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author:

Xu, Z. (Xu, Z..) [1] | Liu, M. (Liu, M..) [2] | Zhang, Y. (Zhang, Y..) [3] | Yang, F. (Yang, F..) [4]

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Scopus

Abstract:

The rapid progress in the development and implementation of smart electronics and flexible devices has stimulated the need to produce energy storage units of high efficiency at low cost. In this work, we use laser-induced graphene to construct in-plane micro-supercapacitors (μ-SCs) and delve into the effects of inter-finger spacing, finger width, deformation state, and temperature on the electrochemical performance of the μ-SCs with five different gel polymer electrolytes made from H2SO4, H3PO4, KOH, NaOH, and NaCl, respectively. The μ-SCs with the electrolyte from the PVA/H2SO4 gel polymer exhibit the best performance under bending and torsion. Increasing temperature causes a slight increase of the specific areal capacitance. Increasing the inter-finger spacing reduces the specific areal capacitance, and the finger width has a limited effect on the specific areal capacitance. The capacitance retention of the μ-SCs with the electrolyte from the PVA/H2SO4 gel polymer is 94.24 % of the initial capacitance after 10,000 electrochemical cycles at a scan rate of 0.1 V/s. The specific areal capacitance of integrated μ-SCs constructed from individual μ-SCs with the PVA/H2SO4 gel polymer is inversely proportional to the number of μ-SCs for the series connection and proportional to the number of μ-SCs for the parallel connection. This study provides a feasible method to produce flexible μ-SCs of high efficiency at low cost. © 2024 Elsevier Ltd

Keyword:

Gel polymer electrolytes In-plane micro-supercapacitor Interdigital structure Laser-induced graphene

Community:

  • [ 1 ] [Xu Z.]Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing, School of Mechanical Engineering and Automation, Fuzhou University, Fujian, Fuzhou, 350108, China
  • [ 2 ] [Xu Z.]State Key Laboratory of Intelligent Manufacturing Equipment and Technology, School of Mechanical Science and Engineering, Huazhong University of Science and Technology, Wuhan, 430074, China
  • [ 3 ] [Xu Z.]The Engineering Research Center for CAD/CAM of Fujian Universities, Putian University, Fujian, Putian, 351100, China
  • [ 4 ] [Liu M.]Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing, School of Mechanical Engineering and Automation, Fuzhou University, Fujian, Fuzhou, 350108, China
  • [ 5 ] [Zhang Y.]Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing, 400714, China
  • [ 6 ] [Yang F.]Materials Program, Department of Chemical and Materials Engineering, University of Kentucky, Lexington, 40506, KY, United States

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Source :

Journal of Energy Storage

ISSN: 2352-152X

Year: 2025

Volume: 105

8 . 9 0 0

JCR@2023

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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