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author:

Qie, Yuan (Qie, Yuan.) [1] | Hu, Hailong (Hu, Hailong.) [2] (Scholars:胡海龙) | Yu, Kuibao (Yu, Kuibao.) [3] | Zhong, Chao (Zhong, Chao.) [4] | Ju, Songman (Ju, Songman.) [5] | Liu, Yanbing (Liu, Yanbing.) [6] | Guo, Tailiang (Guo, Tailiang.) [7] (Scholars:郭太良) | Li, Fushan (Li, Fushan.) [8] (Scholars:李福山)

Indexed by:

EI Scopus SCIE

Abstract:

The photolithographic patterning of fine quantum dot (QD) films is of great significance for the construction of QD optoelectronic device arrays. However, the photolithography methods reported so far either introduce insulating photoresist or manipulate the surface ligands of QDs, each of which has negative effects on device performance. Here, we report a direct photolithography strategy without photoresist and without engineering the QD surface ligands. Through cross-linking of the surrounding semiconductor polymer, QDs are spatially confined to the network frame of the polymer to form high-quality patterns. More importantly, the wrapped polymer incidentally regulates the energy levels of the emitting layer, which is conducive to improving the hole injection capacity while weakening the electron injection level, to achieve balanced injection of carriers. The patterned QD light-emitting diodes (with a pixel size of 1.5 mu m) achieve a high external quantum efficiency of 16.25% and a brightness of >1.4 x 10(5) cd/m(2). This work paves the way for efficient high-resolution QD light-emitting devices.

Keyword:

cross-linking direct photolithography high resolution light-emitting diode quantum dot

Community:

  • [ 1 ] [Qie, Yuan]Fuzhou Univ, Inst Optoelect Technol, Fuzhou 350116, Peoples R China
  • [ 2 ] [Hu, Hailong]Fuzhou Univ, Inst Optoelect Technol, Fuzhou 350116, Peoples R China
  • [ 3 ] [Yu, Kuibao]Fuzhou Univ, Inst Optoelect Technol, Fuzhou 350116, Peoples R China
  • [ 4 ] [Zhong, Chao]Fuzhou Univ, Inst Optoelect Technol, Fuzhou 350116, Peoples R China
  • [ 5 ] [Liu, Yanbing]Fuzhou Univ, Inst Optoelect Technol, Fuzhou 350116, Peoples R China
  • [ 6 ] [Guo, Tailiang]Fuzhou Univ, Inst Optoelect Technol, Fuzhou 350116, Peoples R China
  • [ 7 ] [Li, Fushan]Fuzhou Univ, Inst Optoelect Technol, Fuzhou 350116, Peoples R China
  • [ 8 ] [Ju, Songman]Dalian Univ, Coll Phys Sci & Technol, Dalian 116622, Peoples R China
  • [ 9 ] [Hu, Hailong]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China
  • [ 10 ] [Guo, Tailiang]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China
  • [ 11 ] [Li, Fushan]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China

Reprint 's Address:

  • 胡海龙 李福山

    [Hu, Hailong]Fuzhou Univ, Inst Optoelect Technol, Fuzhou 350116, Peoples R China;;[Li, Fushan]Fuzhou Univ, Inst Optoelect Technol, Fuzhou 350116, Peoples R China;;[Hu, Hailong]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China;;[Li, Fushan]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China

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Source :

NANO LETTERS

ISSN: 1530-6984

Year: 2024

Issue: 4

Volume: 24

Page: 1254-1260

9 . 6 0 0

JCR@2023

Cited Count:

WoS CC Cited Count: 3

SCOPUS Cited Count: 3

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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