, the GMBW is more effective at reducing the peak contaminant concentration than the GCLW when the head loss is > 1.9 m. This study may provide a scientific basis for the selection, installation and maintenance of cut-off walls under different conditions at PFAS contaminated sites.

Keyword:

Contaminant migration Cut-off wall PFAS Pollution management Two-domain adsorption model

Community:

  • [ 1 ] [Shi, Yanghui]Fuzhou Univ, Zijin Sch Geol & Min, Fuzhou 350108, Peoples R China
  • [ 2 ] [Yan, Xuan]Fuzhou Univ, Zijin Sch Geol & Min, Fuzhou 350108, Peoples R China
  • [ 3 ] [Yan, Huaxiang]Fuzhou Univ, Zijin Sch Geol & Min, Fuzhou 350108, Peoples R China
  • [ 4 ] [Shi, Yanghui]Univ Manchester, Sch Engn, Dept Mech Aerosp & Civil Engn, Manchester M13 9PL, England
  • [ 5 ] [Shi, Yanghui]Zhejiang Univ Co Ltd, Architectural Design & Res Inst, 148 Tianmushan Rd, Hangzhou 310058, Peoples R China
  • [ 6 ] [Wu, Jiawei]Zhejiang Univ Co Ltd, Architectural Design & Res Inst, 148 Tianmushan Rd, Hangzhou 310058, Peoples R China
  • [ 7 ] [Wang, Qiao]Hefei Univ Technol, Sch Resource & Environm Engn, Hefei 230009, Peoples R China

Reprint 's Address:

  • [Yan, Huaxiang]Fuzhou Univ, Zijin Sch Geol & Min, Fuzhou 350108, Peoples R China

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Source :

JOURNAL OF HAZARDOUS MATERIALS

ISSN: 0304-3894

Year: 2025

Volume: 494

1 2 . 2 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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