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author:

Zhou, Y. (Zhou, Y..) [1] | Yang, D. (Yang, D..) [2] | Jiang, G. (Jiang, G..) [3] | Teng, C. (Teng, C..) [4] | Zhang, Y. (Zhang, Y..) [5] (Scholars:张云霄) | Yao, T. (Yao, T..) [6]

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EI Scopus PKU CSCD

Abstract:

Barium titanate based dielectric ceramics have been widely used in science and technology, industry and daily life because of their good dielectric and positive temperature coefficient characteristics. Under the demands of emerging fields, it is of great significance to develop dielectric ceramic materials with low Curie temperature and high room temperature resistivity characteristics. Therefore, a ceramic material doped with different concentrations of yttrium oxide (Y2O3) with positive temperature coefficient (PTC), barium strontium titanate (Ba0.7Sr0.3TiO3, BST), was prepared by the conventional solid-state reaction. The physical and chemical properties of the samples are observed by X-ray diffraction and scanning electron microscope. The broadband dielectric spectrometer and resistivity-temperature measurement system are used to obtain the dielectric-temperature properties and resistivity-temperature characteristics of the samples, and a four-quadrant model is constructed to analyze the influence mechanism of yttrium (Y) on the dielectric-temperature properties and resistivity-temperature characteristics of the material. The results show that the relative permittivity and Curie temperature increase first and then decrease with the increase of Y2O3 content, while the resistivity at room temperature shows an opposite trend. The relative permittivity (>105) can be significantly increased by doping 0.0008 mol Y2O3, and has a lower Curie temperature (34.1 ℃) and a higher resistivity at room temperature (5.6×106 Ω·cm). The synergistic regulation of low Curie temperature and high resistivity characteristics is realized, which broadens the application range of PTC materials. © 2023 Science Press. All rights reserved.

Keyword:

barium strontium titanate Curie temperature dielectric-temperature properties resistivity at room temperature resistivity-temperature characteristics

Community:

  • [ 1 ] [Zhou Y.]The Wind Solar Storage Division of State Key Laboratory of Control and Simulation of Power System and Generation Equipment, School of Electrical Engineering, Xinjiang University, Urumqi, 830047, China
  • [ 2 ] [Zhou Y.]State Key Laboratory of Control and Simulation of Power System and Generation Equipment, Department of Electrical Engineering, Tsinghua University, Beijing, 100084, China
  • [ 3 ] [Yang D.]The Wind Solar Storage Division of State Key Laboratory of Control and Simulation of Power System and Generation Equipment, School of Electrical Engineering, Xinjiang University, Urumqi, 830047, China
  • [ 4 ] [Jiang G.]The Wind Solar Storage Division of State Key Laboratory of Control and Simulation of Power System and Generation Equipment, School of Electrical Engineering, Xinjiang University, Urumqi, 830047, China
  • [ 5 ] [Teng C.]College of Information Engineering, Zhejiang University of Technology, Hangzhou, 310023, China
  • [ 6 ] [Zhang Y.]College of Electrical Engineering and Automation, Fuzhou University, Fuzhou, 350108, China
  • [ 7 ] [Yao T.]State Key Laboratory of Control and Simulation of Power System and Generation Equipment, Department of Electrical Engineering, Tsinghua University, Beijing, 100084, China

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Source :

High Voltage Engineering

ISSN: 1003-6520

CN: 42-1239/TM

Year: 2023

Issue: 11

Volume: 49

Page: 4686-4694

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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