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author:

Lv, Yuancai (Lv, Yuancai.) [1] (Scholars:吕源财) | Ma, Jiachen (Ma, Jiachen.) [2] | Yu, Zhendong (Yu, Zhendong.) [3] | Liu, Shuting (Liu, Shuting.) [4] | Yang, Guifang (Yang, Guifang.) [5] | Liu, Yifan (Liu, Yifan.) [6] | Lin, Chunxiang (Lin, Chunxiang.) [7] (Scholars:林春香) | Ye, Xiaoxia (Ye, Xiaoxia.) [8] (Scholars:叶晓霞) | Shi, Yongqian (Shi, Yongqian.) [9] (Scholars:施永乾) | Liu, Minghua (Liu, Minghua.) [10]

Indexed by:

EI Scopus SCIE

Abstract:

Enriching and detecting the trace pollutants in actual matrices are critical to evaluating the water quality. Herein, a novel nanofibrous membrane, named PAN-SiO2@TpPa, was prepared by in situ growing & beta;-ketoenamine-linked covalent organic frameworks (COF-TpPa) on the aminated polyacrylonitrile (PAN) nanofibers, and adopted for enriching the trace polychlorinated biphenyls (PCBs) in various natural water body (river, lake and sea water) through the solid-phase micro-extraction (SPME) process. The resulted nanofibrous membrane owned abundant functional groups (-NH-, -OH and aromatic groups), outstandingly thermal and chemical stability, and excellent ability in extracting PCBs congeners. Based on the SPME process, the PCBs congeners could be quantitatively analyzed by the traditional gas chromatography (GC) method, with the satisfactory linear relationship (R2>0.99), low detection limit (LODs, 0.1-5 ng L-1), high enrichment factors (EFs, 2714-3949) and multiple recycling (>150 runs). Meanwhile, when PAN-SiO2@TpPa was adopted in the real water samples, the low matrix effects on the enrichment of PCBs at both 5 and 50 ng L-1 over PAN-SiO2@TpPa membrane firmly revealed the feasibility of enriching the trace PCBs in real water. Besides, the related mechanism of extracting PCBs on PANSiO2@TpPa mainly involved the synergistic effect of hydrophobic effect, 7C-7C stacking and hydrogen bonding.

Keyword:

Covalent organic frameworks Enrichment Nanofibrous membrane Solid -phase micro -extraction Trace pollutants

Community:

  • [ 1 ] [Lv, Yuancai]Fuzhou Univ, Coll Environm & Safety Engn, Fujian Prov Engn Res Ctr Rural Waste Recycling Tec, Dept Environm Sci & Engn, 2 Xueyuan Rd, Fuzhou 350116, Fujian, Peoples R China
  • [ 2 ] [Ma, Jiachen]Fuzhou Univ, Coll Environm & Safety Engn, Fujian Prov Engn Res Ctr Rural Waste Recycling Tec, Dept Environm Sci & Engn, 2 Xueyuan Rd, Fuzhou 350116, Fujian, Peoples R China
  • [ 3 ] [Yu, Zhendong]Fuzhou Univ, Coll Environm & Safety Engn, Fujian Prov Engn Res Ctr Rural Waste Recycling Tec, Dept Environm Sci & Engn, 2 Xueyuan Rd, Fuzhou 350116, Fujian, Peoples R China
  • [ 4 ] [Liu, Shuting]Fuzhou Univ, Coll Environm & Safety Engn, Fujian Prov Engn Res Ctr Rural Waste Recycling Tec, Dept Environm Sci & Engn, 2 Xueyuan Rd, Fuzhou 350116, Fujian, Peoples R China
  • [ 5 ] [Liu, Yifan]Fuzhou Univ, Coll Environm & Safety Engn, Fujian Prov Engn Res Ctr Rural Waste Recycling Tec, Dept Environm Sci & Engn, 2 Xueyuan Rd, Fuzhou 350116, Fujian, Peoples R China
  • [ 6 ] [Lin, Chunxiang]Fuzhou Univ, Coll Environm & Safety Engn, Fujian Prov Engn Res Ctr Rural Waste Recycling Tec, Dept Environm Sci & Engn, 2 Xueyuan Rd, Fuzhou 350116, Fujian, Peoples R China
  • [ 7 ] [Ye, Xiaoxia]Fuzhou Univ, Coll Environm & Safety Engn, Fujian Prov Engn Res Ctr Rural Waste Recycling Tec, Dept Environm Sci & Engn, 2 Xueyuan Rd, Fuzhou 350116, Fujian, Peoples R China
  • [ 8 ] [Shi, Yongqian]Fuzhou Univ, Coll Environm & Safety Engn, Fujian Prov Engn Res Ctr Rural Waste Recycling Tec, Dept Environm Sci & Engn, 2 Xueyuan Rd, Fuzhou 350116, Fujian, Peoples R China
  • [ 9 ] [Liu, Minghua]Fuzhou Univ, Coll Environm & Safety Engn, Fujian Prov Engn Res Ctr Rural Waste Recycling Tec, Dept Environm Sci & Engn, 2 Xueyuan Rd, Fuzhou 350116, Fujian, Peoples R China
  • [ 10 ] [Yang, Guifang]Putian Univ, Fujian Prov Key Lab Ecol Toxicol Effects & Control, Putian 351100, Peoples R China
  • [ 11 ] [Liu, Minghua]Putian Univ, Fujian Prov Key Lab Ecol Toxicol Effects & Control, Putian 351100, Peoples R China

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Source :

WATER RESEARCH

ISSN: 0043-1354

Year: 2023

Volume: 235

1 1 . 5

JCR@2023

1 1 . 5 0 0

JCR@2023

ESI Discipline: ENVIRONMENT/ECOLOGY;

ESI HC Threshold:33

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 11

SCOPUS Cited Count: 13

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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