Indexed by:
Abstract:
A novel activated carbon (CCH-TS) derived from chitosan hydrogel (CH) coated tea saponin (TS) was prepared to investigate its removal performance for methylene blue (MB). CCH-TS was characterized by thermogravimetric analysis, field-emission scanning electron microscope, fourier transform infrared spectroscopy, X-ray diffraction, X-ray photoelectron spectroscopy, Brunauer-Emmett-Teller, and zeta potential analysis. The results showed that CCH-TS had a high specific area of 3504 m(2)/g with a large pore volume of 6.03 m(3)/g. In the batch mode adsorption experiments, the effects of initial pH values, adsorbent concentration, initial MB concentration and contact time, and adsorption temperature on the adsorption performance of CCH-TS for MB were studied. The experimental results were fitted by pseudo-first-order kinetic, pseudo-second-order kinetic and intra-particle diffusion models. Furthermore, Langmuir, Freundlich and Temkin isotherms were employed to analyze the equilibrium adsorption data. It was found that these data were fitted to Langmuir isotherm best with a maximum adsorption capacity of 604.10 mg/g, while pseudo-second-order kinetic model could describe the adsorption process more accurately. Thermodynamic analysis implied that the adsorption process was spontaneous and exothermic. Therefore, a facile one-step route to preparation of activated carbon with a high specific area and efficient dye removal ability was achieved.
Keyword:
Reprint 's Address:
Email:
Version:
Source :
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
ISSN: 2213-2929
Year: 2021
Issue: 3
Volume: 9
7 . 9 6 8
JCR@2021
7 . 4 0 0
JCR@2023
ESI Discipline: ENGINEERING;
ESI HC Threshold:105
JCR Journal Grade:1
CAS Journal Grade:2
Cited Count:
WoS CC Cited Count: 32
SCOPUS Cited Count: 36
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 4
Affiliated Colleges: