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Simplifying device structure for improving performance stability of colloidal quantum dots-based light emitting devices (QD-LEDs) is of importance for advanced photoelectric application. In this work, a QD-LED with ultrasimple structure is demonstrated, which is working in single-terminal-injection mode driven under alternating current field. The QD-LEDs are only composed of electrodes, insulator, and QD layer without any other organic functional layers, forming an ultra-thin structure of indium tin oxide (ITO)/Al2O3/QDs/Ag. The effect of the Al2O3 thickness on the device performance is discussed. Different from conventional devices, the QD-LEDs show high stability, which can work stably in air without any further sealing treatment and can work normally in the wide temperature range from -190 degrees C to 100 degrees C without obvious degration. Finally, the working mechanism related to the electron accumulation and interface-capture is proposed. We believe this work can extend the working mechanism model of QD-LEDs, provide guidance for improving QD-LEDs, and provide methods for obtaining advanced QD-based light-emitting technology.
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JOURNAL OF LUMINESCENCE
ISSN: 0022-2313
Year: 2025
Volume: 281
3 . 3 0 0
JCR@2023
Cited Count:
SCOPUS Cited Count:
ESI Highly Cited Papers on the List: 0 Unfold All
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30 Days PV: 0