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author：

Yang, Lin (Yang, Lin.) [1] | Fu, Yudong (Fu, Yudong.) [2] | Liu, Honghai (Liu, Honghai.) [3] | Nie, Qiaojun (Nie, Qiaojun.) [4] | Zhang, Ming (Zhang, Ming.) [5] | Shen, Zhongrong (Shen, Zhongrong.) [6]

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EI

Abstract：

Zinc　(Zn)　metal　anodes　have　been　extensively　investigated　in　aqueous　Zn-ion　batteries　(AZIBs).　Nevertheless,　severe　dendrite　issues　caused　by　uneven　ion　diffusion　and　Zn　deposition　greatly　influence　the　stability　and　safety　of　AZIBs.　Herein,　a　novel　three-electrode　tubular　cell　assembled　from　simple　materials　is　constructed　for　both　electrochemical　measurement　and　visual　characterization.　Measured　by　the　tubular　cell,　a　water-in-salt　electrolyte　(WiSE)　exhibits　excellent　ionic　conductivity　(33.29　mS　cm-1)　and　reduced　corrosivity,　which　is　prepared　by　incorporating　cellulose　and　polyethylene　glycol　(PEG)　into　concentrated　zinc　chloride　(ZnCl2)　solution.　The　results　reveal　that　the　functional　groups　of　cellulose　and　PEG　in　WiSE　can　regulate　the　solvation　structure　of　Zn2+,　thereby　alleviating　consecutive　side　reactions　and　inhibiting　the　formation　of　byproducts.　The　inherent　ion　channels　formed　by　the　polymer　chains　and　the　physical　barriers　constructed　by　PEG　on　the　Zn　surface　further　facilitated　the　uniform　deposition　of　Zn2+　along　the　(002)　crystal　plane,　enabling　the　Zn　symmetric　battery　to　achieve　an　ultralong　cycle　life　of　1000　h　at　a　current　density　of　2　mA　cm-2　©　2023　American　Chemical　Society.

Keyword：

Cellulose Chlorine compounds Deposition Electrochemical electrodes Electrolytes Ions Secondary batteries Zinc chloride

Community：

  • [ 1 ] [Yang, Lin]College of Furnishings and Industrial Design, Nanjing Forestry University, Nanjing; 210037, China
  • [ 2 ] [Yang, Lin]Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Nanjing Forestry University, Nanjing; 210037, China
  • [ 3 ] [Fu, Yudong]College of Furnishings and Industrial Design, Nanjing Forestry University, Nanjing; 210037, China
  • [ 4 ] [Fu, Yudong]Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Nanjing Forestry University, Nanjing; 210037, China
  • [ 5 ] [Fu, Yudong]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 6 ] [Liu, Honghai]College of Furnishings and Industrial Design, Nanjing Forestry University, Nanjing; 210037, China
  • [ 7 ] [Liu, Honghai]Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Nanjing Forestry University, Nanjing; 210037, China
  • [ 8 ] [Nie, Qiaojun]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 9 ] [Nie, Qiaojun]Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institutes, Chinese Academy of Sciences, Xiamen; 361021, China
  • [ 10 ] [Nie, Qiaojun]College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 11 ] [Zhang, Ming]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 12 ] [Zhang, Ming]Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institutes, Chinese Academy of Sciences, Xiamen; 361021, China
  • [ 13 ] [Shen, Zhongrong]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 14 ] [Shen, Zhongrong]Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institutes, Chinese Academy of Sciences, Xiamen; 361021, China

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Source ：

ACS Sustainable Chemistry and Engineering

Year： 2023

Issue： 28

Volume： 11

Page： 10311-10323

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WoS CC Cited Count：

SCOPUS Cited Count： 2

ESI Highly Cited Papers on the List： 0 Unfold All

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30 Days PV： 0

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