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author:

Liu, Wugang (Liu, Wugang.) [1] | Shi, Yao (Shi, Yao.) [2] | Hu, Yitu (Hu, Yitu.) [3] | Sui, Yanan (Sui, Yanan.) [4] | Qian, Gang (Qian, Gang.) [5] | Luo, Yu (Luo, Yu.) [6] | Duan, Xuezhi (Duan, Xuezhi.) [7] | Jiang, Lilong (Jiang, Lilong.) [8] | Zhou, Xinggui (Zhou, Xinggui.) [9]

Indexed by:

SCIE

Abstract:

Ammonia decomposition is a crucial pathway for hydrogen production, holding significant promise for sustainable and efficient energy generation. Initial investigations in this study reveal that internal diffusion limitations, influenced by the size of industrial catalyst particles, severely impact catalytic performance in an External Wall-Heated Reactor (EWHR), with smaller powders causing excessive pressure drop. The introduction of washcoated SiSiC foam effectively mitigates diffusion limitations, thereby enhancing the ammonia decomposition performance. In non-reactive conditions, the Internal Joule-Heated Reactor (IJHR) demonstrates remarkable thermal response and energy efficiency due to its in-situ Joule heating compared to the EWHR. For ammonia decomposition process, the IJHR also exhibits superior catalytic performance and lower energy consumption, achieving peak energy efficiency at 600 degrees C. The integration of IJHR with washcoated SiSiC foam represents an innovative breakthrough in hydrogen production via ammonia decomposition, aligning with the revolutionary design concept of IJHR to enhance efficiency and energy savings for industrial-scale applications.

Keyword:

Ammonia decomposition Energy efficiency Internal Joule-Heated Reactor Washcoated SiSiC foam

Community:

  • [ 1 ] [Liu, Wugang]East China Univ Sci & Technol, State Key Lab Chem Engn & Low Carbon Technol, Shanghai 200237, Peoples R China
  • [ 2 ] [Shi, Yao]East China Univ Sci & Technol, State Key Lab Chem Engn & Low Carbon Technol, Shanghai 200237, Peoples R China
  • [ 3 ] [Hu, Yitu]East China Univ Sci & Technol, State Key Lab Chem Engn & Low Carbon Technol, Shanghai 200237, Peoples R China
  • [ 4 ] [Sui, Yanan]East China Univ Sci & Technol, State Key Lab Chem Engn & Low Carbon Technol, Shanghai 200237, Peoples R China
  • [ 5 ] [Qian, Gang]East China Univ Sci & Technol, State Key Lab Chem Engn & Low Carbon Technol, Shanghai 200237, Peoples R China
  • [ 6 ] [Duan, Xuezhi]East China Univ Sci & Technol, State Key Lab Chem Engn & Low Carbon Technol, Shanghai 200237, Peoples R China
  • [ 7 ] [Zhou, Xinggui]East China Univ Sci & Technol, State Key Lab Chem Engn & Low Carbon Technol, Shanghai 200237, Peoples R China
  • [ 8 ] [Luo, Yu]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Fuzhou 350002, Peoples R China
  • [ 9 ] [Jiang, Lilong]Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Fuzhou 350002, Peoples R China

Reprint 's Address:

  • [Shi, Yao]East China Univ Sci & Technol, State Key Lab Chem Engn & Low Carbon Technol, Shanghai 200237, Peoples R China;;[Qian, Gang]East China Univ Sci & Technol, State Key Lab Chem Engn & Low Carbon Technol, Shanghai 200237, Peoples R China

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Source :

CHEMICAL ENGINEERING SCIENCE

ISSN: 0009-2509

Year: 2025

Volume: 315

4 . 1 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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