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author:

Yang, Longwen (Yang, Longwen.) [1] | Du, Aochen (Du, Aochen.) [2] | Zheng, Xingke (Zheng, Xingke.) [3] | Ye, Yun (Ye, Yun.) [4] (Scholars:叶芸) | Chen, Enguo (Chen, Enguo.) [5] (Scholars:陈恩果) | Xu, Sheng (Xu, Sheng.) [6] (Scholars:徐胜) | Guo, Tailiang (Guo, Tailiang.) [7] (Scholars:郭太良)

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EI Scopus SCIE

Abstract:

All-inorganic perovskite quantum dots (PQDs) have excellent photoelectric performance, such as high photoluminescence quantum yield (PLQY), narrow full width at half-maximum (FWHM), and emission spectra covering the visible light wavelength. The emission color can be tuned over the full visible spectral region making them promising for white-light-emitting diodes (WLEDs). Further control over the optical and magnetic properties of PQDs can be achieved through doping of transition metal ions such as Mn2+ ions. In this paper, a rapid doping method is employed at room temperature by using strong-acid cation-exchange resin during the metal ions doping process, which shortens the doping time, and Mn:CsPb(Cl/Br)3 QDs were obtained. By controlling the reaction time between strong-acid cation-exchange resin and PQDs, we achieve different levels of manganese doping, resulting in a new, to the best of our knowledge, fluorescence peak at 600 nm. The introduction of strong-acid cation-exchange resin preserves the integrity of the PQD structure, while completing the doping within 30 min. Due to the low cost and mild reaction conditions of resin, it is expected that the Mn:CsPb(Cl/Br)3 QDs can be mass-produced in large quantities. In addition, in order to provide high-quality white light emission, and prevent anion exchange reactions when mixed with CsPbBr3 QDs, the CsPbBr3 QDs are coated with silicon. Finally, by combining ultraviolet-lightemitting diodes (UVLEDs) with the aforementioned PQD mixture, this paper successfully fabricates WLEDs and demonstrates its excellent photoelectric performance. The constructed WLEDs produce warm white light with a high color rendering index (CRI) of 91 and a high correlated color temperature (CCT) of 5966 K, and the luminous efficacy (LE) of WLEDs is 41 lmW-1. (c) 2024 Optica Publishing Group

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Community:

  • [ 1 ] [Yang, Longwen]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China
  • [ 2 ] [Du, Aochen]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China
  • [ 3 ] [Zheng, Xingke]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China
  • [ 4 ] [Ye, Yun]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China
  • [ 5 ] [Chen, Enguo]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China
  • [ 6 ] [Xu, Sheng]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China
  • [ 7 ] [Guo, Tailiang]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China
  • [ 8 ] [Yang, Longwen]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China
  • [ 9 ] [Du, Aochen]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China
  • [ 10 ] [Zheng, Xingke]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China
  • [ 11 ] [Ye, Yun]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China
  • [ 12 ] [Chen, Enguo]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China
  • [ 13 ] [Xu, Sheng]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China
  • [ 14 ] [Guo, Tailiang]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China

Reprint 's Address:

  • 叶芸

    [Ye, Yun]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China;;[Ye, Yun]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Peoples R China

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Source :

JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS

ISSN: 0740-3224

Year: 2024

Issue: 3

Volume: 41

Page: 809-819

1 . 8 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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